Directeur de thèse

Al L2,3-edges from selected materials containing aluminum in different site geometries have been measured using high resolution X-ray absorption near edge structure (XANES) spectroscopy. The differences in both edge onset position and edge shape are explained in terms of chemical bonding and Al environment. The relative intensities of features at Al L2,3edge can be assigned to site distortion in the different geometries. The high resolution allows the calculation of electronic parameters such as the spin-orbit coupling and the exchange energy. Al L2,3 XANES of sodium aluminosilicate glasses shows that Al remains a network former during Fe for Al substitution, with an electronic structure similar to framework silicates.

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