Quenching experiment on Cr-alloy-coated cladding for accident-tolerant fuel in water pool under low and high subcooling conditions

Abstract A transient pool boiling experiment was conducted to investigate the quenching performance of Cr-alloy-coated cladding in the simulated conditions of a loss-of-coolant accident (LOCA). Cr-alloy-coated cladding is a potential candidate for accident-tolerant fuel (ATF), which is developed to suppress hydrogen generation at high temperature in the event of an LOCA or beyond design basis accident. Cr-alloy-coated cladding and Zircaloy-4 cladding were used in the quenching experiment under low and high subcooling conditions, i.e., 0 °C and 50 °C. The thicknesses of the Cr-alloy-coated layer were 20 and 50 μm. Each cladding specimen was heated up to 600 °C in a furnace and quenched in a water pool at constant temperature. The quenching experiment showed the formation of film boiling and transition to nuclear boiling at the low subcooling temperature of 0 °C. No film boiling was observed at high subcooling at 50 °C. The effect of surface roughness was found to be insignificant for quenching performance. Rather, cladding oxidation, particularly for the Zircaloy-4 specimens, had a remarkable influence on the minimum film boiling temperature (MFBT) and quenching time. The Cr-alloy-coated cladding did not show the effect of surface oxidation as expected because of very low cladding oxidation. There is no significant difference in the quenching performance of the Zircaloy-4 cladding and the Cr-alloy-coated cladding at the high subcooling temperature of 50 °C. Furthermore, the Cr-alloy-coated cladding tends to decrease the quenching time with higher MFBT as the coating thickness decreases.

[1]  Liwu Fan,et al.  An experimental study of the accelerated quenching rate and enhanced pool boiling heat transfer on rodlets with a superhydrophilic surface in subcooled water , 2018 .

[2]  Yang-Hyun Koo,et al.  Adhesion property and high-temperature oxidation behavior of Cr-coated Zircaloy-4 cladding tube prepared by 3D laser coating , 2015 .

[3]  O. Burggraf An Exact Solution of the Inverse Problem in Heat Conduction Theory and Applications , 1964 .

[4]  Yang-Hyun Koo,et al.  Development Status of Accident-tolerant Fuel for Light Water Reactors in Korea , 2016 .

[5]  F. Cheung,et al.  Effects of Substrate Materials and Surface Conditions on the Minimum Film-Boiling Temperature , 2018, Nuclear Technology.

[6]  F. Cheung,et al.  An experimental investigation of the effects of surface conditions on pool-boiling heat transfer for various materials , 2017 .

[7]  J. Sinha,et al.  EFFECTS OF SURFACE ROUGHNESS, OXIDATION LEVEL, AND LIQUID SUBCOOLING ON THE MINIMUM FILM BOILING TEMPERATURE , 2003 .

[8]  Milan Hnizdil,et al.  Effects of oxide layer on Leidenfrost temperature during spray cooling of steel at high temperatures , 2015 .

[9]  F. Cheung,et al.  Parametric investigation of film boiling heat transfer on the quenching of vertical rods in water pool , 2018, Applied Thermal Engineering.

[10]  R. E. Henry A correlation for the minimum film boiling temperature , 1974 .

[11]  Liwu Fan,et al.  Regulated transient pool boiling of water during quenching on nanostructured surfaces with modified wettability from superhydrophilic to superhydrophobic , 2014 .

[12]  S. M. Bajorek,et al.  Experimental Investigation of Minimum Film Boiling Temperature for Vertical Cylinders at Elevated Pressure , 2002 .

[13]  Ben-Ran Fu,et al.  Quenching characteristics of a continuously-heated rod in natural sea water , 2016 .

[14]  Sunwoo Kim,et al.  Parametric investigation on transient boiling heat transfer of metal rod cooled rapidly in water pool , 2017 .

[15]  Tae Hyun Chun,et al.  Effect of change in surface condition induced by oxidation on transient pool boiling heat transfer of vertical stainless steel and copper rodlets , 2014 .

[16]  Michael L. Corradini,et al.  Transient pool boiling heat transfer of oxidized and roughened Zircaloy-4 surfaces during water quenching , 2018 .

[17]  Steven J. Zinkle,et al.  Accident tolerant fuels for LWRs: A perspective , 2014 .

[18]  K. Prabhu,et al.  Effect of surface roughness on metal/quenchant interfacial heat transfer and evolution of microstructure , 2007 .

[19]  Jacopo Buongiorno,et al.  On the quenching of steel and zircaloy spheres in water-based nanofluids with alumina, silica and diamond nanoparticles , 2009 .

[20]  Il-Hyun Kim,et al.  Out-of-pile performance of surface-modified Zr cladding for accident tolerant fuel in LWRs , 2018, Journal of Nuclear Materials.

[21]  P. J. Berenson Film-Boiling Heat Transfer From a Horizontal Surface , 1961 .

[22]  Edward M. Greitzer,et al.  Film boiling on vertical surfaces , 1972 .