Montreal Protocol Benefits simulated with CCM SOCOL

Abstract. Ozone depletion is caused by the anthropogenic increase of halogen-containing species in the atmosphere, which results in the enhancement of the concentration of reactive chlorine and bromine in the stratosphere. To reduce the influence of anthropogenic ozone-depleting substances (ODS), the Montreal Protocol was agreed by Governments in 1987, with several Amendments and Adjustments adopted later. In order to assess the benefits of the Montreal Protocol and its Amendments and Adjustments (MPA) on ozone and UV radiation, two different runs of the chemistry-climate model (CCM) SOCOL have been carried out. The first run was driven by the emission of ozone depleting substances (ODS) prescribed according to the restrictions of the MPA. For the second run we allow the ODS to grow by 3% annually. We find that the MPA would have saved up to 80% of the global annual total ozone by the end of the 21st century. Our calculations also show substantial changes of the stratospheric circulation pattern as well as in surface temperature and precipitations that could occur in the world without MPA implementations. To illustrate the changes in UV radiation at the surface and to emphasise certain features, which can only be seen for some particular regions if the influence of the cloud cover changes is accounted for, we calculate geographical distribution of the erythemally weighted irradiance ( E ery ). For the no Montreal Protocol simulation E ery increases by factor of 4 to 16 between the 1970s and 2100. For the scenario including the Montreal Protocol it is found that UV radiation starts to decrease in 2000, with continuous decline of 5% to 10% at middle latitudes in the both Northern and Southern Hemispheres.

[1]  D. Marsh,et al.  "World avoided" simulations with the Whole Atmosphere Community Climate Model , 2012 .

[2]  R. Seager,et al.  The Importance of the Montreal Protocol in Protecting Earth’s Hydroclimate , 2013 .

[3]  A. Smedley,et al.  Total ozone and surface UV trends in the United Kingdom: 1979–2008 , 2012 .

[4]  Philip J. Rasch Atmospheric General Circulation Modeling , 2012 .

[5]  T. Shepherd,et al.  Projections of UV radiation changes in the 21st century: impact of ozone recovery and cloud effects , 2011 .

[6]  R. McKenzie,et al.  UV impacts avoided by the Montreal Protocol , 2011, Photochemical & photobiological sciences : Official journal of the European Photochemistry Association and the European Society for Photobiology.

[7]  B. Mayer,et al.  Evaluation of radiation scheme performance within chemistry climate models , 2011 .

[8]  T. Shepherd,et al.  A Robust Mechanism for Strengthening of the Brewer–Dobson Circulation in Response to Climate Change: Critical-Layer Control of Subtropical Wave Breaking , 2011 .

[9]  Veronika Eyring,et al.  Multimodel climate and variability of the stratosphere , 2011 .

[10]  Veronika Eyring,et al.  Multi-model assessment of stratospheric ozone return dates and ozone recovery in CCMVal-2 models , 2010 .

[11]  Martyn P. Chipperfield,et al.  Anthropogenic forcing of the Northern Annular Mode in CCMVal-2 models , 2010 .

[12]  Veronika Eyring,et al.  Review of the formulation of present-generation stratospheric chemistry-climate models and associated external forcings , 2010 .

[13]  N. Gillett,et al.  Quantitative assessment of Southern Hemisphere ozone in chemistry-climate model simulations , 2010 .

[14]  Veronika Eyring,et al.  SPARC Report on the Evaluation of Chemistry-Climate Models , 2010 .

[15]  T. Shepherd,et al.  Large climate-induced changes in ultraviolet index and stratosphere-to-troposphere ozone flux , 2009 .

[16]  S. Brönnimann,et al.  Technical Note: Chemistry-climate model SOCOL: version 2.0 with improved transport and chemistry/microphysics schemes , 2008 .

[17]  L. Oman,et al.  What would have happened to the ozone layer if chlorofluorocarbons (CFCs) had not been regulated , 2008 .

[18]  P. Braesicke,et al.  The World Avoided by the Montreal Protocol , 2008 .

[19]  C. Brühl,et al.  Clear sky UV simulations for the 21st century based on ozone and temperature projections from Chemistry-Climate Models , 2008 .

[20]  C. Brühl,et al.  Multimodel projections of stratospheric ozone in the 21st century , 2007 .

[21]  David W. Fahey,et al.  The importance of the Montreal Protocol in protecting climate , 2007, Proceedings of the National Academy of Sciences.

[22]  K. Trenberth,et al.  Observations: Surface and Atmospheric Climate Change , 2007 .

[23]  W. Collins,et al.  Global climate projections , 2007 .

[24]  Volker Grewe,et al.  Assessment of temperature, trace species, and ozone in chemistry-climate model simulations of the recent past , 2006 .

[25]  Bernhard Mayer,et al.  Atmospheric Chemistry and Physics Technical Note: the Libradtran Software Package for Radiative Transfer Calculations – Description and Examples of Use , 2022 .

[26]  E. Manzini,et al.  Chemistry-climate model SOCOL: a validation of the present-day climatology , 2005 .

[27]  H. Slaper,et al.  UV radiation in the Netherlands: Assessing long‐term variability and trends in relation to ozone and clouds , 2005 .

[28]  Luis Kornblueh,et al.  The atmospheric general circulation model ECHAM5 Part II: Sensitivity of simulated climate to horizontal and vertical resolution , 2004 .

[29]  Greg E. Bodeker,et al.  Ozone profile differences between Europe and New Zealand: Effects on surface UV irradiance and its estimation from satellite sensors , 2003 .

[30]  Trends in Italian total cloud amount, 1951‐1996 , 2001 .

[31]  Michael E. Schlesinger,et al.  Assessment of the effect of the Montreal Protocol on atmospheric ozone , 2001 .

[32]  Michael E. Schlesinger,et al.  Hybrid scheme for three-dimensional advective transport , 1999 .

[33]  M. Schlesinger,et al.  The UIUC three‐dimensional stratospheric chemical transport model: Description and evaluation of the simulated source gases and ozone , 1999 .

[34]  N. McFarlane,et al.  Impact of the Doppler spread parameterization on the simulation of the middle atmosphere circulation using the MA/ECHAM4 general circulation model , 1997 .

[35]  S. Andersen,et al.  Ozone layer: the road not taken , 1996, Nature.

[36]  J. C. Leun,et al.  The Ozone Layer , 1990 .

[37]  E. Shettle Models of aerosols, clouds, and precipitation for atmospheric propagation studies , 1990 .

[38]  K. Stamnes,et al.  Numerically stable algorithm for discrete-ordinate-method radiative transfer in multiple scattering and emitting layered media. , 1988, Applied optics.

[39]  Eugene Leeb Ozone layer , 1988, Nature.

[40]  J. Farman,et al.  Large losses of total ozone in Antarctica reveal seasonal ClOx/NOx interaction , 1985, Nature.