From the Caribbean to West Africa: Four weeks of continuous dust and marine aerosol profiling with shipborne polarization/Raman lidar – a contribution to SALTRACE

Continuous vertically resolved monitoring of marine aerosol, Saharan dust, and marine/dust aerosol mixtures was performed with multiwavelength polarization/Raman lidar aboard the German research vessel R/V Meteor during a one-month transatlantic cruise from Guadeloupe to Cabo Verde over 4500 km (from 61.5° W to 2° W, mostly along 14.5° N) in April–May 2013, as part of SALTRACE (Saharan Aerosol Long-range Transport and Aerosol–Cloud Interaction Experiment). An overview of measured aerosol optical properties over the tropical Atlantic is given in terms of spectrally resolved particle backscatter and extinction coefficients, lidar ratio, and linear depolarization ratio. Height profiles from the marine boundary layer (MBL) up to the top of the Saharan Air Layer (SAL) are presented. MBL and SAL mean lidar ratios were around 20 and 40 sr. These values indicate clean marine conditions in the MBL and entrainment of marine particles into the lower part of the SAL. In the central and upper parts of the SAL, the lidar ratios were most frequently 50–60 sr and thus typical for Saharan dust. The MBL and SAL mean depolarization ratios were close to 0.05 and between 0.2–0.3, respectively, which reflects almost dust-free conditions in the MBL and the occurrence of a mixture of marine and dust particles in the SAL. The conceptual model, describing the long-range transport and removal processes of Saharan dust over the North Atlantic, is discussed and confronted with the lidar observations along the west-to-east track of the slowly moving research vessel. The role of turbulent downward mixing as an efficient dust removal process is illuminated. In a follow-up article (Rittmeister et al., 2017), the lidar observations of dust extinction coefficient and derived mass concentration profiles are compared with respective dust profiles simulated with three well-established European atmospheric aerosol and dust prediction models (MACC, NMMB/BSC-Dust, SKIRON).

[1]  Corinna Hoose,et al.  Heterogeneous ice nucleation on atmospheric aerosols: a review of results from laboratory experiments , 2012 .

[2]  V. Freudenthaler,et al.  The Saharan Aerosol Long-range TRansport and Aerosol-Cloud-Interaction Experiment 1 ( SALTRACE ) : overview and selected highlights 2 , 2016 .

[3]  D. Winker,et al.  A height resolved global view of dust aerosols from the first year CALIPSO lidar measurements , 2008 .

[4]  R. Draxler,et al.  NOAA’s HYSPLIT Atmospheric Transport and Dispersion Modeling System , 2015 .

[5]  S. H. Melfi,et al.  Validation of the Saharan dust plume conceptual model using lidar, meteosat, and ECMWF Data , 1999 .

[6]  Didier Tanré,et al.  Retrieval of optical and physical properties of African dust from multiwavelength Raman lidar measurements during the SHADOW campaign in Senegal , 2016 .

[7]  B. Albrecht,et al.  Vertical structure of aerosols, temperature, and moisture associated with an intense African dust event observed over the eastern Caribbean , 2012 .

[8]  R. Engelmann,et al.  Contrasting the impact of aerosols at northern and southern midlatitudes on heterogeneous ice formation , 2011 .

[9]  J. Heintzenberg The SAMUM-1 experiment over Southern Morocco: overview and introduction , 2009 .

[10]  R. Engelmann,et al.  An overview of the first decade of Polly NET : an emerging network of automated Raman-polarization lidars for continuous aerosol profiling , 2016 .

[11]  Michael Schulz,et al.  Global dust model intercomparison in AeroCom phase I , 2011 .

[12]  Albert Ansmann,et al.  Profiling of Saharan dust and biomass-burning smoke with multiwavelength polarization Raman lidar at Cape Verde , 2011 .

[13]  R. Engelmann,et al.  Central Asian Dust Experiment (CADEX): Multiwavelength Polarization Raman Lidar Observations in Tajikistan , 2016 .

[14]  Sonia M. Kreidenweis,et al.  Effect of chemical mixing state on the hygroscopicity and cloud nucleation properties of calcium mineral dust particles , 2009 .

[15]  Albert Ansmann,et al.  Optical properties of long-range transported Saharan dust over Barbados as measured by dual-wavelength depolarization Raman lidar measurements , 2015 .

[16]  J. Seewald,et al.  Cloud condensation nucleus activity comparison of dry- and wet-generated mineral dust aerosol: the significance of soluble material , 2013 .

[17]  Albert Ansmann,et al.  The automated multiwavelength Raman polarization and water-vapor lidar PollyXT: The neXT generation , 2016 .

[18]  R. Engelmann,et al.  Further evidence for significant smoke transport from Africa to Amazonia , 2011 .

[19]  Alexander Smirnov,et al.  Maritime Aerosol Network as a component of Aerosol Robotic Network , 2009 .

[20]  Z. Levin,et al.  The Effects of Desert Particles Coated with Sulfate on Rain Formation in the Eastern Mediterranean , 1996 .

[21]  Albert Ansmann,et al.  Saharan dust and heterogeneous ice formation: Eleven years of cloud observations at a central European EARLINET site , 2010 .

[22]  V. Freudenthaler,et al.  Optical and microphysical properties of smoke over Cape Verde inferred from multiwavelength lidar measurements , 2011 .

[23]  O. Reitebuch,et al.  Saharan dust long-range transport across the Atlantic studied by an airborneDoppler wind lidar and the MACC model , 2016 .

[24]  B. Holben,et al.  Saharan dust transport to the caribbean during PRIDE: 2. Transport, vertical profiles, and deposition in simulations of in situ and remote sensing observations : Puerto Rico Dust Experiment (PRIDE1) , 2003 .

[25]  Toby N. Carlson,et al.  Vertical and areal distribution of Saharan dust over the western equatorial north Atlantic Ocean , 1972 .

[26]  V. Freudenthaler,et al.  Saharan dust contribution to the Caribbean summertime boundary layer –a lidar study during SALTRACE , 2016 .

[27]  G. S. Kent,et al.  Scientific investigations planned for the lidar in-space technology experiment (LITE) , 1993 .

[28]  O. Torres,et al.  ENVIRONMENTAL CHARACTERIZATION OF GLOBAL SOURCES OF ATMOSPHERIC SOIL DUST IDENTIFIED WITH THE NIMBUS 7 TOTAL OZONE MAPPING SPECTROMETER (TOMS) ABSORBING AEROSOL PRODUCT , 2002 .

[29]  Albert Ansmann,et al.  Tracking the Saharan Air Layer with shipborne lidar across the tropical Atlantic , 2014 .

[30]  Jacques Pelon,et al.  The seasonal vertical distribution of the Saharan Air Layer and its modulation by the wind , 2013 .

[31]  Albert Ansmann,et al.  Saharan Mineral Dust Experiments SAMUM–1 and SAMUM–2: what have we learned? , 2011 .

[32]  K. Prather,et al.  Improvements to an Empirical Parameterization of Heterogeneous Ice Nucleation and Its Comparison with Observations , 2013 .

[33]  M. Petters,et al.  Hygroscopicity and cloud droplet activation of mineral dust aerosol , 2009 .

[34]  Ina Tegen,et al.  Modeling the mineral dust aerosol cycle in the climate system , 2003 .

[35]  V. Freudenthaler,et al.  Depolarization ratio profiling at several wavelengths in pure Saharan dust during SAMUM 2006 , 2009 .

[36]  S. Martin,et al.  Transport of North African dust from the Bodélé depression to the Amazon Basin: a case study , 2010 .

[37]  M. Petters,et al.  Integrating laboratory and field data to quantify the immersion freezing ice nucleation activity of mineral dust particles , 2014 .

[38]  David M. Winker,et al.  CALIPSO lidar observations of the optical properties of Saharan dust: A case study of long‐range transport , 2008 .

[39]  Gunnar Myhre,et al.  Global sensitivity experiments of the radiative forcing due to mineral aerosols , 2001 .