Propulsion Mechanism of Catalytic Microjet Engines

We describe the propulsion mechanism of the catalytic microjet engines that are fabricated using rolled-up nanotech. Microjets have recently shown numerous potential applications in nanorobotics but currently there is a lack of an accurate theoretical model that describes the origin of the motion as well as the mechanism of self-propulsion. The geometric asymmetry of a tubular microjet leads to the development of a capillary force, which tends to propel a bubble toward the larger opening of the tube. Because of this motion in an asymmetric tube, there emerges a momentum transfer to the fluid. In order to compensate this momentum transfer, a jet force acting on the tube occurs. This force, which is counterbalanced by the linear drag force, enables tube velocities of the order of 100 μm/s. This mechanism provides a fundamental explanation for the development of driving forces that are acting on bubbles in tubular microjets.

[1]  Susana Campuzano,et al.  Micromachine-enabled capture and isolation of cancer cells in complex media. , 2011, Angewandte Chemie.

[2]  T. Mallouk,et al.  Powering nanorobots. , 2009, Scientific American.

[3]  Y. Mei,et al.  Dynamics of catalytic tubular microjet engines: dependence on geometry and chemical environment. , 2011, Nanoscale.

[4]  Wei Gao,et al.  Nano/Microscale motors: biomedical opportunities and challenges. , 2012, ACS nano.

[5]  Geoffrey A. Ozin,et al.  Dream Nanomachines , 2005 .

[6]  Oliver G. Schmidt,et al.  Versatile Approach for Integrative and Functionalized Tubes by Strain Engineering of Nanomembranes on Polymers , 2008 .

[7]  I. Cantat,et al.  Viscous force exerted on a foam at a solid boundary: Influence of the liquid fraction and of the bubble size , 2006, cond-mat/0609466.

[8]  Joseph Wang,et al.  Can man-made nanomachines compete with nature biomotors? , 2009, ACS nano.

[9]  Ayusman Sen,et al.  Fantastic voyage: designing self-powered nanorobots. , 2012, Angewandte Chemie.

[10]  O. Schmidt,et al.  Catalytic microtubular jet engines self-propelled by accumulated gas bubbles. , 2009, Small.

[11]  G. Ozin,et al.  Fuel for thought: chemically powered nanomotors out-swim nature's flagellated bacteria. , 2010, ACS nano.

[12]  Yanyan Cao,et al.  Catalytic nanomotors: autonomous movement of striped nanorods. , 2004, Journal of the American Chemical Society.

[13]  M. Manjare,et al.  Bubble driven quasioscillatory translational motion of catalytic micromotors. , 2012, Physical review letters.

[14]  Martin Pumera,et al.  Magnetic Control of Tubular Catalytic Microbots for the Transport, Assembly, and Delivery of Micro‐objects , 2010 .

[15]  Martin Pumera,et al.  Nanorobots: the ultimate wireless self-propelled sensing and actuating devices. , 2009, Chemistry, an Asian journal.

[16]  W. Xi,et al.  Self-propelled nanotools. , 2012, ACS nano.

[17]  Martin Pumera,et al.  Nanomotors: Magnetic Control of Tubular Catalytic Microbots for the Transport, Assembly, and Delivery of Micro-objects (Adv. Funct. Mater. 15/2010) , 2010 .

[18]  Martin Pumera,et al.  Nanomaterials meet microfluidics. , 2011, Chemical communications.

[19]  D. Bartels,et al.  Temperature Dependence of Oxygen Diffusion in H2O and D2O , 1996 .

[20]  Wei Gao,et al.  Catalytically propelled micro-/nanomotors: how fast can they move? , 2012, Chemical record.

[21]  Yiping Zhao,et al.  Bubble-Propelled Microjets: Model and Experiment , 2013 .