Observation of collision induced processes in rubidium-ethane vapour

Abstract The collision-induced stimulated resonant emission on 5 2 P 1/2 –5 2 S 1/2 transition in rubidium vapour in the presence of ethane as a buffer gas is measured. This effect is investigated experimentally and analyzed theoretically in the small gain approximation. Within this approximation, the main differences between the generation of collision induced amplified spontaneous emission (ASE) signal in cesium–ethane, rubidium–ethane and sodium–ethane mixture were estimated. The dependencies of the ASE intensity on the energy of the laser pump and ethane pressure are measured and the efficiency of the ASE signal generation as a function of the exciting energy is given. The model of longitudinally pumped alkali metal–molecular gas amplifier was developed in order to explain the unusual behaviour of the dependence of the efficiency of the ASE signal generation in the rubidium–ethane mixture on the Gaussian pump beam exciting energy. Some analogies with erbium and ytterbium doped fiber amplification processes are given.

[1]  Shang-yi Ch'en,et al.  Broadening and Shift of Spectral Lines Due to the Presence of Foreign Gases , 1957 .

[2]  D. Hanna,et al.  Nonlinear Optics of Free Atoms and Molecules , 1980 .

[3]  Czub,et al.  Influence of resonant pulse propagation on collision-induced stimulated effects in the S1/2-P1/2,3/2 system. , 1996, Physical review. A, Atomic, molecular, and optical physics.

[4]  Z. Konefał,et al.  Stimulated processes in sodium vapour in the presence of molecular buffer gas systems , 1996 .

[5]  John Pitre,et al.  SENSITIZED FLUORESCENCE IN VAPORS OF ALKALI METALS: IX. ENERGY TRANSFER IN COLLISIONS BETWEEN SODIUM AND INERT GAS ATOMS , 1967 .

[6]  W. E. Baylis,et al.  Inelastic Collisions Between Excited Alkali Atoms and Molecules IX. An Isotope Effect in the Cross Sections for 62P1/2↔62P3/2 Mixing in Cesium, Induced in Collisions with Deuterated Methanes , 1974 .

[7]  Z Konefal,et al.  Temporal and spatial evolution of collision-induced stimulated effects in alkali atoms , 1998 .

[8]  M. Ignaciuk,et al.  Observation of collision-induced amplified emission in Na-noble gas system , 1993 .

[9]  M. Ignaciuk,et al.  Stimulated collision induced processes in sodium vapor in the presence of helium , 1990 .

[10]  L. Krause,et al.  Inelastic collisions between excited alkali atoms and molecules. VII. Sensitized fluorescence and quenching in mixtures of rubidium with H2, HD, D2, N2, CH4, CD4, C2H4, and C2.H6 , 1970 .

[11]  V. Kempter,et al.  Quenching cross sections for alkali-inert gas collisions , 1979 .

[12]  M. Ignaciuk,et al.  Investigation of collisionally induced stimulated scattering in sodium vapor with temporal and spectral resolution , 1995 .

[13]  L. Krause,et al.  SENSITIZED FLUORESCENCE IN VAPORS OF ALKALI METALS: VI. ENERGY TRANSFER IN COLLISIONS BETWEEN RUBIDIUM AND INERT GAS ATOMS , 1966 .

[14]  R. S. Quimby Output saturation in a 980-nm pumped erbium-doped fiber amplifier. , 1991, Applied optics.