Macroscopic yielding in jammed solids is accompanied by a nonequilibrium first-order transition in particle trajectories.

We use computer simulations to analyze the yielding transition during large-amplitude oscillatory shear of a simple model for soft jammed solids. Simultaneous analysis of global mechanical response and particle-scale motion demonstrates that macroscopic yielding, revealed by a smooth crossover in mechanical properties, is accompanied by a sudden change in the particle dynamics, which evolves from nondiffusive motion to irreversible diffusion as the amplitude of the shear is increased. We provide numerical evidence that this sharp change corresponds to a nonequilibrium first-order dynamic phase transition, thus establishing the existence of a well-defined microscopic dynamic signature of the yielding transition in amorphous materials in oscillatory shear.

[1]  R. Sarpong,et al.  Bio-inspired synthesis of xishacorenes A, B, and C, and a new congener from fuscol† †Electronic supplementary information (ESI) available. See DOI: 10.1039/c9sc02572c , 2019, Chemical science.

[2]  K. Dahmen,et al.  Reversibility and criticality in amorphous solids , 2015, Nature Communications.

[3]  P. Schall,et al.  Sharp symmetry-change marks the mechanical failure transition of glasses , 2015, Scientific Reports.

[4]  Ludovic Berthier,et al.  Hyperuniform density fluctuations and diverging dynamic correlations in periodically driven colloidal suspensions. , 2015, Physical review letters.

[5]  Ludovic Berthier,et al.  Diverging viscosity and soft granular rheology in non-Brownian suspensions. , 2014, Physical review. E, Statistical, nonlinear, and soft matter physics.

[6]  Suresh Narayanan,et al.  Echoes in x-ray speckles track nanometer-scale plastic events in colloidal gels under shear. , 2014, Physical review. E, Statistical, nonlinear, and soft matter physics.

[7]  R. Ganapathy,et al.  Experimental signatures of a nonequilibrium phase transition governing the yielding of a soft glass. , 2014, Physical review. E, Statistical, nonlinear, and soft matter physics.

[8]  E. Bouchbinder,et al.  Variable-amplitude oscillatory shear response of amorphous materials. , 2014, Physical review. E, Statistical, nonlinear, and soft matter physics.

[9]  L. Cipelletti,et al.  A microscopic view of the yielding transition in concentrated emulsions. , 2014, Soft matter.

[10]  D. M. Miedema,et al.  Shear banding of colloidal glasses: observation of a dynamic first-order transition. , 2014, Physical review letters.

[11]  C. E. Fiore Minimal mechanism leading to discontinuous phase transitions for short-range systems with absorbing states. , 2013, Physical review. E, Statistical, nonlinear, and soft matter physics.

[12]  Nathan C Keim,et al.  Mechanical and microscopic properties of the reversible plastic regime in a 2D jammed material. , 2013, Physical review letters.

[13]  R. Bonnecaze,et al.  Local mobility and microstructure in periodically sheared soft particle glasses and their connection to macroscopic rheology , 2013 .

[14]  P. Arratia,et al.  Yielding and microstructure in a 2D jammed material under shear deformation , 2013, 1304.2253.

[15]  S. Sastry,et al.  Oscillatory athermal quasistatic deformation of a model glass. , 2013, Physical review. E, Statistical, nonlinear, and soft matter physics.

[16]  J. Brady,et al.  Complex oscillatory yielding of model hard-sphere glasses. , 2013, Physical review letters.

[17]  C. O’Hern,et al.  Particle-scale reversibility in athermal particulate media below jamming. , 2013, Physical review. E, Statistical, nonlinear, and soft matter physics.

[18]  T. Lookman,et al.  Onset of irreversibility and chaos in amorphous solids under periodic shear. , 2013, Physical review. E, Statistical, nonlinear, and soft matter physics.

[19]  Nikolai V Priezjev Heterogeneous relaxation dynamics in amorphous materials under cyclic loading. , 2013, Physical review. E, Statistical, nonlinear, and soft matter physics.

[20]  S-L-Y Xu,et al.  Contact processes in crowded environments. , 2012, Physical review. E, Statistical, nonlinear, and soft matter physics.

[21]  Michelle Girvan,et al.  Onset of irreversibility in cyclic shear of granular packings. , 2011, Physical review. E, Statistical, nonlinear, and soft matter physics.

[22]  Gareth H. McKinley,et al.  A review of nonlinear oscillatory shear tests: Analysis and application of large amplitude oscillatory shear (LAOS) , 2011 .

[23]  G. Biroli,et al.  Theoretical perspective on the glass transition and amorphous materials , 2010, 1011.2578.

[24]  M. Wilhelm,et al.  Nonlinear response of dense colloidal suspensions under oscillatory shear: mode-coupling theory and Fourier transform rheology experiments. , 2010, Physical review. E, Statistical, nonlinear, and soft matter physics.

[25]  J. R. Bruyn,et al.  Rheological and microrheological measurements of soft condensed matter , 2010 .

[26]  J. Gollub,et al.  Random organization in periodically driven systems , 2008 .

[27]  C. O’Hern,et al.  Reversible plasticity in amorphous materials , 2007 .

[28]  J. F. Brady,et al.  Chaos and threshold for irreversibility in sheared suspensions , 2005, Nature.

[29]  R. Spigler,et al.  The Kuramoto model: A simple paradigm for synchronization phenomena , 2005 .

[30]  P. Pusey,et al.  Rearrangements in hard-sphere glasses under oscillatory shear strain. , 2002, Physical review. E, Statistical, nonlinear, and soft matter physics.

[31]  H. Hinrichsen Non-equilibrium critical phenomena and phase transitions into absorbing states , 2000, cond-mat/0001070.

[32]  Peter Sollich Rheological constitutive equation for a model of soft glassy materials , 1997, cond-mat/9712001.

[33]  David J. Pine,et al.  Yielding and Rearrangements in Disordered Emulsions , 1997 .

[34]  D. Weitz,et al.  Yielding and flow of monodisperse emulsions , 1996 .

[35]  D. Durian,et al.  Foam mechanics at the bubble scale. , 1995, Physical review letters.