Near-field scanning optical microscopy of ferroelectric domain walls

We have observed domain walls in ferroelectric LiTaO3 crystals using a polarization and phase sensitive near-field scanning optical microscope. The strain induced birefringence was used to observe the domain walls. The domain walls are measured to be 1 μm wide and show a variation of strain along the domain walls probably due to defects. These measurements allow an estimate of the birefringence at the domain wall of 6×10−5 and associated shear strain of 4×10−5.

[1]  Mool C. Gupta,et al.  Origin of internal field and visualization of 180° domains in congruent LiTaO3 crystals , 1996 .

[2]  Zhigang Suo,et al.  Nonequilibrium thermodynamics of ferroelectric domain evolution , 1996 .

[3]  Mool C. Gupta,et al.  OBSERVATION OF INTERNAL FIELD IN LITAO3 SINGLE CRYSTALS : ITS ORIGIN AND TIME-TEMPERATURE DEPENDENCE , 1996 .

[4]  Susanne Stemmer,et al.  Atomistic structure of 90° domain walls in ferroelectric PbTiO3 thin films , 1995 .

[5]  P. Würfel,et al.  Material characterization with a simple laser scanning microscope. , 1993, Applied optics.

[6]  J. M. Cowley,et al.  Observation of ferroelectric domain boundaries in BaTiO3 by transmission and reflection electron microscopy , 1993 .

[7]  E. Betzig,et al.  Polarization contrast in near-field scanning optical microscopy. , 1992, Applied optics.

[8]  E. Betzig,et al.  Near-Field Optics: Microscopy, Spectroscopy, and Surface Modification Beyond the Diffraction Limit , 1992, Science.

[9]  D. Joy,et al.  Electron holographic study of ferroelectric domain walls , 1992 .

[10]  B. Terris,et al.  Imaging of ferroelectric domain walls by force microscopy , 1990 .

[11]  T. S. Narasimhamurty Photoelastic and Electro-Optic Properties of Crystals , 1981 .

[12]  Daniel Courjon,et al.  Near field optics , 1993 .

[13]  C. Randall,et al.  A transmission electron microscopy investigation of the R3m → R3c phase transition in Pb(Zr,Ti)O3 ceramics , 1993 .

[14]  J. Kobayashi Optical Observation of Domain Motion in Ferroelectric BaTiO3 , 1967 .