Beryllium‐7: The Cinderella of fallout radionuclide sediment tracers?

Current concern for the sustainable management of soil resources and the many adverse effects of increased sediment loads on streams and river systems has generated a need for more information on rates and patterns of soil loss and an improved understanding of catchment sediment budgets. Traditional measurement techniques are frequently unable to meet the requirements and fallout radionuclides have been shown to offer considerable potential for tracing the mobilization, transfer, redistribution and storage of soil and sediment within catchments and river systems. Caesium‐137 and lead‐210 have been the most widely used fallout radionuclide sediment tracers, but their half‐lives mean that the information that they provide is in most instances limited to the medium term (e.g. 25–120 years). The need for information on shorter timescales has directed attention to the potential for using beryllium‐7, which has a considerable shorter half‐life, for tracing soil and sediment redistribution over short timescales (e.g. days–weeks). To date, however, there have been relatively few attempts to exploit this potential. This situation is likely to be in part a reflection of the emphasis of early work on 137Cs and 210Pb and the more recent nature of work using 7Be. However, it may also reflect the limitations and constraints imposed by the nature of 7Be fallout and the short half‐life of this radionuclide. This contribution explores recent work in using 7Be as a sediment tracer and the constraints imposed by its origin and behaviour. Attention is directed to fallout inputs, the application of 7Be to tracing soil and sediment redistribution on slopes and on river floodplains, its use as a source fingerprint and other related applications. The likely future potential of 7Be as a sediment tracer is assessed. Copyright © 2012 John Wiley & Sons, Ltd.

[1]  Desmond E. Walling,et al.  Sediment Source Fingerprinting (Tracing) and Sediment Budgets as Tools in Targeting River and Watershed Restoration Programs , 2013 .

[2]  V. Golosov,et al.  Application of Chernobyl‐derived 137Cs fallout for sediment redistribution studies: lessons from European Russia , 2013 .

[3]  C. Sanders,et al.  Lead-210 and Beryllium-7 fallout rates on the southeastern coast of Brazil. , 2011, Journal of environmental radioactivity.

[4]  Xin-bao Zhang,et al.  Comparison of the soil losses from (7)Be measurements and the monitoring data by erosion pins and runoff plots in the Three Gorges Reservoir region, China. , 2011, Applied radiation and isotopes : including data, instrumentation and methods for use in agriculture, industry and medicine.

[5]  A. Elmore,et al.  Beryllium‐7 in soils and vegetation along an arid precipitation gradient in Owens Valley, California , 2011 .

[6]  J. Terry,et al.  Assessing the utility of 210Pb geochronology for estimating sediment accumulation rates on river floodplains in Fiji , 2011 .

[7]  N. Gratiot,et al.  Sediment dynamics during the rainy season in tropical highland catchments of central Mexico using fallout radionuclides , 2010 .

[8]  D. Walling,et al.  Use of beryllium-7 to study the effectiveness of woody trash barriers in reducing sediment delivery to streams after forest clearcutting , 2010 .

[9]  Sheng Li,et al.  Using repeated measurements of 137Cs and modelling to identify spatial patterns of tillage and water erosion within potato production in Atlantic Canada , 2009 .

[10]  D. Walling,et al.  Extending the timescale for using beryllium 7 measurements to document soil redistribution by erosion , 2009 .

[11]  C. Renshaw,et al.  Flow and sediment regimes at tributary junctions on a regulated river: impact on sediment residence time and benthic macroinvertebrate communities , 2009 .

[12]  D. Walling,et al.  Comparative advantages and limitations of the fallout radionuclides (137)Cs, (210)Pb(ex) and (7)Be for assessing soil erosion and sedimentation. , 2008, Journal of environmental radioactivity.

[13]  Mark D. Tomer,et al.  Quantifying relative contributions from sediment sources in Conservation Effects Assessment Project watersheds , 2008, Journal of Soil and Water Conservation.

[14]  D. Walling,et al.  The catchment sediment budget as a management tool , 2008 .

[15]  D. Montgomery Soil erosion and agricultural sustainability , 2007, Proceedings of the National Academy of Sciences.

[16]  C. Renshaw,et al.  The use of short‐lived radionuclides to quantify transitional bed material transport in a regulated river , 2007 .

[17]  M. Baskaran,et al.  Seasonal variations on the residence times and partitioning of short-lived radionuclides (234Th, 7Be and 210Pb) and depositional fluxes of 7Be and 210Pb in Tampa Bay, Florida , 2007 .

[18]  D. Walling,et al.  Use of beryllium-7 to document soil redistribution following forest harvest operations. , 2006, Journal of environmental quality.

[19]  D. Walling,et al.  Partitioning the Contributions of Sheet and Rill Erosion Using Beryllium‐7 and Cesium‐137 , 2006 .

[20]  Christopher G. Wilson,et al.  The 7Be/210Pbxs ratio as an indicator of suspended sediment age or fraction new sediment in suspension , 2005 .

[21]  P. J. Whiting,et al.  Suspended sediment sources and transport distances in the Yellowstone River basin , 2005 .

[22]  P. J. Whiting,et al.  Short‐term erosion rates from a 7Be inventory balance , 2003 .

[23]  Andrew Parker,et al.  Pesticides and other micro-organic contaminants in freshwater sedimentary environments—a review , 2003 .

[24]  D. Walling,et al.  Using cosmogenic beryllium–7 as a tracer in sediment budget investigations , 2002 .

[25]  R. Kostaschuk,et al.  Rates of floodplain accretion in a tropical island river system impacted by cyclones and large floods , 2002 .

[26]  J. Carretero,et al.  Atmospheric deposition of 7Be at a coastal Mediterranean station , 2001 .

[27]  P. J. Whiting,et al.  Depth and areal extent of sheet and rill erosion based on radionuclides in soils and suspended sediment , 2001 .

[28]  J. Dominik,et al.  Factors controlling 7Be and 210Pb atmospheric deposition as revealed by sampling individual rain events in the region of Geneva, Switzerland. , 2001, Journal of environmental radioactivity.

[29]  P. Swarzenski,et al.  Beryllium-7 as a tracer of short-term sediment deposition and resuspension in the Fox River, Wisconsin. , 2001, Environmental science & technology.

[30]  Guebuem Kim,et al.  Factors Influencing the Atmospheric Depositional Fluxes of Stable Pb, 210Pb, and 7Be into Chesapeake Bay , 2000 .

[31]  Kazuko Megumi,et al.  Factors, especially sunspot number, causing variations in surface air concentrations and depositions of 7Be in Osaka, Japan , 2000 .

[32]  William H. Blake,et al.  Use of 7Be and 137Cs measurements to document short‐ and medium‐term rates of water‐induced soil erosion on agricultural land , 1999 .

[33]  D. Walling,et al.  Fallout beryllium-7 as a tracer in soil erosion investigations. , 1999, Applied radiation and isotopes : including data, instrumentation and methods for use in agriculture, industry and medicine.

[34]  K. Andersson,et al.  Radionuclide resuspension and mixed deposition at different heights , 1999 .

[35]  P. J. Whiting,et al.  Determining the times and distances of particle transit in a mountain stream using fallout radionuclides , 1999 .

[36]  M. Al-Masri,et al.  Fallout of7Be in Damascus City , 1998 .

[37]  D. Walling,et al.  Use of fallout 137Cs in investigations of overbank sediment deposition on river floodplains , 1997 .

[38]  G. R. Foster,et al.  Predicting soil erosion by water : a guide to conservation planning with the Revised Universal Soil Loss Equation (RUSLE) , 1997 .

[39]  P. Armitage,et al.  Biological Effects of Fine Sediment in the Lotic Environment , 1997, Environmental management.

[40]  A. Murray,et al.  Distribution and Variability of 7Be in Soils Under Different Surface Cover Conditions and its Potential for Describing Soil Redistribution Processes , 1996 .

[41]  D. Walling,et al.  Use of Fallout Pb-210 Measurements to Investigate Longer-Term Rates and Patterns of Overbank Sediment Deposition on the Floodplains of Lowland Rivers , 1996 .

[42]  L. Cantelli,et al.  Preliminary investigations on7Be as a tracer in the study of environmental processes , 1995 .

[43]  C. H. Coleman,et al.  Atmospheric depositional fluxes of 7Be and 210Pb at Galveston and College Station, Texas , 1993 .

[44]  P. Wallbrink,et al.  Use of fallout radionuclides as indicators of erosion processes , 1993 .

[45]  G. Wong,et al.  Atmospheric depositional characteristics of beryllium 7 and lead 210 along the southeastern Virginia coast , 1989 .

[46]  M. Harvey,et al.  7Be deposition in a high-rainfall area of New Zealand , 1989 .

[47]  J. Dibb Atmospheric deposition of beryllium 7 in the Chesapeake Bay region , 1989 .

[48]  A. I. Saleh,et al.  Beryllium-7 deposition at Fayetteville, Arkansas, and excess polonium-210 from the 1980 eruption of Mount St. Helens. , 1985 .

[49]  W. Casey,et al.  Atmospheric fluxes and marsh‐soil inventories of 7Be and 210Pb , 1985 .

[50]  K. Turekian,et al.  7Be and 210Pb total deposition fluxes at New Haven, Connecticut and at Bermuda , 1983 .

[51]  D. Lal,et al.  Annual fallout of32Si,210Pb,22Na,35S and7Be in rains in India , 1979 .

[52]  J. F. Bleichrodt,et al.  On the Deposition of Cosmic‐Ray‐Produced Beryllium 7 , 1963 .

[53]  D. Peirson Beryllium 7 in Ak and rain , 1963 .

[54]  M. Stoeppler,et al.  Beryllium 7 in the atmosphere , 1963 .

[55]  A. Walton,et al.  The deposition of beryllium 7 and phosphorus 32 in precipitation at north temperate latitudes , 1962 .

[56]  P. J. Whiting,et al.  Measuring Soil Erosion Rates Using Natural ( 7 Be, 210 Pb) and Anthropogenic ( 137 Cs, 239,240 Pu) Radionuclides , 2012 .

[57]  K. D. Denn Sediment budget closure during runoff-generated high flow events in the South Amana sub-watershed, IA , 2010 .

[58]  D. Walling Using fallout radionuclides to investigate erosion and sediment delivery: some recent advances , 2010 .

[59]  M. Nguyen,et al.  Chapter 7 Soil Erosion and Sedimentation Studies Using Environmental Radionuclides , 2009 .

[60]  D. Walling,et al.  Use of (7)Be to document soil erosion associated with a short period of extreme rainfall. , 2008, Journal of environmental radioactivity.

[61]  C. Doering Measurements of the distribution and behaviour of Beryllium-7 in the natural environment , 2007 .

[62]  D. Walling,et al.  Tracing versus monitoring: new challenges and opportunities in erosion and sediment delivery research. , 2006 .

[63]  A. Ioannidou,et al.  Precipitation scavenging of 7Be and 137Cs radionuclides in air. , 2006, Journal of environmental radioactivity.

[64]  Jon Brodie,et al.  Sources of sediment to the Great Barrier Reef World Heritage Area. , 2005, Marine pollution bulletin.

[65]  J. Ritchie,et al.  BIBLIOGRAPHY OF PUBLICATIONS OF 137 CESIUM STUDIES RELATED TO EROSION AND SEDIMENT DEPOSITION , 2004 .

[66]  F. Zapata,et al.  Handbook for the assessment of soil erosion and sedimentation using environmental radionuclides , 2003 .

[67]  S. Norton,et al.  Environmental Chemistry of Beryllium-7 , 2002 .

[68]  P. J. Whiting,et al.  Soil erosion and sediment sources in an Ohio watershed using beryllium-7, cesium-137, and lead-210. , 2002, Journal of environmental quality.

[69]  D. Walling,et al.  Conversion Models for Use in Soil-Erosion, Soil-Redistribution and Sedimentation Investigations , 2002 .

[70]  M. E. Brigham,et al.  Analysis of suspended-sediment concentrations and radioisotope levels in the Wild Rice River basin, northwestern Minnesota, 1973-98 , 2001 .

[71]  J. N. Smith,et al.  Why should we believe 210Pb sediment geochronologies? , 2001, Journal of environmental radioactivity.

[72]  A. Murray,et al.  Fallout of 7Be in South Eastern Australia , 1994 .

[73]  V. Nijampurkar,et al.  Polar fallout of radionuclides 32Si, 7Be and 210Pb and past accumulation rate of ice at Indian station, Dakshin Gangotri, East Antarctica , 1993 .

[74]  K. Bunzl,et al.  Background levels of atmospheric deposition to ground and temporal variation of 129I, 127I, 137Cs and 7Be in a rural area of Germany , 1992 .

[75]  D. Walling,et al.  Use of radiometric fingerprints to derive information on suspended sediment sources , 1992 .

[76]  J. Hayashi [Sampling methods]. , 1982, Josanpu zasshi = The Japanese journal for midwife.