Sediment fingerprinting to determine the source of suspended sediment in a southern Piedmont stream.

Thousands of stream miles in the southern Piedmont region are impaired because of high levels of suspended sediment. It is unclear if the source is upland erosion from agricultural sources or bank erosion of historic sediment deposited in the flood plains between 1830 and 1930 when cotton farming was extensive. The objective of this study was to determine the source of high stream suspended sediment concentrations in a typical southern Piedmont watershed using sediment fingerprinting techniques. Twenty-one potential tracers were tested for their ability to discriminate between sources, conservative behavior, and lack of redundancy. Tracer concentrations were determined in potential sediment sources (forests, pastures, row crop fields, stream banks, and unpaved roads and construction sites), and suspended sediment samples collected from the stream and analyzed using mixing models. Results indicated that 137Cs and 15N were the best tracers to discriminate potential sediment sources in this watershed. The delta15N values showed distinct signatures in all the potential suspended sediment sources, and delta15N was a unique tracer to differentiate stream bank soil from upland subsurface soils, such as soil from construction sites, unpaved roads, ditches, and field gullies. Mixing models showed that about 60% of the stream suspended sediment originated from eroding stream banks, 23 to 30% from upland subsoil sources (e.g., construction sites and unpaved roads), and about 10 to 15% from pastures. The results may be applicable to other watersheds in the Piedmont depending on the extent of urbanization occurring in these watersheds. Better understanding of the sources of fine sediment has practical implications on the type of sediment control measures to be adopted. Investment of resources in improving water quality should consider the factors causing stream bank erosion and erosion from unpaved roads and construction sites to water quality impairment.

[1]  I. Foster,et al.  Sediment and water quality in river catchments , 1995 .

[2]  D. Adriano Trace elements in terrestrial environments , 2001 .

[3]  C. Leibundgut,et al.  Tracers in Hydrology , 2009 .

[4]  G. Bouyoucos DIRECTIONS FOR MAKING MECHANICAL ANALYSES OF SOILS BY THE HYDROMETER METHOD , 1936 .

[5]  J. Lewin,et al.  Source identification for suspended sediments , 1980 .

[6]  D. Walling,et al.  Selecting fingerprint properties for discriminating potential suspended sediment sources in river basins , 2002 .

[7]  D. Walling,et al.  USE OF COMPOSITE FINGERPRINTS TO DETERMINE THE PROVENANCE OF THE CONTEMPORARY SUSPENDED SEDIMENT LOAD TRANSPORTED BY RIVERS , 1998 .

[8]  F. Zapata The use of environmental radionuclides as tracers in soil erosion and sedimentation investigations: recent advances and future developments , 2003 .

[9]  Evalyn Irene Albright Background concentrations of trace elements in soils and rocks of the Georgia piedmont , 2004 .

[10]  J. Ritchie,et al.  137Cesium and soil carbon in a small agricultural watershed , 2003 .

[11]  A. Austin,et al.  Global patterns of the isotopic composition of soil and plant nitrogen , 2003 .

[12]  D. Leigh MERCURY CONTAMINATION AND FLOODPLAIN SEDIMENTATION FROM FORMER GOLD MINES IN NORTH GEORGIA , 1994 .

[13]  M. Gavrilescu,et al.  Characterization and remediation of soils contaminated with uranium. , 2009, Journal of hazardous materials.

[14]  A. Simon,et al.  Disturbance, stream incision, and channel evolution: The roles of excess transport capacity and boundary materials in controlling channel response , 2006 .

[15]  W Muschack,et al.  Pollution of street run-off by traffic and local conditions. , 1990, The Science of the total environment.

[16]  D. Rennie,et al.  CHANGES IN NATURAL 15N ABUNDANCE ASSOCIATED WITH PEDOGENIC PROCESSES IN SOIL. II. CHANGES ON DIFFERENT SLOPE POSITIONS , 1980 .

[17]  M. Nearing,et al.  Multi‐year tracking of sediment sources in a small agricultural watershed using rare earth elements , 2005 .

[18]  A. Nicholas,et al.  A multi-parameter approach to fingerprinting suspended-sediment sources , 1993 .

[19]  S. Carpenter,et al.  NONPOINT POLLUTION OF SURFACE WATERS WITH PHOSPHORUS AND NITROGEN , 1998 .

[20]  J. McDonnell,et al.  Quantifying contributions to storm runoff through end‐member mixing analysis and hydrologic measurements at the Panola Mountain Research Watershed (Georgia, USA) , 2001 .

[21]  A. Papanicolaou,et al.  The Use of Carbon and Nitrogen Isotopes to Study Watershed Erosion Processes 1 , 2007 .

[22]  J. Ritchie,et al.  Wheat field erosion rates and channel bottom sediment sources in an intensively cropped northeastern Oregon drainage basin , 2004 .

[23]  A. Papanicolaou,et al.  Application of the spatial distribution of nitrogen stable isotopes for sediment tracing at the watershed scale , 2008 .

[24]  A. G. Brown The potential use of pollen in the identification of suspended sediment sources , 1985 .

[25]  D. Walling Tracing suspended sediment sources in catchments and river systems. , 2005, The Science of the total environment.

[26]  Desmond E. Walling,et al.  Fingerprinting suspended sediment sources in the catchment of the River Ouse, Yorkshire, UK , 1999 .

[27]  S. Hayes,et al.  Polyacrylamide Use for Erosion and Turbidity Control on Construction Sites , 2005 .

[28]  Domy C. Adriano,et al.  Trace Elements in Terrestrial Environments: Biogeochemistry, Bioavailability, and Risks of Metals , 2001 .

[29]  D. Merritts,et al.  Natural Streams and the Legacy of Water-Powered Mills , 2008, Science.

[30]  D. Walling,et al.  Use of floodplain sediment cores to investigate recent historical changes in overbank sedimentation rates and sediment sources in the catchment of the River Ouse, Yorkshire, UK , 1999 .

[31]  S. Billings,et al.  Incorporation of Plant Residues into Soil Organic Matter Fractions With Grassland Management Practices in the North American Midwest , 2006, Ecosystems.

[32]  S. Trimble,et al.  Man-induced soil erosion on the Southern Piedmont, 1700-1970. , 2008 .

[33]  D. Richter,et al.  Changes in stable isotopic signatures of soil nitrogen and carbon during 40 years of forest development , 2006, Oecologia.

[34]  Watershed Effects on Streamflow Quantity and Quality in Six Watersheds of Gwinnett County, Georgia , 2007 .

[35]  R. Naiman,et al.  Biophysical interactions and the structure and dynamics of riverine ecosystems: the importance of biotic feedbacks , 1999, Hydrobiologia.

[36]  D. Walling USING ENVIRONMENTAL RADIONUCLIDES TO TRACE SEDIMENT MOBILISATION AND DELIVERY IN RIVER BASINS AS AN AID TO CATCHMENT MANAGEMENT , 2004 .

[37]  D. Rennie,et al.  Changes in natural 15N abundance associated with pedogenic processes in soil. I. Changes associated with saline seeps. , 1980 .

[38]  J. Meyer,et al.  Streams in the Urban Landscape , 2001 .

[39]  H. Shugart,et al.  Insights into nitrogen and carbon dynamics of ectomycorrhizal and saprotrophic fungi from isotopic evidence , 1999, Oecologia.

[40]  Wade L. Nutter,et al.  CHANNEL MORPHOLOGY EVOLUTION AND OVERBANK FLOW IN THE GEORGIA PIEDMONT 1 , 1999 .

[41]  Richard P. Hooper,et al.  Multivariate analysis of stream water chemical data: The use of principal components analysis for the end‐member mixing problem , 1992 .

[42]  Monitoring, modeling, and fingerprinting suspended sediment in a southern Piedmont stream , 2009 .

[43]  M. Wolman,et al.  Effects of construction on fluvial sediment, urban and suburban areas of Maryland , 1967 .

[44]  J. Ritchie,et al.  Soil and soil organic carbon redistribution on the landscape , 2007 .

[45]  J. Walden,et al.  Use of mineral magnetic measurements to fingerprint suspended sediment sources: approaches and techniques for data analysis , 1997 .