A global model for the afterglow of pure argon and of argon with negatively charged dust particles

Zero-dimensional, space-averaged global models of argon dust-free and dusty afterglow plasmas are developed, which describe the time behaviour of electron ne(t) and Ar* metastable nm(t) densities. The theoretical description is based on the assumption that the free electron density is smaller than the dust charge density. In pure argon, fairly good agreement with the experimentally measured densities and their decay times in the afterglow is obtained when the electron energy loss term to the chamber walls is included in the electron energy balance equation. In dusty plasma afterglow, the agreement between theory and experiment is less satisfactory. The calculated metastable density is 3 times smaller than the measured one and the electron decay is much faster in the late afterglows. The difference should probably arise from the assumption that the electron energy distribution function is Maxwellian. Different sources of secondary electrons in the dusty plasma afterglow are analysed. Comparison of the model with experimental results of argon dusty plasma suggests that the metastable pooling could be the source of the experimentally observed electron density increase in the early afterglow but electron generation from metastable–dust interactions cannot be fully discarded.

[1]  I. Stefanović,et al.  FAST TRACK COMMUNICATION: The influence of C2H2 and dust formation on the time dependence of metastable argon density in pulsed plasmas , 2010 .

[2]  P. Shukla,et al.  Colloquium: fundamentals of dust-plasma interactions , 2009 .

[3]  L. Couëdel,et al.  Influence of the ambipolar-to-free diffusion transition on dust particle charge in a complex plasma afterglow , 2008 .

[4]  I. Stefanović,et al.  Secondary electron emission of carbonaceous dust particles. , 2006, Physical review. E, Statistical, nonlinear, and soft matter physics.

[5]  L. Couëdel,et al.  Residual dust charges in discharge afterglow. , 2006, Physical review. E, Statistical, nonlinear, and soft matter physics.

[6]  I. Stefanović,et al.  The response of a capacitively coupled discharge to the formation of dust particles: Experiments and modeling , 2006 .

[7]  A. Kudryavtsev,et al.  Nonlocal effects in a bounded afterglow plasma with fast electrons , 2006, IEEE Transactions on Plasma Science.

[8]  I. Stefanović,et al.  Anomalous behaviour of the electron density in a pulsed complex plasma , 2006 .

[9]  Gregor E. Morfill,et al.  Complex (dusty) plasmas: current status, open issues, perspectives , 2005 .

[10]  G. Morfill,et al.  Particle charge in the bulk of gas discharges. , 2005, Physical review. E, Statistical, nonlinear, and soft matter physics.

[11]  Luís L Alves,et al.  An update of argon inelastic cross sections for plasma discharges , 2005 .

[12]  Jae Koo Lee,et al.  Particle-in-cell simulation of gas breakdown in microgaps , 2004, physics/0409131.

[13]  M. Yu,et al.  Molecular Dynamics Simulation of Dust Clusters in Plasmas , 2005 .

[14]  A. Piel,et al.  Dust Coulomb balls: three-dimensional plasma crystals. , 2004, Physical review letters.

[15]  L. Boufendi,et al.  Experimental investigations of void dynamics in a dusty discharge , 2004 .

[16]  Kostya Ostrikov,et al.  Dynamic self-organization phenomena in complex ionized gas systems : new paradigms and technological aspects , 2004 .

[17]  V. Tsytovich,et al.  Kinetic theory of dusty plasmas. V. The hydrodynamic equations , 2004 .

[18]  J. Allen,et al.  The floating potential of spherical probes and dust grains. II: Orbital motion theory , 2003, Journal of Plasma Physics.

[19]  Shuyan Xu,et al.  Nanopowder management and control of plasma parameters in electronegative SiH4 plasmas , 2003 .

[20]  I. Stefanović,et al.  Infrared fingerprints and periodic formation of nanoparticles in Ar/C2H2 plasmas , 2003 .

[21]  J. Goree,et al.  Decharging of complex plasmas: first kinetic observations. , 2003, Physical review letters.

[22]  A. Bouchoule,et al.  Industrial developments of scientific insights in dusty plasmas , 2002 .

[23]  S. Garaj,et al.  Field emission properties of carbon nanohorn films , 2002 .

[24]  Uwe Kortshagen,et al.  Experimental study of diffusive cooling of electrons in a pulsed inductively coupled plasma. , 2002, Physical review. E, Statistical, nonlinear, and soft matter physics.

[25]  J. Goree,et al.  Three-dimensional strongly coupled plasma crystal under gravity conditions. , 2000, Physical review letters.

[26]  M. Childs,et al.  Plasma charge-density ratios in a dusty plasma , 2000 .

[27]  J. Goree,et al.  Condensed Plasmas under Microgravity , 1999 .

[28]  U. Kortshagen,et al.  Modeling of particulate coagulation in low pressure plasmas. , 1999, Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics.

[29]  L. Overzet,et al.  Effect of metastable atom reactions on the electron energy probability functions in afterglows , 1998 .

[30]  Sumio Ashida,et al.  Spatially averaged (global) model of time modulated high density argon plasmas , 1995 .

[31]  A. Bouchoule,et al.  High concentration effects in dusty plasmas , 1994 .

[32]  J. Rabalais Low energy ion-surface interactions , 1994 .

[33]  K. E. Greenberg,et al.  Electron and metastable densities in parallel-plate radio-frequency discharges , 1993 .

[34]  D. J. Economou,et al.  Fluid simulations of glow discharges: Effect of metastable atoms in argon , 1993 .

[35]  Tachibana Excitation of the 1s5,1s4, 1s3, and 1s2 levels of argon by low-energy electrons. , 1986, Physical review. A, General physics.

[36]  C. M. Ferreira,et al.  Populations in the metastable and the resonance levels of argon and stepwise ionization effects in a low‐pressure argon positive column , 1985 .

[37]  R. Gerber,et al.  Ambipolar-to-Free Diffusion: The Temporal Behavior of the Electrons and Ions , 1973 .

[38]  R. Freiberg,et al.  MICROWAVE INVESTIGATION OF THE TRANSITION FROM AMBIPOLAR TO FREE DIFFUSION IN AFTERGLOW PLASMAS. , 1968 .

[39]  M. A. Biondi Studies of the Mechanism of Electron-Ion Recombination. I , 1963 .

[40]  P. J. Walsh,et al.  Effect of Simultaneous Doppler and Collision Broadening and of Hyperfine Structure on the Imprisonment of Resonance Radiation , 1959 .

[41]  M. A. Biondi Ionization by the Collision of Pairs of Metastable Atoms , 1951 .

[42]  R. Newton Ejection of Electrons by Ions at High Fields , 1948 .