Three-state Potts nematic order in stacked frustrated spin models with SO(3) symmetry

We propose stacked two-dimensional lattice designs of frustrated and SO(3) symmetric spin models consisting of antiferromagnetic (AFM) triangular and ferromagnetic (FM) sixfold symmetric sublattices that realize emergent Z3 Potts nematic order. Considering bilinear-biquadratic spin interactions, our models describe an SO(3)-symmetric triangular lattice AFM subject to a fluctuating magnetization arising from the FM coupled sublattice. We focus on the classical AFM-FM windmill model and map out the zero- and finite-temperature phase diagram using Monte Carlo simulations and analytical calculations. We discover a state with composite Potts nematic order above the ferrimagnetic three-sublattice up-up-down ground state and relate it to Potts phases in SO(3)-broken Heisenberg and Ising AFMs in external magnetic fields. Finally, we show that the biquadratic exchange in our model is automatically induced by thermal and quantum fluctuations in the purely bilinear Heisenberg model, easing the requirements for realizing these lattice designs experimentally.

[1]  K. Novoselov,et al.  Breaking through the Mermin-Wagner limit in 2D van der Waals magnets , 2022, Nature Communications.

[2]  Jun Yu Li,et al.  Charge-density-wave-driven electronic nematicity in a kagome superconductor , 2022, Nature.

[3]  Kenji Watanabe,et al.  Nematicity and competing orders in superconducting magic-angle graphene , 2020, Science.

[4]  J. Schmalian,et al.  Z3-vestigial nematic order due to superconducting fluctuations in the doped topological insulators NbxBi2Se3 and CuxBi2Se3 , 2020, Nature Communications.

[5]  R. Fernandes,et al.  Nematicity with a twist: Rotational symmetry breaking in a moiré superlattice , 2019, Science Advances.

[6]  J. Orenstein,et al.  Three-state nematicity in the triangular lattice antiferromagnet Fe1/3NbS2 , 2019, Nature Materials.

[7]  D. Ralph,et al.  Probing and controlling magnetic states in 2D layered magnetic materials , 2019, Nature Reviews Physics.

[8]  Sylvain Schwartz,et al.  Quantum Kibble–Zurek mechanism and critical dynamics on a programmable Rydberg simulator , 2018, Nature.

[9]  J. Schmalian,et al.  Intertwined Vestigial Order in Quantum Materials: Nematicity and Beyond , 2018, Annual Review of Condensed Matter Physics.

[10]  J. Schmalian,et al.  Vestigial nematic order and superconductivity in the doped topological insulator CuxBi2Se3 , 2017, 1712.07523.

[11]  T. Takata,et al.  Mathematical Proceedings of the Cambridge Philosophical Society , 2017 .

[12]  Srihari Keshavamurthy,et al.  Annual Review of Physical Chemistry, 2015 , 2016 .

[13]  N. Prokof'ev,et al.  Superfluid States of Matter , 2015 .

[14]  O. Starykh Unusual ordered phases of highly frustrated magnets: a review , 2014, Reports on progress in physics. Physical Society.

[15]  W. Marsden I and J , 2012 .

[16]  M. Zhitomirsky,et al.  Magnetic phase diagrams of classical triangular and kagome antiferromagnets , 2010, Journal of physics. Condensed matter : an Institute of Physics journal.

[17]  Michael J. Lawler,et al.  Nematic Fermi Fluids in Condensed Matter Physics , 2009, 0910.4166.

[18]  James S. Langer,et al.  Annual review of condensed matter physics , 2010 .

[19]  C. Vaz,et al.  Magnetism in ultrathin film structures , 2008 .

[20]  N. Ashcroft,et al.  A superconductor to superfluid phase transition in liquid metallic hydrogen , 2004, Nature.

[21]  A. J. Jin,et al.  Layer-by-layer ordering of ultrathin liquid crystal films on the three-level Potts model , 2000 .

[22]  T. Nikuni,et al.  Fluctuation-induced phase in in a transverse magnetic field: theory , 1998, cond-mat/9802307.

[23]  A. J. Jin,et al.  Novel results of extremely thin substrate-free liquid-crystal films obtained from calorimetric and computer simulation studies , 1994 .

[24]  T. Stoebe,et al.  Thermal properties of ‘stacked hexatic phases’ in liquid crystals , 1993 .

[25]  A. V. Chubukov,et al.  Quantum theory of an antiferromagnet on a triangular lattice in a magnetic field , 1991 .

[26]  Henk W. J. Blöte,et al.  Triangular SOS models and cubic-crystal shapes , 1984 .

[27]  J. Villain,et al.  Order as an effect of disorder , 1980 .

[28]  O. Vilches Phase Transitions in Monomolecular Layer Films Physisorbed on Crystalline Surfaces , 1980 .

[29]  J. Villain A magnetic analogue of stereoisomerism : application to helimagnetism in two dimensions , 1977 .

[30]  J. Walker,et al.  Antiferromagnetict riangular Ising model , 1976 .

[31]  S. Alexander Lattice gas transition of He on Grafoil. A continuous transition with cubic terms , 1975 .

[32]  B. D. Metcalf Phase diagram of a nearest neighbor triangular antiferromagnet in an external field , 1973 .