Multiple tuning of magnetic biskyrmions using in situ L-TEM in centrosymmetric MnNiGa alloy

Magnetic skyrmions are topologically protected spin configurations and have recently received growingly attention in magnetic materials. The existence of biskyrmions within a broad temperature range has been identified in our newly-discovered MnNiGa material, promising for potential application in physics and technological study. Here, the biskyrmion microscopic origination from the spin configuration evolution of stripe ground state is experimentally identified. The biskyrmion manipulations based on the influences of the basic microstructures and external factors such as grain boundary confinement, sample thickness, electric current, magnetic field and temperature have been systematically studied by using real-space Lorentz transmission electron microscopy. These multiple tuning options help to understand the essential properties of MnNiGa and predict a significant step forward for the realization of skyrmion-based spintronic devices.

[1]  Kazuo Ishizuka,et al.  Phase measurement of atomic resolution image using transport of intensity equation. , 2005, Journal of electron microscopy.

[2]  Y. Tokura,et al.  Magnetic stripes and skyrmions with helicity reversals , 2012, Proceedings of the National Academy of Sciences.

[3]  Y. Tokura,et al.  Thermally activated helicity reversals of skyrmions , 2016 .

[4]  Kang L. Wang,et al.  Blowing magnetic skyrmion bubbles , 2015, Science.

[5]  Y. Tokura,et al.  Lorentz transmission electron microscopy on nanometric magnetic bubbles and skyrmions in bilayered manganites La1.2Sr1.8(Mn1−yRuy)2O7 with controlled magnetic anisotropy , 2015 .

[6]  P. Fischer,et al.  Synthesizing skyrmion bound pairs in Fe-Gd thin films , 2016, 1603.07882.

[7]  Run‐Wei Li,et al.  Experimental realization of two-dimensional artificial skyrmion crystals at room temperature , 2014 .

[8]  D. Wu,et al.  Creating an artificial two-dimensional Skyrmion crystal by nanopatterning. , 2013, Physical review letters.

[9]  S. Mitsudo,et al.  Structural and magnetic properties of Ni2In type (Mn1 − xNix)65Ga35 compounds , 1999 .

[10]  Young Sun,et al.  Real-Space Observation of Nonvolatile Zero-Field Biskyrmion Lattice Generation in MnNiGa Magnet. , 2017, Nano letters.

[11]  Theory of helical spin crystals: Phases, textures, and properties , 2006, cond-mat/0608128.

[12]  T. Skyrme A Unified Field Theory of Mesons and Baryons , 1962 .

[13]  Yu-heng Zhang,et al.  Enhanced Stability of the Magnetic Skyrmion Lattice Phase under a Tilted Magnetic Field in a Two-Dimensional Chiral Magnet. , 2017, Nano letters.

[14]  Y. Tokura,et al.  Variation of skyrmion forms and their stability in MnSi thin plates , 2015 .

[15]  C. Pfleiderer,et al.  Spontaneous skyrmion ground states in magnetic metals , 2006, Nature.

[16]  Y. Tokura,et al.  Interplay between topological and thermodynamic stability in a metastable magnetic skyrmion lattice , 2016 .

[17]  Y. Tokura,et al.  Biskyrmion states and their current-driven motion in a layered manganite , 2014, Nature Communications.

[18]  A. Saxena,et al.  Noncircular skyrmion and its anisotropic response in thin films of chiral magnets under a tilted magnetic field , 2015, 1508.06361.

[19]  Mark L. Vousden,et al.  Ground state search, hysteretic behaviour, and reversal mechanism of skyrmionic textures in confined helimagnetic nanostructures , 2013, Scientific Reports.

[20]  P. Böni,et al.  Spin Transfer Torques in MnSi at Ultralow Current Densities , 2010, Science.

[21]  Y. Tokura,et al.  Gauge fields in real and momentum spaces in magnets: monopoles and skyrmions , 2012, Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences.

[22]  Current-driven dynamics of skyrmions stabilized in MnSi nanowires revealed by topological Hall effect , 2015, Nature communications.

[23]  F. Hu,et al.  A Centrosymmetric Hexagonal Magnet with Superstable Biskyrmion Magnetic Nanodomains in a Wide Temperature Range of 100–340 K , 2016, Advanced materials.

[24]  Yu-heng Zhang,et al.  Edge-mediated skyrmion chain and its collective dynamics in a confined geometry , 2015, Nature Communications.

[25]  P. Böni,et al.  Topological Hall effect in the A phase of MnSi. , 2009, Physical review letters.

[26]  A. Fert,et al.  Skyrmions on the track. , 2013, Nature nanotechnology.

[27]  Y. Tokura,et al.  Topological properties and dynamics of magnetic skyrmions. , 2013, Nature nanotechnology.

[28]  Y. Tokura,et al.  Skyrmion flow near room temperature in an ultralow current density , 2012, Nature Communications.

[29]  Shizeng Lin Edge instability in a chiral stripe domain under an electric current and skyrmion generation , 2015, 1510.07353.

[30]  C. Marrows,et al.  Magnetic microscopy and topological stability of homochiral Néel domain walls in a Pt/Co/AlOx trilayer , 2015, Nature Communications.

[31]  S. Nasu,et al.  Real-space observation of current-driven domain wall motion in submicron magnetic wires. , 2003, Physical review letters.

[32]  Y. Tokura,et al.  Real-space observation of a two-dimensional skyrmion crystal , 2010, Nature.

[33]  Yu-heng Zhang,et al.  Direct Imaging of a Zero-Field Target Skyrmion and Its Polarity Switch in a Chiral Magnetic Nanodisk. , 2017, Physical review letters.

[34]  P. Grundy,et al.  Lorentz microscopy of bubble domains and changes in domain wall state in hexaferrites , 1973 .

[35]  N. Nagaosa,et al.  Theory of antiskyrmions in magnets , 2016, Nature Communications.

[36]  M. Kramer,et al.  Generation of high-density biskyrmions by electric current , 2017, npj Quantum Materials.