Numerical analysis of mixing enhancement for micro-electroosmotic flow

Micro-electroosmotic flow is usually slow with negligible inertial effects and diffusion-based mixing can be problematic. To gain an improved understanding of electroosmotic mixing in microchannels, a numerical study has been carried out for channels patterned with wall blocks, and channels patterned with heterogeneous surfaces. The lattice Boltzmann method has been employed to obtain the external electric field, electric potential distribution in the electrolyte, the flow field, and the species concentration distribution within the same framework. The simulation results show that wall blocks and heterogeneous surfaces can significantly disturb the streamlines by fluid folding and stretching leading to apparently substantial improvements in mixing. However, the results show that the introduction of such features can substantially reduce the mass flow rate and thus effectively prolongs the available mixing time when the flow passes through the channel. This is a non-negligible factor on the effectiveness o...

[1]  Zhenhua Chai,et al.  Study of electro-osmotic flows in microchannels packed with variable porosity media via lattice boltzmann method , 2007 .

[2]  Harold T. Evensen,et al.  Automated fluid mixing in glass capillaries , 1998 .

[3]  Liqing Ren,et al.  Electroosmotic flow in heterogeneous microchannels , 2001 .

[4]  L. Fu,et al.  Analysis of electroosmotic flow with step change in zeta potential. , 2003, Journal of colloid and interface science.

[5]  F. Toschi,et al.  Surface roughness-hydrophobicity coupling in microchannel and nanochannel flows. , 2006, Physical review letters.

[6]  J. Santiago Electroosmotic flows in microchannels with finite inertial and pressure forces. , 2001, Analytical chemistry.

[7]  G. Whitesides,et al.  Patterning electro-osmotic flow with patterned surface charge. , 2000, Physical review letters.

[8]  W. Tao,et al.  Thermal boundary condition for the thermal lattice Boltzmann equation. , 2005, Physical review. E, Statistical, nonlinear, and soft matter physics.

[9]  D. Erickson,et al.  Influence of Surface Heterogeneity on Electrokinetically Driven Microfluidic Mixing , 2002 .

[10]  R. J. Hunter,et al.  Zeta Potential in Colloid Science , 1981 .

[11]  Moran Wang,et al.  Lattice Poisson-Boltzmann simulations of electro-osmotic flows in microchannels. , 2006, Journal of colloid and interface science.

[12]  Q. Zou,et al.  On pressure and velocity boundary conditions for the lattice Boltzmann BGK model , 1995, comp-gas/9611001.

[13]  Wen-Quan Tao,et al.  Field synergy principle for enhancing convective heat transfer--its extension and numerical verifications , 2002 .

[14]  L. Biferale,et al.  Mesoscopic modelling of heterogeneous boundary conditions for microchannel flows , 2005, Journal of Fluid Mechanics.

[15]  D. Kwok,et al.  Lattice Boltzmann model of microfluidics in the presence of external forces. , 2003, Journal of colloid and interface science.

[16]  Ruey-Jen Yang,et al.  Computational analysis of electrokinetically driven flow mixing in microchannels with patterned blocks , 2004 .

[17]  L. Luo,et al.  Theory of the lattice Boltzmann method: From the Boltzmann equation to the lattice Boltzmann equation , 1997 .

[18]  Ya-Ling He,et al.  Electroosmotic flow and mixing in microchannels with the lattice Boltzmann method , 2006 .

[19]  Carolyn L. Ren,et al.  Improved understanding of the effect of electrical double layer on pressure-driven flow in microchannels , 2005 .

[20]  I. Puri,et al.  Lattice Boltzmann method simulation of electroosmotic stirring in a microscale cavity , 2008 .

[21]  Tom van de Goor,et al.  Modeling Flow Profiles and Dispersion in Capillary Electrophoresis with Nonuniform .zeta. Potential , 1994 .

[22]  Xiaoyi He,et al.  Lattice Boltzmann simulation of electrochemical systems , 2000 .

[23]  Ajdari,et al.  Electro-osmosis on inhomogeneously charged surfaces. , 1995, Physical review letters.

[24]  Y. Qian,et al.  Lattice BGK Models for Navier-Stokes Equation , 1992 .

[25]  Sauro Succi,et al.  Electrorheology in nanopores via lattice Boltzmann simulation. , 2004, The Journal of chemical physics.

[26]  Shiyi Chen,et al.  LATTICE BOLTZMANN METHOD FOR FLUID FLOWS , 2001 .

[27]  Shizhi Qian,et al.  A chaotic electroosmotic stirrer. , 2002, Analytical chemistry.

[28]  Dinan Wang,et al.  Modeling of Electrokinetically Driven Flow Mixing Enhancement in Microchannels with Patterned Heterogeneous Surface and Blocks , 2007 .

[29]  R. Benzi,et al.  The lattice Boltzmann equation: theory and applications , 1992 .

[30]  Baoming Li,et al.  Electrokinetic microfluidic phenomena by a lattice Boltzmann model using a modified Poisson-Boltzmann equation with an excluded volume effect. , 2004, The Journal of chemical physics.

[31]  Howard H. Hu,et al.  Numerical simulation of electroosmotic flow. , 1998, Analytical chemistry.

[32]  T. Kenny,et al.  Electroosmotic capillary flow with nonuniform zeta potential , 2000, Analytical Chemistry.

[33]  Zhaoli Guo,et al.  A lattice Boltzmann algorithm for electro-osmotic flows in microfluidic devices. , 2005, The Journal of chemical physics.