Coherent injection locking of quantum cascade laser frequency combs

Quantum cascade laser (QCL) frequency combs are a promising candidate for chemical sensing and biomedical diagnostics1–4. They are electrically pumped and compact, making them an ideal platform for on-chip integration5. Until now, optical feedback is fatal for frequency comb generation in QCLs6. This property limits the potential for integration. Here, we demonstrate coherent electrical injection locking of the repetition frequency to a stabilized radio-frequency oscillator. We prove that the injection-locked QCL spectrum can be phase-locked, resulting in the generation of a frequency comb. We show that injection locking is not only a versatile tool for all-electrical frequency stabilization, but also mitigates the fatal effect of optical feedback. A prototype self-detected dual-comb set-up consisting only of an injection-locked dual-comb chip, a lens and a mirror demonstrates the enormous potential for on-chip dual-comb spectroscopy. These results pave the way to miniaturized and all-solid-state mid-infrared spectrometers.Quantum cascade laser frequency combs are coherently locked to an external radio-frequency source even in extremely high-feedback conditions. The internal phase-locking mechanism and the possibility of all-electric stabilization are investigated.

[1]  F. Tittel,et al.  Quartz-enhanced photoacoustic spectroscopy-based sensor system for sulfur dioxide detection using a CW DFB-QCL , 2014 .

[2]  D. Kane,et al.  Characterization of arbitrary femtosecond pulses using frequency-resolved optical gating , 1993 .

[3]  Thomas Udem,et al.  Cavity-enhanced dual-comb spectroscopy , 2009, 0908.1928.

[4]  T. Hänsch,et al.  Optical frequency metrology , 2002, Nature.

[5]  Mattias Beck,et al.  Evidence of linear chirp in mid-infrared quantum cascade lasers , 2018, Optica.

[6]  J. Faist,et al.  Quantum Cascade Laser , 1994, Science.

[7]  Theodor W. Hänsch,et al.  Absolute Optical Frequency Measurement of the Cesium D 1 Line with a Mode-Locked Laser , 1999 .

[8]  Jerome Faist,et al.  Dual-comb spectroscopy based on quantum-cascade-laser frequency combs , 2014, Nature Communications.

[9]  Boris Mizaikoff,et al.  Advances in Mid-Infrared Spectroscopy for Chemical Analysis. , 2016, Annual review of analytical chemistry.

[10]  Federico Capasso,et al.  Time-dependent population inversion gratings in laser frequency combs , 2018 .

[11]  I. Walmsley,et al.  Spectral phase interferometry for direct electric-field reconstruction of ultrashort optical pulses. , 1998, Optics letters.

[12]  Peter Friedli,et al.  Four-wave mixing in a quantum cascade laser amplifier , 2013 .

[13]  B. Razavi A study of injection locking and pulling in oscillators , 2004, IEEE Journal of Solid-State Circuits.

[14]  Qing Hu,et al.  Terahertz laser frequency combs , 2014 .

[15]  Yamac Dikmelik,et al.  Coherent frequency combs produced by self frequency modulation in quantum cascade lasers , 2014 .

[16]  J. Faist,et al.  Mid-infrared frequency comb based on a quantum cascade laser , 2012, Nature.

[17]  J. Faist,et al.  Quantum Cascade Laser , 1994, Science.

[18]  Mattias Beck,et al.  On-chip dual-comb based on quantum cascade laser frequency combs , 2015, 1510.09158.

[19]  C. Zah,et al.  Single-mode instability in standing-wave lasers: The quantum cascade laser as a self-pumped parametric oscillator , 2016, 1711.00187.

[20]  Yang Yang,et al.  Computational multiheterodyne spectroscopy , 2016, Science Advances.

[21]  Werner Schrenk,et al.  Monolithically integrated mid-infrared lab-on-a-chip using plasmonics and quantum cascade structures , 2014, Nature Communications.

[22]  Carlo Sirtori,et al.  Coherent sampling of active mode-locked terahertz quantum cascade lasers and frequency synthesis , 2011 .

[23]  Yves Bidaux,et al.  Dual comb operation of λ ̃ 8.2 μm quantum cascade laser frequency comb with 1 W optical power , 2017 .

[24]  Knight,et al.  Optical frequency synthesizer for precision spectroscopy , 2000, Physical review letters.

[25]  A. Bismuto,et al.  Injection locking of mid‐infrared quantum cascade laser at 14 GHz, by direct microwave modulation , 2014 .

[26]  I. Sagnes,et al.  Injection-locking of terahertz quantum cascade lasers up to 35GHz via RF amplitude modulation , 2010, 35th International Conference on Infrared, Millimeter, and Terahertz Waves.

[27]  Yang Yang,et al.  Evaluating the coherence and time-domain profile of quantum cascade laser frequency combs. , 2015, Optics express.

[28]  Mattias Beck,et al.  Quantum Cascade Laser Frequency Combs , 2015, 1510.09075.