Effect of diffusion on residence time distribution in chaotic channel flow

We consider the residence time distribution (RTD) of a liquid flowing through a spatially periodic channel. It is shown that chaotic advection significantly reduces deviation of the RTD which then consist of two parts: the main pulse which does not depend on the Peclet number and a long tail which is formed in the near-boundary layer, where the advection is weak. Boundary layer approximation provides the dependence of the statistical moments of the RTD on Peclet number. It is shown that the length of the tail increases with Pe, while its mass decreases. The numerical results support the theoretical findings.

[1]  A. Guzmán,et al.  Dynamical flow characterization of transitional and chaotic regimes in converging–diverging channels , 1996, Journal of Fluid Mechanics.

[2]  C. Y. Kong,et al.  Chromatographic impulse response technique with curve fitting to measure binary diffusion coefficients and retention factors using polymer-coated capillary columns. , 2004, Journal of chromatography. A.

[3]  Paul Watts,et al.  Benchmarking of Microreactor Applications , 2004 .

[4]  P. V. Danckwerts Continuous flow systems , 1953 .

[5]  P. Legentilhomme,et al.  Residence time distribution of a purely viscous non-Newtonian fluid in helically coiled or spatially chaotic flows , 2006 .

[6]  H. Aref Stirring by chaotic advection , 1984, Journal of Fluid Mechanics.

[7]  Anthony Leonard,et al.  Diffusion of a passive scalar from a no-slip boundary into a two-dimensional chaotic advection field , 1998, Journal of Fluid Mechanics.

[8]  António A. Vicente,et al.  Residence times and mixing of a novel continuous oscillatory flow screening reactor , 2004 .

[9]  Nam-Trung Nguyen,et al.  Micromixers?a review , 2005 .

[10]  A. Boozer,et al.  Finite time Lyapunov exponent and advection-diffusion equation , 1996 .

[11]  J. Ottino The Kinematics of Mixing: Stretching, Chaos, and Transport , 1989 .

[12]  Jean-Luc Thiffeault,et al.  Advection–diffusion in Lagrangian coordinates , 2003 .

[13]  G. Taylor Dispersion of soluble matter in solvent flowing slowly through a tube , 1953, Proceedings of the Royal Society of London. Series A. Mathematical and Physical Sciences.

[14]  Hassan Peerhossaini,et al.  Residence time distribution in twisted pipe flows: helically coiled system and chaotic system , 1997 .

[15]  H. Brenner,et al.  Dispersion resulting from flow through spatially periodic porous media , 1980, Philosophical Transactions of the Royal Society of London. Series A, Mathematical and Physical Sciences.

[16]  Stephen Wiggins,et al.  Residence-time distributions for chaotic flows in pipes. , 1999, Chaos.

[17]  O. Levenspiel Chemical Reaction Engineering , 1972 .

[18]  I. Kang,et al.  Chaotic mixing and mass transfer enhancement bypulsatile laminar flow in an axisymmetric wavy channel , 1999 .

[19]  Julio M. Ottino,et al.  A case study of chaotic mixing in deterministic flows: The partitioned-pipe mixer , 1987 .

[20]  A. Boozer,et al.  A Lagrangian analysis of advection-diffusion equation for a three dimensional chaotic flow , 1999 .

[21]  P. C. Chatwin,et al.  The effects of curvature and buoyancy on the laminar dispersion of solute in a horizontal tube , 1967, Journal of Fluid Mechanics.

[22]  Hassan Aref,et al.  The development of chaotic advection , 2002 .

[23]  Howard A. Stone,et al.  ENGINEERING FLOWS IN SMALL DEVICES , 2004 .