High-Performance, Ultra-Broadband, Ultraviolet to Terahertz Photodetectors Based on Suspended Carbon Nanotube Films.

Ultra-broad spectral detection is critical for several technological applications in imaging, sensing, spectroscopy, and communication. Carbon nanotube (CNT) films are a promising material for ultra-broadband photodetectors because their absorption spectra cover the entire ultraviolet to the terahertz range. However, because of the high binding energy of excitons, photodetectors based on CNT films always require a strong electric field, asymmetric electrical contacts, or hybrid structures with other materials. Here, we report an ultra-broadband bolometric photodetector based on a suspended CNT film. With an abundant distribution of tube diameters and an appropriate morphology (spider web-like), the CNT films display a strong absorption spectrum from the ultraviolet up to the terahertz region. Under illumination, heat generated from the electron-photon interaction dominates the photoresponse of our devices. For small changes in temperature, the photocurrent shows a convincing linear dependence with the absorbed light's power across 3 orders of magnitude. When the channel length is reduced to 100 μm, the device demonstrates a high performance with an ultraviolet responsivity of up to 0.58 A/W with a bias voltage of 0.2 V and a short response time of ∼150 μs in vacuum, which is better than that of many other photodetectors based on CNTs. Moreover, this performance could be further enhanced by optimization.