Fault sealing and caprock integrity for CO2 storage: an in situ injection experiment

Abstract. The success of geological carbon storage depends on the assurance of permanent containment for injected carbon dioxide (CO2) in the storage formation at depth. One of the critical elements of the safekeeping of CO2 is the sealing capacity of the caprock overlying the storage formation despite faults and/or fractures, which may occur in it. In this work, we present an ongoing injection experiment performed in a fault hosted in clay at the Mont Terri underground rock laboratory (NW Switzerland). The experiment aims to improve our understanding of the main physical and chemical mechanisms controlling (i) the migration of CO2 through a fault damage zone, (ii) the interaction of the CO2 with the neighboring intact rock, and (iii) the impact of the injection on the transmissivity in the fault. To this end, we inject CO2-saturated saline water in the top of a 3 m thick fault in the Opalinus Clay, a clay formation that is a good analog of common caprock for CO2 storage at depth. The mobility of the CO2 within the fault is studied at the decameter scale by using a comprehensive monitoring system. Our experiment aims to close the knowledge gap between laboratory and reservoir scales. Therefore, an important aspect of the experiment is the decameter scale and the prolonged duration of observations over many months. We collect observations and data from a wide range of monitoring systems, such as a seismic network, pressure temperature and electrical conductivity sensors, fiber optics, extensometers, and an in situ mass spectrometer for dissolved gas monitoring. The observations are complemented by laboratory data on collected fluids and rock samples. Here we show the details of the experimental concept and installed instrumentation, as well as the first results of the preliminary characterization. An analysis of borehole logging allows for identifying potential hydraulic transmissive structures within the fault zone. A preliminary analysis of the injection tests helped estimate the transmissivity of such structures within the fault zone and the pressure required to mechanically open such features. The preliminary tests did not record any induced microseismic events. Active seismic tomography enabled sharp imaging the fault zone.

[1]  Ipcc Global Warming of 1.5°C , 2022 .

[2]  L. Laloui,et al.  Experimental assessment of the hydro-mechanical behaviour of a shale caprock during CO2 injection , 2021 .

[3]  D. Giardini,et al.  Shale fault zone structure and stress dependent anisotropic permeability and seismic velocity properties (Opalinus Clay, Switzerland) , 2021 .

[4]  L. Stalker,et al.  CSIRO In-Situ Lab: A multi-pronged approach to surface gas and groundwater monitoring at geological CO2 storage sites , 2020, Chemical Geology.

[5]  F. Amann,et al.  In situ observation of helium and argon release during fluid-pressure-triggered rock deformation , 2020, Scientific Reports.

[6]  Y. Guglielmi,et al.  Coupled processes in clay during tunnel excavation , 2020 .

[7]  J. Rutqvist,et al.  Estimating perturbed stress from 3-D borehole displacements induced by fluid injection in fractured or faulted shales , 2020, Geophysical Journal International.

[8]  J. Rutqvist,et al.  Complexity of Fault Rupture and Fluid Leakage in Shale: Insights From a Controlled Fault Activation Experiment , 2020, Journal of Geophysical Research: Solid Earth.

[9]  F. Schopper,et al.  On the Variability of Pressure Propagation During Hydraulic Stimulation Based on Seismic Velocity Observations , 2020, Journal of Geophysical Research: Solid Earth.

[10]  L. Stalker,et al.  In-Situ Laboratory for CO2 controlled-release experiments and monitoring in a fault zone in Western Australia , 2019, ASEG Extended Abstracts.

[11]  A. Credoz,et al.  The CO2CRC Otway Controlled CO2 Release Experiment in a Fault: Geomechanical Characterisation Pre-Injection , 2019, Fifth International Conference on Fault and Top Seals.

[12]  R. Pini,et al.  Spatial Mapping of Fracture Aperture Changes With Shear Displacement Using X‐ray Computerized Tomography , 2019, Journal of Geophysical Research: Solid Earth.

[13]  J. Carrera,et al.  Induced seismicity in geologic carbon storage , 2019, Solid Earth.

[14]  J. Rutqvist,et al.  Joint opening or hydroshearing? Analyzing a fracture zone stimulation at Fenton Hill , 2019, Geothermics.

[15]  Reza Barati,et al.  A review of the current progress of CO2 injection EOR and carbon storage in shale oil reservoirs , 2019, Fuel.

[16]  S. Wiemer,et al.  CO2 Sequestration: Studying Caprock And Fault Sealing Integrity, The CS-D Experiment In Mont Terri , 2018, Fifth CO2 Geological Storage Workshop.

[17]  R. Miri,et al.  Fluid‐Rock Interactions in Clay‐Rich Seals , 2018, Geological Carbon Storage.

[18]  A. Ferretti,et al.  Monitoring and Modeling Caprock Integrity at the In Salah Carbon Dioxide Storage Site, Algeria , 2018, Geological Carbon Storage.

[19]  A. Busch,et al.  Migration and Leakage of CO 2 From Deep Geological Storage Sites , 2018, Geological Carbon Storage.

[20]  R. Schaa,et al.  The CO2CRC Otway shallow CO2 controlled release experiment: Preparation for Phase 2 , 2018, Energy Procedia.

[21]  H. Maurer,et al.  Imaging of radioactive-waste repository with vertically transversely isotropic full-waveform inversion , 2018, SEG Technical Program Expanded Abstracts 2018.

[22]  C. Collettini,et al.  Frictional Properties of Opalinus Clay: Implications for Nuclear Waste Storage , 2018 .

[23]  H. Hellevang Critical Factors for Considering CO2 Injectivity in Saline Aquifers , 2018 .

[24]  Philippe Renard,et al.  Hytool: an open source matlab toolbox for the interpretation of hydraulic tests using analytical solutions , 2017, J. Open Source Softw..

[25]  Stefan Finsterle,et al.  Inverse modeling of ground surface uplift and pressure with iTOUGH-PEST and TOUGH-FLAC: The case of CO2 injection at In Salah, Algeria , 2017, Comput. Geosci..

[26]  V. Vilarrasa,et al.  Caprock Integrity and Induced Seismicity from Laboratory and Numerical Experiments , 2017 .

[27]  J. Rutqvist,et al.  Long-term thermal effects on injectivity evolution during CO2 storage , 2017 .

[28]  Linda Stalker,et al.  What have we learned about CO2 leakage from field injection tests , 2017 .

[29]  Jonny Rutqvist,et al.  Can Fault Leakage Occur Before or Without Reactivation? Results from an in Situ Fault Reactivation Experiment at Mont Terri , 2017 .

[30]  V. Dietze,et al.  Litho- and biostratigraphy of the Opalinus Clay and bounding formations in the Mont Terri rock laboratory (Switzerland) , 2017, Swiss Journal of Geosciences.

[31]  F. Amann,et al.  High-resolution mini-seismic methods applied in the Mont Terri rock laboratory (Switzerland) , 2017, Swiss Journal of Geosciences.

[32]  Peter Connolly,et al.  Mont Terri rock laboratory, 20 years of research: introduction, site characteristics and overview of experiments , 2017, Swiss Journal of Geosciences.

[33]  E. Frank,et al.  Geomechanical behaviour of Opalinus Clay at multiple scales: results from Mont Terri rock laboratory (Switzerland) , 2017, Swiss Journal of Geosciences.

[34]  C. Nussbaum,et al.  Tectonic evolution around the Mont Terri rock laboratory, northwestern Swiss Jura: constraints from kinematic forward modelling , 2017, Swiss Journal of Geosciences.

[35]  D. Jaeggi,et al.  Tectonic structure of the “Main Fault” in the Opalinus Clay, Mont Terri rock laboratory (Switzerland) , 2017, Swiss Journal of Geosciences.

[36]  M. Brennwald,et al.  A Portable and Autonomous Mass Spectrometric System for On-Site Environmental Gas Analysis. , 2016, Environmental science & technology.

[37]  Jonny Rutqvist,et al.  Fault activation and induced seismicity in geological carbon storage – Lessons learned from recent modeling studies , 2016 .

[38]  T. Daley,et al.  Estimation of rock frame weakening using time-lapse crosswell: The Frio brine pilot project , 2016 .

[39]  Jean-Charles Manceau,et al.  Well integrity assessment by a 1:1 scale wellbore experiment: Exposition to dissolved CO2 and overcoring , 2016 .

[40]  Scott Thomas Broome,et al.  Effects of CO2 on mechanical variability and constitutive behavior of the Lower Tuscaloosa Formation, Cranfield Injection Site, USA , 2016 .

[41]  G Rother,et al.  Observational evidence confirms modelling of the long-term integrity of CO2-reservoir caprocks , 2016, Nature Communications.

[42]  M. Voutilainen,et al.  The Internal Architecture and Permeability Structures of Faults in Shale Formations , 2016 .

[43]  Muriel Cozier,et al.  The UN COP21 Climate Change Conference and the role of CCS , 2015 .

[44]  S. Noirez,et al.  The DEMO-CO2 project: A vadose zone CO2 and tracer leakage field experiment , 2015 .

[45]  J. Carrera,et al.  Geologic carbon storage is unlikely to trigger large earthquakes and reactivate faults through which CO2 could leak , 2015, Proceedings of the National Academy of Sciences.

[46]  O. Pfiffner Geology of the Alps , 2014 .

[47]  J. Rutqvist,et al.  Effects of fault‐zone architecture on earthquake magnitude and gas leakage related to CO2 injection in a multi‐layered sedimentary system , 2014 .

[48]  M. Lebedev,et al.  A laboratory study of the elastic and anelastic properties of the sandstone flooded with supercritical CO2 at seismic frequencies , 2014 .

[49]  Ruben Juanes,et al.  Coupled Modeling of Multiphase Flow and Fault Poromechanics During Geologic CO2 Storage , 2014 .

[50]  A. Bauer,et al.  The effect of CO2 on the mechanical properties of the Captain Sandstone: Geological storage of CO2 at the Goldeneye field (UK) , 2013 .

[51]  Susan D. Hovorka,et al.  Monitoring a large-volume injection at Cranfield, Mississippi—Project design and recommendations , 2013 .

[52]  C. Tsang,et al.  ISRM Suggested Method for Step-Rate Injection Method for Fracture In-Situ Properties (SIMFIP): Using a 3-Components Borehole Deformation Sensor , 2013, Rock Mechanics and Rock Engineering.

[53]  S. Durucan,et al.  A Coupled Reservoir Simulation-geomechanical Modelling Study of the CO2 Injection-induced Ground Surface Uplift Observed at Krechba, in Salah , 2013 .

[54]  Jonny Rutqvist,et al.  Modeling of deep fracture zone opening and transient ground surface uplift at KB-502 CO2 injection well, In Salah, Algeria , 2013 .

[55]  Steven M Gorelick,et al.  Earthquake triggering and large-scale geologic storage of carbon dioxide , 2012, Proceedings of the National Academy of Sciences.

[56]  Jonny Rutqvist,et al.  The Geomechanics of CO2 Storage in Deep Sedimentary Formations , 2012, Geotechnical and Geological Engineering.

[57]  G. Dresen,et al.  Source Parameters of Picoseismicity Recorded at Mponeng Deep Gold Mine, South Africa: Implications for Scaling Relations , 2011 .

[58]  Philip Ringrose,et al.  Geomechanical Response to CO2 Injection at Krechba, InSalah, Algeria , 2011 .

[59]  Christophe Nussbaum,et al.  Analysis of tectonic structures and excavation induced fractures in the Opalinus Clay, Mont Terri underground rock laboratory (Switzerland) , 2011 .

[60]  Jonny Rutqvist,et al.  Status of the TOUGH-FLAC simulator and recent applications related to coupled fluid flow and crustal deformations , 2011, Comput. Geosci..

[61]  S. Vialle,et al.  Laboratory measurements of elastic properties of carbonate rocks during injection of reactive CO2‐saturated water , 2011 .

[62]  Zoe K. Shipton,et al.  A review of recent developments concerning the structure, mechanics and fluid flow properties of fault zones , 2010 .

[63]  Toby Aiken,et al.  Geological storage of CO2 in saline aquifers—A review of the experience from existing storage operations , 2010 .

[64]  D. Gibert,et al.  Anisotropy of electrical conductivity of the excavation damaged zone in the Mont Terri Underground Rock Laboratory , 2010 .

[65]  Baojun Bai,et al.  Characteristics of CO2 sequestration in saline aquifers , 2010 .

[66]  Don W. Vasco,et al.  Satellite‐based measurements of surface deformation reveal fluid flow associated with the geological storage of carbon dioxide , 2010 .

[67]  P. Aagaard,et al.  Caprock interaction with CO2: a laboratory study of reactivity of shale with supercritical CO2 and brine mixtures at 250°C and 110bars , 2011 .

[68]  Anthony Credoz,et al.  Experimental and modeling study of geochemical reactivity between clayey caprocks and CO2 in geological storage conditions , 2009 .

[69]  D. Gibert,et al.  Seismic tomography of the Excavation Damaged Zone of the Gallery 04 in the Mont Terri Rock Laboratory , 2008 .

[70]  François Renard,et al.  Enhanced deformation of limestone and sandstone in the presence of high pCO2 fluids , 2007 .

[71]  D. Janecky,et al.  Experimental evaluation of mixed fluid reactions between supercritical carbon dioxide and NaCl brine: Relevance to the integrity of a geologic carbon repository , 2005 .

[72]  Paul Marschall,et al.  Characterisation of Gas Transport Properties of the Opalinus Clay, a Potential Host Rock Formation for Radioactive Waste Disposal , 2005 .

[73]  Paul Bossart,et al.  Geological and hydraulic characterisation of the excavation disturbed zone in the Opalinus Clay of the Mont Terri Rock Laboratory , 2002 .

[74]  Tsuyoshi Ishida,et al.  Acoustic emission monitoring of hydraulic fracturing in laboratory and field , 2001 .

[75]  P. Bossart,et al.  The Mont Terri rock laboratory, a new international research project in a Mesozoic shale formation, in Switzerland , 1999 .

[76]  A. Green,et al.  Refraction tomography over a buried waste disposal site , 1998 .

[77]  T. Mukerji,et al.  The Rock Physics Handbook , 1998 .

[78]  James P. Evans,et al.  Fault zone architecture and permeability structure , 1996 .

[79]  C. Neuzil On conducting the modified ‘Slug’ test in tight formations , 1982 .

[80]  Review of Current Progress , 1969 .

[81]  J. D. Bredehoeft,et al.  Response of a finite-diameter well to an instantaneous charge of water. Paper No. H-21 , 1966 .

[82]  S. W. Lohman,et al.  Nonsteady flow to a well of constant drawdown in an extensive aquifer , 1952 .