Comparative analysis of energy intensity and carbon emissions in wastewater treatment in USA, Germany, China and South Africa

Currently almost all wastewater treatment plants (WWTPs) require a large amount of energy input to process the influent, mostly as electricity, and the associated carbon emissions are in aggregate significant. In order to achieve carbon neutrality, it is important to understand direct and indirect carbon emissions generated by WWTPs. Here, we focused on electricity use in WWTPs as it is a major source of carbon emissions. Specifically, we compared the electricity intensity and associated carbon emissions of WWTPs in four countries: the USA, Germany, China, and South Africa. We found that 100% energy self-sufficient WWTPs are feasible by a combination of increased energy efficiency and energy harvesting from the wastewater. Carbon emissions of WWTPs depend strongly on the electricity fuel mix, wastewater treatment technologies, treatment capacity, and influent and effluent water quality. A few WWTPs operating in developed countries (USA and Germany) have already achieved almost 100% (or higher) electricity self-sufficiency through energy efficiency and harvesting biogas and electricity. In comparison with Germany, WWTPs in the USA are more heterogeneous and the range of unit carbon emission intensity is much wider. In some areas where the organic content in wastewater is lower and less biogas is produced, it is still possible to achieve energy self-sufficiency by using thermal energy from wastewater. Industrial wastewater in China in general consumes more electricity and the carbon intensity of electricity is also higher, resulting in much higher unit carbon emissions as compared with other countries. In megacities such as Shanghai, larger capacity of centralized WWTPs can decrease the unit carbon emissions significantly. These findings provide a global perspective on the state of WWTPs and are helpful to improve the understanding, designing and operating of WWTPs from the perspective of achieving carbon neutrality.

[1]  Konrad Koch,et al.  Co-digestion of food waste in municipal wastewater treatment plants: Effect of different mixtures on methane yield and hydrolysis rate constant , 2015 .

[2]  Sisi Chen,et al.  Effects of thermal hydrolysis on organic matter solubilization and anaerobic digestion of high solid sludge , 2015 .

[3]  Weiwei Mo,et al.  Can municipal wastewater treatment systems be carbon neutral? , 2012, Journal of environmental management.

[4]  P. Jeníček,et al.  Energy self-sufficient sewage wastewater treatment plants: is optimized anaerobic sludge digestion the key? , 2013, Water science and technology : a journal of the International Association on Water Pollution Research.

[5]  K. Kaygusuz Energy for sustainable development: A case of developing countries , 2012 .

[6]  Piotr Oleskowicz-Popiel,et al.  Enhancement of biogas production at the municipal wastewater treatment plant by co-digestion with poultry industry waste , 2016 .

[7]  Elizabeth Plater-Zyberk,et al.  Net-zero water management: achieving energy-positive municipal water supply , 2016 .

[8]  S. Hermanowicz,et al.  A novel technique for evaluating foam dynamics in anaerobic digesters. , 2013, Water science and technology : a journal of the International Association on Water Pollution Research.

[9]  Fei Zhang,et al.  A new method for nutrients removal and recovery from wastewater using a bioelectrochemical system. , 2014, Bioresource technology.

[10]  Kelly T. Sanders,et al.  Critical review: Uncharted waters? The future of the electricity-water nexus. , 2015, Environmental science & technology.

[11]  Xin Huang,et al.  Evaluation of the potential for operating carbon neutral WWTPs in China. , 2015, Water research.

[12]  Fei Zhang,et al.  Energy extraction from a large-scale microbial fuel cell system treating municipal wastewater , 2015 .

[13]  L. Corominas,et al.  A dynamic modelling approach to evaluate GHG emissions from wastewater treatment plants , 2012 .

[14]  C. Fimml,et al.  Energy self-sufficiency as a feasible concept for wastewater treatment systems , 2007 .

[15]  Bryan W. Karney,et al.  Life-Cycle Energy Use and Greenhouse Gas Emissions Inventory for Water Treatment Systems , 2007 .

[16]  D J I Gustavsson,et al.  Carbon footprints of Scandinavian wastewater treatment plants. , 2013, Water science and technology : a journal of the International Association on Water Pollution Research.

[17]  Petar Sabev Varbanov,et al.  Ways to optimize the energy balance of municipal wastewater systems: lessons learned from Austrian applications , 2015 .

[18]  Sangwon Suh,et al.  Environmental impacts of products in china. , 2011, Environmental science & technology.

[19]  Manfred Lenzen,et al.  Renewable Energy in the Context of Sustainable Development , 2011 .

[20]  Qiong Zhang,et al.  Energy-nutrients-water nexus: integrated resource recovery in municipal wastewater treatment plants. , 2013, Journal of environmental management.

[21]  Younggy Kim,et al.  Enhanced digestion of waste activated sludge using microbial electrolysis cells at ambient temperature. , 2015, Water research.

[22]  Mark C.M. van Loosdrecht,et al.  Towards a more sustainable municipal wastewater treatment system , 1997 .

[23]  H. Asselt,et al.  All Hands on Deck! Mobilizing Climate Change Action Beyond the UNFCCC , 2012 .

[24]  Corinne Le Quéré,et al.  The challenge to keep global warming below 2 °C , 2013 .

[25]  J. Keller,et al.  Greenhouse gas production in wastewater treatment: process selection is the major factor. , 2003, Water science and technology : a journal of the International Association on Water Pollution Research.

[26]  S. Pavlostathis,et al.  Co-digestion of municipal sludge and external organic wastes for enhanced biogas production under realistic plant constraints. , 2015, Water research.

[27]  L. T. Angenent,et al.  Comparing the inhibitory thresholds of dairy manure co-digesters after prolonged acclimation periods: Part 1--Performance and operating limits. , 2015, Water research.

[28]  Lu Lu,et al.  Microbial Electrolytic Carbon Capture for Carbon Negative and Energy Positive Wastewater Treatment. , 2015, Environmental science & technology.

[29]  Zdravko Kravanja,et al.  Optimal design for heat-integrated water-using and wastewater treatment networks , 2014 .

[30]  Jeonghwan Kim,et al.  Domestic wastewater treatment as a net energy producer--can this be achieved? , 2011, Environmental science & technology.

[31]  Janice Izabel Druzian,et al.  From waste to energy: Microalgae production in wastewater and glycerol , 2013 .

[32]  Bernadette K. McCabe,et al.  Review of pre-treatments used in anaerobic digestion and their potential application in high-fat cattle slaughterhouse wastewater. , 2015 .

[33]  Wen-Wei Li,et al.  Towards sustainable wastewater treatment by using microbial fuel cells-centered technologies , 2013 .

[34]  T. A. Larsen CO₂-neutral wastewater treatment plants or robust, climate-friendly wastewater management? A systems perspective. , 2015, Water research.

[35]  Michael E. Webber,et al.  Energy recovery from wastewater treatment plants in the United States: A case study of the energy-water nexus , 2010 .

[36]  Eric Johnson Handbook on Life Cycle Assessment Operational Guide to the ISO Standards , 2003 .

[37]  G. Mohanakrishna,et al.  Multiple process integrations for broad perspective analysis of fermentative H2 production from wastewater treatment: Technical and environmental considerations , 2013 .

[38]  Hongtao Wang,et al.  Chemically enhanced primary treatment (CEPT) for removal of carbon and nutrients from municipal wastewater treatment plants: a case study of Shanghai. , 2009, Water science and technology : a journal of the International Association on Water Pollution Research.

[39]  B. Wett,et al.  Synergistic co-digestion of solid-organic-waste and municipal-sewage-sludge: 1 plus 1 equals more than 2 in terms of biogas production and solids reduction. , 2015, Water research.

[40]  Zhen Zhou,et al.  Inhibitory effects of sulfide on nitrifying biomass in the anaerobic–anoxic–aerobic wastewater treatment process , 2014 .

[41]  Youcai Zhao,et al.  Greenhouse gases emissions accounting for typical sewage sludge digestion with energy utilization and residue land application in China. , 2013, Waste management.

[42]  Frank Schultmann,et al.  Electricity and substitute natural gas generation from the conversion of wastewater treatment plant sludge. , 2014 .

[43]  M Molinos-Senante,et al.  Energy efficiency in Spanish wastewater treatment plants: a non-radial DEA approach. , 2011, The Science of the total environment.

[44]  D. Batstone,et al.  Analysis of the potential to recover energy and nutrient resources from cattle slaughterhouses in Australia by employing anaerobic digestion , 2014 .

[45]  T. Chiramba,et al.  Water and Wastewater Treatment in Africa – Current Practices and Challenges , 2014 .

[46]  Kebin He,et al.  Energy policy: A low-carbon road map for China , 2013, Nature.

[47]  Erika Matulionytė-Jarašūnė Renewable energy in the context of sustainable development , 2012 .

[48]  Silvia Fiore,et al.  Evaluation of the energy efficiency of a large wastewater treatment plant in Italy , 2016 .

[49]  Zhen He,et al.  Sediment microbial fuel cells for wastewater treatment: challenges and opportunities , 2015 .

[50]  Belinda S.M. Sturm,et al.  An energy evaluation of coupling nutrient removal from wastewater with algal biomass production , 2011 .

[51]  Christian Remy Project CoDiGreen Work package 2: LCA study of Braunschweig wastewater scheme , 2012 .

[52]  C. Kang,et al.  Opportunity for offshore wind to reduce future demand for coal-fired power plants in China with consequent savings in emissions of CO2. , 2014, Environmental science & technology.

[53]  Jixiang Zhang,et al.  Co-liquefaction of swine manure and mixed-culture algal biomass from a wastewater treatment system to produce bio-crude oil , 2014 .

[54]  Bernadette K. McCabe,et al.  A case study for biogas generation from covered anaerobic ponds treating abattoir wastewater: investigation of pond performance and potential biogas production , 2014 .

[55]  T. R. Sreekrishnan,et al.  High strength wastewater treatment accompanied by power generation using air cathode microbial fuel cell , 2013 .

[56]  Randall Spalding-fecher What is the carbon emission factor for the South African electricity grid , 2017 .