Thermal fluctuations in artificial spin ice.

Artificial spin ice systems have been proposed as a playground for the study of monopole-like magnetic excitations, similar to those observed in pyrochlore spin ice materials. Currents of magnetic monopole excitations have been observed, demonstrating the possibility for the realization of magnetic-charge-based circuitry. Artificial spin ice systems that support thermal fluctuations can serve as an ideal setting for observing dynamical effects such as monopole propagation and as a potential medium for magnetricity investigations. Here, we report on the transition from a frozen to a dynamic state in artificial spin ice with a square lattice. Magnetic imaging is used to determine the magnetic state of the islands in thermal equilibrium. The temperature-induced onset of magnetic fluctuations and excitation populations are shown to depend on the lattice spacing and related interaction strength between islands. The excitations are described by Boltzmann distributions with their factors in the frozen state relating to the blocking temperatures of the array. Our results provide insight into the design of thermal artificial spin ice arrays where the magnetic charge density and response to external fields can be studied in thermal equilibrium.

[1]  Dominique Mailly,et al.  Experimental evidence of the Neel-Brown model of magnetization reversal , 1997 .

[2]  Andrea Taroni,et al.  Melting artificial spin ice , 2012 .

[3]  S. Bramwell,et al.  GEOMETRICAL FRUSTRATION IN THE FERROMAGNETIC PYROCHLORE HO2TI2O7 , 1997 .

[4]  Laura J. Heyderman,et al.  Real-space observation of emergent magnetic monopoles and associated Dirac strings in artificial kagome spin ice , 2011 .

[5]  R. Chopdekar,et al.  Thermalized ground state of artificial kagome spin ice building blocks , 2012 .

[6]  A. Libál,et al.  Realizing colloidal artificial ice on arrays of optical traps. , 2006, Physical review letters.

[7]  Tuning magnetic frustration of nanomagnets in triangular-lattice geometry , 2008, 0812.4468.

[8]  R. Cowburn,et al.  Room temperature magnetic quantum cellular automata , 2000, Science.

[9]  L. Pauling The Structure and Entropy of Ice and of Other Crystals with Some Randomness of Atomic Arrangement , 1935 .

[10]  R. Moessner,et al.  Magnetic monopoles in spin ice , 2007, Nature.

[11]  W. Kleemann,et al.  TOPICAL REVIEW: Supermagnetism , 2009 .

[12]  Michel J. P. Gingras,et al.  Spin Ice State in Frustrated Magnetic Pyrochlore Materials , 2001, Science.

[13]  Laura J. Heyderman,et al.  Exploring hyper-cubic energy landscapes in thermally active finite artificial spin-ice systems , 2013, Nature Physics.

[14]  S. Calder,et al.  Measurement of the charge and current of magnetic monopoles in spin ice , 2009, Nature.

[15]  S. Bramwell,et al.  Creation and measurement of long-lived magnetic monopole currents in spin ice , 2011 .

[16]  J. W. Stout,et al.  The Entropy of Water and the Third Law of Thermodynamics. The Heat Capacity of Ice from 15 to 273°K. , 1936 .

[17]  A Stein,et al.  Disorder strength and field-driven ground state domain formation in artificial spin ice: experiment, simulation, and theory. , 2011, Physical review letters.

[18]  Gia-Wei Chern,et al.  Crystallites of magnetic charges in artificial spin ice , 2013, Nature.

[19]  L. F. Cohen,et al.  Direct observation of magnetic monopole defects in an artificial spin-ice system , 2010 .

[20]  R. Stamps,et al.  Artificial ferroic systems: novel functionality from structure, interactions and dynamics , 2013, Journal of physics. Condensed matter : an Institute of Physics journal.

[21]  Aaron Stein,et al.  Thermal ground-state ordering and elementary excitations in artificial magnetic square ice , 2011 .

[22]  A. Taroni,et al.  Dimensionality and confinement effects in δ-doped Pd(Fe) layers , 2010, Journal of physics. Condensed matter : an Institute of Physics journal.

[23]  G. Wysin,et al.  Dynamics and hysteresis in square lattice artificial spin ice , 2012, 1208.6557.

[24]  Paolo Vavassori,et al.  Exploring thermally induced states in square artificial spin-ice arrays , 2013 .

[25]  Lu-ning,et al.  Observation of antiferromagnetic domains in epitaxial thin films , 2000, Science.

[26]  A. Scholl,et al.  Direct observation of thermal relaxation in artificial spin ice. , 2013, Physical review letters.

[27]  J. Osborn Demagnetizing Factors of the General Ellipsoid , 1945 .

[28]  Roderich Moessner,et al.  Colloquium: Artificial spin ice : Designing and imaging magnetic frustration , 2013 .

[29]  A Imre,et al.  Majority Logic Gate for Magnetic Quantum-Dot Cellular Automata , 2006, Science.

[30]  V. Crespi,et al.  Artificial ‘spin ice’ in a geometrically frustrated lattice of nanoscale ferromagnetic islands , 2006, Nature.

[31]  Ludovic D. C. Jaubert,et al.  Monopole and Dirac string Dynamics in Spin Ice , 2009, 0903.1074.