Growth evolution of ZnO films deposited by pulsed laser ablation

We study the surface morphology evolution of ZnO films grown by pulsed laser deposition. Atomic force microscopy measurements show the existence of two growth regimes. Initially, the growth morphology is determined by shadowing effects due to the angular spreading of the plume in the 0.1 mbar oxygen working pressure. For longer deposition times a stepped pyramid-like structure is developed, whose roughening and coarsening behaviours are in agreement with those expected for growth systems with step-edge barriers.

[1]  Paul Meakin,et al.  Fractals, scaling, and growth far from equilibrium , 1998 .

[2]  Thijssen Simulations of polycrystalline growth in 2+1 dimensions. , 1995, Physical review. B, Condensed matter.

[3]  M. Plischke,et al.  Solid-on-solid models of molecular-beam epitaxy. , 1994, Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics.

[4]  Greene,et al.  Surface morphology during multilayer epitaxial growth of Ge(001). , 1995, Physical review letters.

[5]  Palasantzas,et al.  Scanning Tunneling Microscopy Study of the Thick Film Limit of Kinetic Roughening. , 1994, Physical review letters.

[6]  D. Cahill,et al.  Surface roughness and pattern formation during homoepitaxial growth of Ge(001) at low temperatures , 1995 .

[7]  Alain Marty,et al.  Instabilities in crystal growth by atomic or molecular beams , 2000 .

[8]  Guo,et al.  Shadowing instability in three dimensions. , 1993, Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics.

[9]  Luis Vázquez,et al.  Submicron structure and acoustic properties of ZnO films deposited on (100) InP by pulsed laser deposition , 2001 .

[10]  A. Barabasi,et al.  Fractal concepts in surface growth , 1995 .

[11]  Leonardo Golubović,et al.  Interfacial Coarsening in Epitaxial Growth Models without Slope Selection , 1997 .

[12]  J. Krug Origins of scale invariance in growth processes , 1997 .

[13]  G. Thornton,et al.  Imaging the polar and non-polar surfaces of ZnO with STM , 1998 .

[14]  N. Combe,et al.  CHANGING THIN-FILM GROWTH BY MODULATING THE INCIDENT FLUX , 1998 .

[15]  Martin Siegert,et al.  COARSENING DYNAMICS OF CRYSTALLINE THIN FILMS , 1998 .

[16]  Masashi Kawasaki,et al.  Room-temperature ultraviolet laser emission from self-assembled ZnO microcrystallite thin films , 1998 .

[17]  T. Tomoyose,et al.  AFM study of surface roughening in sputter-deposited nickel films on ITO glasses , 2000 .

[18]  D. Kohl,et al.  Low temperature sublimation processes from clean cleaved polar surfaces of zinc oxide crystals during first heating , 1974 .

[19]  János Kertész,et al.  Surface disordering : growth, roughening, and phase transitions , 1992 .

[20]  R. Lareau,et al.  High quality crystalline ZnO buffer layers on sapphire (001) by pulsed laser deposition for III–V nitrides , 1997 .

[21]  Ernst,et al.  Observation of a growth instability during low temperature molecular beam epitaxy. , 1994, Physical review letters.

[22]  Chuan Yi Tang,et al.  A 2.|E|-Bit Distributed Algorithm for the Directed Euler Trail Problem , 1993, Inf. Process. Lett..

[23]  G. Hubler,et al.  Pulsed Laser Deposition of Thin Films , 2003, Handbook of Laser Technology and Applications.

[24]  O. Azzaroni,et al.  Validity of the Kardar-Parisi-Zhang equation in the asymptotic limit of metal electrodeposition , 1999 .

[25]  Sander,et al.  Stable and unstable growth in molecular beam epitaxy. , 1994, Physical review letters.

[26]  A. Lita,et al.  Effects of grain growth on dynamic surface scaling during the deposition of Al polycrystalline thin films , 2000 .

[27]  Jeffries,et al.  Instability of Kinetic Roughening in Sputter-Deposition Growth of Pt on Glass. , 1996, Physical review letters.

[28]  Smilauer,et al.  Coarsening and slope evolution during unstable spitaxial growth. , 1995, Physical review. B, Condensed matter.

[29]  H. Koinuma,et al.  Determination of surface polarity of c-axis oriented ZnO films by coaxial impact-collision ion scattering spectroscopy , 1998 .