Generation of 30  fs pulses from a diode-pumped graphene mode-locked Yb:CaYAlO4 laser.

Stable 30 fs pulses centered at 1068 nm (less than 10 optical cycles) are demonstrated in a diode pumped Yb:CaYAlO4 laser by using high-quality chemical vapor deposited monolayer graphene as the saturable absorber. The mode-locked 8.43 optical-cycle pulses have a spectral bandwidth of ∼50  nm and a pulse repetition frequency of ∼113.5  MHz. To the best of our knowledge, this is the shortest pulse ever reported for graphene mode-locked lasers and mode-locked Yb-doped bulk lasers. Our experimental results demonstrate that graphene mode locking is a very promising practical technique for directly generating few-cycle optical pulses from a laser oscillator.

[1]  Jun Wang,et al.  Dissipative soliton operation of a diode pumped Yb:NaY(WO₄)₂ laser. , 2015, Optics express.

[2]  Liejia Qian,et al.  Wavelength-Versatile Graphene-Gold Film Saturable Absorber Mirror for Ultra-Broadband Mode-Locking of Bulk Lasers , 2014, Scientific Reports.

[3]  Evgeni Sorokin,et al.  Graphene mode-locked Cr:ZnS laser with 41 fs pulse duration. , 2014, Optics express.

[4]  Zhenhua Ni,et al.  Atomic‐Layer Graphene as a Saturable Absorber for Ultrafast Pulsed Lasers , 2009, 0910.5820.

[5]  U. Griebner,et al.  Carbon nanostructure-based saturable absorber mirror for a diode-pumped 500-MHz femtosecond Yb:KLu(WO4)2 laser. , 2014, Optics express.

[6]  S. Banerjee,et al.  Large-Area Synthesis of High-Quality and Uniform Graphene Films on Copper Foils , 2009, Science.

[7]  F Rotermund,et al.  Graphene mode-locked femtosecond Cr:ZnSe laser at 2500 nm. , 2013, Optics letters.

[8]  Fabian Rotermund,et al.  High-quality, large-area monolayer graphene for efficient bulk laser mode-locking near 1.25 μm. , 2011, Optics letters.

[9]  J G Fujimoto,et al.  Sub-two-cycle pulses from a Kerr-lens mode-locked Ti:sapphire laser. , 1999, Optics letters.

[10]  Jian Zhang,et al.  Passively Mode-Locked Tm:YAG Ceramic Laser Based on Graphene , 2015, IEEE Journal of Selected Topics in Quantum Electronics.

[11]  D. Tang,et al.  Graphene mode-locked femtosecond laser at 2 μm wavelength. , 2012, Optics letters.

[12]  Yeong Hwan Ahn,et al.  Efficient Mode-Locking of Sub-70-fs Ti:Sapphire Laser by Graphene Saturable Absorber , 2012 .

[13]  D. Tang,et al.  Femtosecond and continuous-wave laser performance of a diode-pumped Yb3+:CaYAlO4 laser. , 2011, Optics letters.

[14]  C. Hierold,et al.  Spatially resolved Raman spectroscopy of single- and few-layer graphene. , 2006, Nano letters.

[15]  Federico Pirzio,et al.  40-fs Yb3+:CaGdAlO4 laser pumped by a single-mode 350-mW laser diode. , 2012, Optics express.

[16]  P. Georges,et al.  32-fs Kerr-lens mode-locked Yb:CaGdAlO₄ oscillator optically pumped by a bright fiber laser. , 2014, Optics letters.

[17]  D. Wiersma,et al.  Optical pulse compression to 5 fs at a 1-MHz repetition rate. , 1997, Optics letters.

[18]  Randy Knize,et al.  Mode locking of ceramic Nd:yttrium aluminum garnet with graphene as a saturable absorber , 2010 .

[19]  Jing-Liang He,et al.  Graphene saturable absorber mirror for ultra-fast-pulse solid-state laser. , 2011, Optics letters.

[20]  D. Basko,et al.  Raman spectroscopy as a versatile tool for studying the properties of graphene. , 2013, Nature nanotechnology.

[21]  Zhipei Sun,et al.  Nanotube–Polymer Composites for Ultrafast Photonics , 2009 .

[22]  Andre K. Geim,et al.  Raman spectrum of graphene and graphene layers. , 2006, Physical review letters.

[23]  F. Kärtner,et al.  Self-starting 6.5-fs pulses from a Ti:sapphire laser. , 1997, Optics letters.

[24]  J. Didierjean,et al.  47-fs diode-pumped Yb3+:CaGdAlO4 laser. , 2006, Optics letters.

[25]  C. Berger,et al.  Ultrafast Relaxation of Excited Dirac Fermions in Epitaxial Graphene Using Optical Differential Transmission Spectroscopy , 2008 .

[26]  Valentin Petrov,et al.  Diode-pumped mode-locked Yb:YCOB laser generating 35 fs pulses. , 2011, Optics letters.

[27]  L Gallmann,et al.  Semiconductor saturable-absorber mirror assisted Kerr-lens mode-locked Ti:sapphire laser producing pulses in the two-cycle regime. , 1999, Optics letters.

[28]  G. Erbert,et al.  Graphene mode-locked femtosecond Yb:KLuW laser , 2012 .

[29]  J. Miller,et al.  Doping-induced changes in the saturable absorption of monolayer graphene , 2012 .

[30]  Federico Pirzio,et al.  Sub-100-fs Cr:YAG laser mode-locked by monolayer graphene saturable absorber. , 2013, Optics letters.

[31]  Kenji Torizuka,et al.  Sub-40-fs Pulses from a Diode-Pumped Kerr-Lens Mode-Locked Yb-Doped Yttrium Aluminum Garnet Laser , 2011 .

[32]  F. Krausz,et al.  Continuous-wave mode-locked Ti:sapphire laser focusable to 5 x 10(13) W/cm(2). , 1998, Optics letters.

[33]  Jun Xu,et al.  Crystal growth and spectroscopic properties of Yb:CaYAlO4 single crystal , 2010 .

[34]  U. Keller Recent developments in compact ultrafast lasers , 2003, Nature.

[35]  M. Tilsch,et al.  Semiconductor saturable absorber mirrors supporting sub-10-fs pulses , 1997 .

[36]  Michael G. Spencer,et al.  Measurement of Ultrafast Carrier Dynamics in Epitaxial Graphene , 2007, 0712.0119.

[37]  Katrin Paschke,et al.  42-fs diode-pumped Yb:Ca4YO(BO3)3 oscillator. , 2010, Optics express.