Tailoring the excitation of localized surface plasmon-polariton resonances by focusing radially-polarized beams.

We study the interaction of focused radially-polarized light with metal nanospheres. By expanding the electromagnetic field in terms of multipoles, we gain insight on the excitation of localized surface plasmon-polariton resonances in the nanoparticle. We show that focused radially-polarized beams offer more opportunities than a focused plane wave or a Gaussian beam for tuning the near- and far-field system response. These results find applications in nano-optics, optical tweezers, and optical data storage.

[1]  Z. Kam,et al.  Absorption and Scattering of Light by Small Particles , 1998 .

[2]  Nassiredin M. Mojarad,et al.  Plasmon spectra of nanospheres under a tightly focused beam , 2007, 0711.3649.

[3]  Riccardo Borghi,et al.  Highly focused spirally polarized beams. , 2005, Journal of the Optical Society of America. A, Optics, image science, and vision.

[4]  A. Meixner,et al.  Orientational imaging of subwavelength Au particles with higher order laser modes. , 2006, Nano letters.

[5]  T G Brown,et al.  Longitudinal field modes probed by single molecules. , 2001, Physical review letters.

[6]  G Leuchs,et al.  Sharper focus for a radially polarized light beam. , 2003, Physical review letters.

[7]  Mathias Steiner,et al.  Topology measurements of metal nanoparticles with 1 nm accuracy by Confocal Interference Scattering Microscopy. , 2007, Optics express.

[8]  J. Hodges,et al.  Failure of the optical theorem for Gaussian-beam scattering by a spherical particle , 1995 .

[9]  Colin J. R. Sheppard,et al.  Efficient calculation of electromagnetic diffraction in optical systems using a multipole expansion , 1997 .

[10]  R. W. Christy,et al.  Optical Constants of the Noble Metals , 1972 .

[11]  S. Inasawa,et al.  Optical recording media using laser-induced size reduction of Au nanoparticles , 2001 .

[12]  E. Wolf,et al.  Electromagnetic diffraction in optical systems, II. Structure of the image field in an aplanatic system , 1959, Proceedings of the Royal Society of London. Series A. Mathematical and Physical Sciences.

[13]  S. V. Enk Atoms, dipole waves, and strongly focused light beams (8 pages) , 2003, quant-ph/0307216.

[14]  S. Maier,et al.  Plasmonics: Localization and guiding of electromagnetic energy in metal/dielectric structures , 2005 .

[15]  Asher A. Friesem,et al.  The formation of laser beams with pure azimuthal or radial polarization , 2000 .

[16]  A. Meixner,et al.  A novel approach to detect and characterize the scattering patterns of single Au nanoparticles using confocal microscopy , 2008, Journal of microscopy.

[17]  Nassiredin M. Mojarad,et al.  Perfect reflection of light by an oscillating dipole. , 2008, Physical review letters.

[18]  R. Dorn,et al.  The focus of light – theoretical calculation and experimental tomographic reconstruction , 2001 .

[19]  Kathleen S. Youngworth,et al.  Focusing of high numerical aperture cylindrical-vector beams. , 2000, Optics express.

[20]  Nicole J. Moore,et al.  Closed form formula for Mie scattering of nonparaxial analogues of Gaussian beams. , 2008, Optics express.

[21]  P. Török,et al.  Rigorous analysis of spheres in Gauss-Laguerre beams. , 2007, Optics express.

[22]  Richard K. Chang,et al.  Local fields at the surface of noble-metal microspheres , 1981 .

[23]  V. Giannini,et al.  Excitation and emission enhancement of single molecule fluorescence through multiple surface-plasmon resonances on metal trimer nanoantennas. , 2008, Optics letters.

[24]  W. Challener,et al.  Interaction of spherical nanoparticles with a highly focused beam of light. , 2008, Optics express.

[25]  Q. Zhan Trapping metallic Rayleigh particles with radial polarization. , 2004, Optics express.