Neutron Imaging at LANSCE - From Cold to Ultrafast

In recent years, neutron radiography and tomography have been applied at different beam lines at Los Alamos Neutron Science Center (LANSCE), covering a very wide neutron energy range. The field of energy-resolved neutron imaging with epi-thermal neutrons, utilizing neutron absorption resonances for contrast as well as quantitative density measurements, was pioneered at the Target 1 (Lujan center), Flight Path 5 beam line and continues to be refined. Applications include: imaging of metallic and ceramic nuclear fuels, fission gas measurements, tomography of fossils and studies of dopants in scintillators. The technique provides the ability to characterize materials opaque to thermal neutrons and to utilize neutron resonance analysis codes to quantify isotopes to within 0.1 atom %. The latter also allows measuring fuel enrichment levels or the pressure of fission gas remotely. More recently, the cold neutron spectrum at the ASTERIX beam line, also located at Target 1, was used to demonstrate phase contrast imaging with pulsed neutrons. This extends the capabilities for imaging of thin and transparent materials at LANSCE. In contrast, high-energy neutron imaging at LANSCE, using unmoderated fast spallation neutrons from Target 4 [Weapons Neutron Research (WNR) facility] has been developed for applications in imaging of dense, thick objects. Using fast (ns), time-of-flight imaging, enables testing and developing imaging at specific, selected MeV neutron energies. The 4FP-60R beam line has been reconfigured with increased shielding and new, larger collimation dedicated to fast neutron imaging. The exploration of ways in which pulsed neutron beams and the time-of-flight method can provide additional benefits is continuing. We will describe the facilities and instruments, present application examples and recent results of all these efforts at LANSCE.

[1]  Jeffrey J. Derby,et al.  In-Situ Observation of Phase Separation During Growth of Cs2LiLaBr6:Ce Crystals Using Energy-Resolved Neutron Imaging , 2017 .

[2]  Péter,et al.  Facilities , 1978, Higher Education Abstracts.

[3]  Eberhard H. Lehmann,et al.  Neutron Imaging Facilities in a Global Context , 2017, J. Imaging.

[4]  John V. Vallerga,et al.  High spatial resolution neutron sensing microchannel plate detectors , 2007 .

[5]  Michelle A. Espy,et al.  In vivo Observation of Tree Drought Response with Low-Field NMR and Neutron Imaging , 2016, Front. Plant Sci..

[6]  S. A. Werner,et al.  Imaging: Phase radiography with neutrons , 2000, Nature.

[7]  Jean-Baptiste Mouret,et al.  Discovery of a big void in Khufu’s Pyramid by observation of cosmic-ray muons , 2017, Nature.

[8]  Daniel S. Hussey,et al.  New neutron imaging facility at the NIST , 2005 .

[9]  Michal Mocko,et al.  Advantages and limitations of nuclear physics experiments at an ISIS-class spallation neutron source , 2008 .

[10]  Robert Bogue Detecting explosives and chemical weapons: a review of recent developments , 2015 .

[11]  Mark A.M. Bourke,et al.  Non-destructive studies of fuel pellets by neutron resonance absorption radiography and thermal neutron radiography , 2013 .

[12]  Takenao Shinohara,et al.  A new imaging method using pulsed neutron sources for visualizing structural and dynamical information , 2012 .

[13]  John Banhart,et al.  Neutron tomography instrument CONRAD at HZB , 2011 .

[14]  Richard N. Silver,et al.  The Los Alamos Neutron Scattering Center , 1986 .

[15]  Michael A. Forster How Reliable Are Heat Pulse Velocity Methods for Estimating Tree Transpiration , 2017 .

[16]  Anton S. Tremsin,et al.  Spatially resolved remote measurement of temperature by neutron resonance absorption , 2015 .

[17]  J. E. Lynn,et al.  Resonance neutron methods for determining statistical properties of phonon spectra , 1996 .

[18]  Nares Chankow,et al.  Neutron radiography. , 1969, British medical journal.

[19]  F. Merrill,et al.  Qualitative comparison of bremsstrahlung X-rays and 800 MeV protons for tomography of urania fuel pellets. , 2013, The Review of scientific instruments.

[20]  E. Ables,et al.  An 800-MeV proton radiography facility for dynamic experiments , 1998 .

[21]  R. D. Sachs,et al.  Fail-safe neutron shutter used for thermal neutron radiography , 1976 .

[22]  George J. Yates,et al.  High energy neutron radiography , 1996 .

[23]  Adrian S. Losko,et al.  In situ diagnostics of the crystal-growth process through neutron imaging: application to scintillators , 2016, Journal of applied crystallography.

[24]  Andrea Favalli,et al.  Neutron imaging with the short-pulse laser driven neutron source at the Trident laser facility , 2016 .

[25]  L. Grodzins,et al.  Nuclear techniques for finding chemical explosives in airport luggage , 1991 .

[26]  Richard M. Ambrosi,et al.  Optimisation of resolution in accelerator-based fast neutron radiography , 2002 .

[27]  Kurt F. Schoenberg,et al.  The Los Alamos Neutron Science Center , 2006 .

[28]  Mark A.M. Bourke,et al.  Real-time Crystal Growth Visualization and Quantification by Energy-Resolved Neutron Imaging , 2017, Scientific Reports.

[29]  Frank J Vergeldt,et al.  MRI of long-distance water transport: a comparison of the phloem and xylem flow characteristics and dynamics in poplar, castor bean, tomato and tobacco. , 2006, Plant, cell & environment.

[30]  Amanda C. Madden,et al.  Detector Performance for Fast Neutron Radiography and Computed Tomography , 2017, 2017 IEEE Nuclear Science Symposium and Medical Imaging Conference (NSS/MIC).

[31]  Burkhard Schillinger,et al.  New design for the ANTARES-II facility for neutron imaging at FRM II , 2009 .

[32]  Amanda C. Madden,et al.  Development and Characterization of a High-Energy Neutron Time-of-Flight Imaging System , 2017, IEEE Transactions on Nuclear Science.

[33]  Konstantin N. Borozdin,et al.  Surveillance: Radiographic imaging with cosmic-ray muons , 2003, Nature.

[34]  Walter J. Trela,et al.  Neutron Doppler broadening studies of tantalum and tungsten metal , 2002 .

[35]  H. Iwasa,et al.  Characteristics of a New Type Neutron Radiography Using Time-of-Flight Method , 2004 .

[36]  Fujio Maekawa,et al.  Measurement of neutron beam characteristics at the Manuel Lujan Jr. neutron scattering center , 2004 .

[37]  Richard M. Ambrosi,et al.  FACTORS AFFECTING IMAGE FORMATION IN ACCELERATOR-BASED FAST NEUTRON RADIOGRAPHY , 1998 .

[38]  C. Grünzweig,et al.  The ICON beamline – A facility for cold neutron imaging at SINQ , 2011 .

[39]  T. N. Claytor,et al.  High-energy and thermal-neutron imaging and modeling with an amorphous silicon flat-panel detector. , 2001, Applied radiation and isotopes : including data, instrumentation and methods for use in agriculture, industry and medicine.

[40]  J. E. Lynn,et al.  Vibrational properties of Pu and Ga in a Pu-Ga alloy from neutron-resonance Doppler spectroscopy , 1998 .

[41]  Adrian S. Losko,et al.  Non-Destructive Study of Bulk Crystallinity and Elemental Composition of Natural Gold Single Crystal Samples by Energy-Resolved Neutron Imaging , 2017, Scientific Reports.

[42]  Kenzo Miya,et al.  A study on the development of a fast neutron television converter , 1993 .

[43]  Danas Ridikas,et al.  Status and Perspectives of Neutron Imaging Facilities , 2017 .

[44]  Jason McPhate,et al.  Improved efficiency of high resolution thermal and cold neutron imaging , 2011 .

[45]  J. A. James,et al.  IMAT – A New Imaging and Diffraction Instrument at ISIS☆ , 2013 .

[46]  J P Quintana,et al.  Shock temperature measurement using neutron resonance spectroscopy. , 2005, Physical review letters.

[47]  Andrea Favalli,et al.  Bright laser-driven neutron source based on the relativistic transparency of solids. , 2013, Physical review letters.

[48]  John S. Hendricks,et al.  Initial MCNP6 Release Overview , 2012 .

[49]  I. Mor,et al.  Fast Neutron Tomography of Low-Z Object in High-Z Material Shielding , 2015 .

[50]  Ulrich Bonse,et al.  Imaging of ferromagnetic domains by neutron interferometry , 1980 .

[51]  Susumu Ikeda,et al.  Direct Observation of Effective Temperature of Ta Atom in Layer Compound TaS2 by Neutron Resonance Absorption Spectrometer , 2001 .

[52]  Takeshi Nakatani,et al.  Final design of the Energy-Resolved Neutron Imaging System “RADEN” at J-PARC , 2016 .

[53]  E. Guardincerri,et al.  Imaging the inside of thick structures using cosmic rays , 2016 .

[54]  J. P. Barton,et al.  Multi-purpose neutron radiography system , 1996 .

[55]  W. R. N. Edwards,et al.  A method for measuring radial differences in water content of intact tree stems by attenuation of gamma radiation , 1983 .

[56]  J A Anderson,et al.  Search for hidden chambers in the pyramids. , 1970, Science.

[57]  Kenji Iwase,et al.  Imaging of a spatial distribution of preferred orientation of crystallites by pulsed neutron Bragg edge transmission , 2010 .

[58]  I. Mor,et al.  Novel detectors for fast-neutron resonance radiography , 2010 .

[59]  Brian Temple,et al.  Time gating for energy selection and scatter rejection: High-energy pulsed neutron imaging at LANSCE , 2015, SPIE Optical Engineering + Applications.

[60]  C. D. Bowman,et al.  The Los Alamos National Laboratory Spallation Neutron Sources , 1990 .

[61]  H. Kallmann Neutron radiography: by Harold Berger. 146 pages, diagrams, illustr. 6 × 9 in. New York, American Elsevier Pub., Co., 1965. Price, $9.00 , 1966 .

[62]  Jack S. Brenizer,et al.  A Review of Significant Advances in Neutron Imaging from Conception to the Present , 2013 .

[63]  P. Vontobel,et al.  PROPERTIES OF THE RADIOGRAPHY FACILITY NEUTRA AT SINQ AND ITS POTENTIAL FOR USE AS EUROPEAN REFERENCE FACILITY , 2001 .

[64]  T. N. Claytor,et al.  Time-gated energy-selected cold neutron radiography , 1998 .

[65]  Richard M. Ambrosi,et al.  The effect of the imaging geometry and the impact of neutron scatter on the detection of small features in accelerator-based fast neutron radiography , 2004 .

[66]  Andrea Favalli,et al.  Laser-plasmas in the relativistic-transparency regime: Science and applications , 2017, Physics of plasmas.

[67]  C. M. Frankle,et al.  A high-rate 10B-loaded liquid scintillation detector for parity-violation studies in neutron resonances , 2000 .

[68]  N. M. Larson,et al.  Updated Users' Guide for SAMMY Multilevel R-matrix Fits to Neutron Data Using Bayes' Equation , 1998 .

[69]  Konstantin N. Borozdin,et al.  Analysis of muon radiography of the Toshiba nuclear critical assembly reactor , 2014 .

[70]  Harold Berger,et al.  NEUTRON RADIOGRAPHY Methods, Capabilities, and Applications , 1965 .

[71]  R. G. Downing,et al.  Efficiency optimization of microchannel plate (MCP) neutron imaging detectors. I. Square channels with 10B doping , 2005 .

[72]  Nikolay Kardjilov,et al.  High-resolution investigations of edge effects in neutron imaging , 2009 .

[73]  Michihiro Furusaka,et al.  High wavelength-resolution Bragg-edge/dip transmission imaging instrument with a supermirror guide-tube coupled to a decoupled thermal-neutron moderator at Hokkaido University Neutron Source , 2017, Physica B: Condensed Matter.

[74]  J. V. Vallerga,et al.  Non-contact measurement of partial gas pressure and distribution of elemental composition using energy-resolved neutron imaging , 2017 .