Nonlinear effects with ultrashort laser pulses

Propagation of an intense femtosecond laser pulse through a transparent nonlinear medium such as dielectric leads to a number of phenomena. In our experiment we observed complex spatial, spectral, and temporal structures appearing in the initially smooth femtosecond laser pulse when the pulse power is comparable to or higher than the critical power for self-focusing. We have also developed a complete, 3-dimensional theoretical model to describe the observed phenomena.

[1]  A. Zewail,et al.  Femtosecond real-time probing of reactions. V. The reaction of IHgI , 1989 .

[2]  Alexander M. Sergeev,et al.  Femtosecond energy transfer within the LH2 peripheral antenna of the photosynthetic purple bacteria Rhodobacter sphaeroides and Rhodopseudomonas palustris LL , 1993 .

[3]  A. Zewail,et al.  Femtosecond dynamics of transition states: the classical saddle-point barrier reactions , 1998 .

[4]  A. Othonos Probing ultrafast carrier and phonon dynamics in semiconductors , 1998 .

[5]  Robert Eugene Blankenship,et al.  Femtosecond energy transfer and spectral equilibration in bacteriochlorophyll a--protein antenna trimers from the green bacterium Chlorobium tepidum. , 1994, Biophysical journal.

[6]  D. Kane,et al.  Characterization of arbitrary femtosecond pulses using frequency-resolved optical gating , 1993 .

[7]  Jerzy S. Krasinski,et al.  Interferometric measurement of femtosecond pulse distortion by lenses , 1996 .

[8]  Rick Trebino,et al.  Improved ultrashort pulse-retrieval algorithm for frequency-resolved optical gating , 1994 .

[9]  Govind P. Agrawal,et al.  Nonlinear Fiber Optics , 1989 .

[10]  G. Mourou,et al.  Terawatt to Petawatt Subpicosecond Lasers , 1994, Science.

[11]  M. Trippenbach,et al.  Propagation of light pulses in nonisotropic media , 1996 .

[12]  I. A. Walmsley,et al.  Self-referencing spectral interferometry for measuring ultrashort optical pulses , 1999 .

[13]  E. V. Khoroshilov,et al.  Femtosecond energy transfer between chromophores in allophycocyanin trimers , 1992 .

[14]  V. Petrov,et al.  Self-focusing of light pulses in the presence of normal group-velocity dispersion. , 1992, Optics letters.

[15]  A. Zewail,et al.  Femtosecond real-time probing of reactions. XXI. Direct observation of transition-state dynamics and structure in charge-transfer reactions , 1996 .

[16]  Hall,et al.  Direct link between microwave and optical frequencies with a 300 THz femtosecond laser comb , 2000, Physical review letters.

[17]  Marek Trippenbach,et al.  Interferometric measurement of femtosecond wave-packet tilting in rutile crystal , 1997 .

[18]  Yia-Chung Chang,et al.  Ultrafast carrier dynamics in a highly excited GaN epilayer , 2001 .

[19]  S A Diddams,et al.  Amplitude and phase measurements of femtosecond pulse splitting in nonlinear dispersive media. , 1998, Optics letters.

[20]  Reichert,et al.  Phase coherent vacuum-ultraviolet to radio frequency comparison with a mode-locked laser , 2000, Physical review letters.

[21]  Fibich Small beam nonparaxiality arrests self-focusing of optical beams. , 1996, Physical review letters.

[22]  Ranka,et al.  Observation of Pulse Splitting in Nonlinear Dispersive Media. , 1996, Physical review letters.

[23]  J. Rothenberg Pulse splitting during self-focusing in normally dispersive media. , 1992, Optics letters.

[24]  S. Rosenthal,et al.  Ultrafast Carrier Dynamics in CdSe Nanocrystals Determined by Femtosecond Fluorescence Upconversion Spectroscopy , 2001 .

[25]  T. Clement,et al.  Propagation Dynamics of Intense Femtosecond Pulses: Multiple Splittings, Coalescence, and Continuum Generation , 1999 .

[26]  M. Trippenbach,et al.  Effects of self-steepening and self-frequency shifting on short-pulse splitting in dispersive nonlinear media , 1998 .

[27]  Gadi Fibich,et al.  A modulation method for self-focusing in the perturbed critical nonlinear Schrödinger equation , 1998 .