The Prediction of Heavy Metal Permeate Flux in Complexation-Microfiltration Process: Polynomial Neural Network Approach

Membrane filtration techniques are distinguished among methods for wastewater treatment and fully correspond to the requirements of the green concept of chemistry and production. The limiting factor for greater application of these methods is the phenomenon of fouling and the decline of the permeate flux. In this study, polynomial neural network based on group method data handling (GMDH) algorithm was applied to predict the performance of the complexation-microfiltration process for the removal of Pb(II), Zn(II), and Cd(II) from synthetic wastewater. The influence of working parameters such as pH, initial concentration of metal ions, type of complexing agent, and pressure on flux was experimentally determined. The data obtained were used as input parameters for the GMDH model as well as for the multiple linear regression (MLR) model. Root mean square error (RMSE), mean absolute error (MAE), and mean absolute percent error (MAPE) were used for evaluation purposes. Results showed that the developed model has excellent performance in flux prediction with R2 of 0.9648.

[1]  Ali Talebi,et al.  Development of a Hybrid Wavelet Packet- Group Method of Data Handling (WPGMDH) Model for Runoff Forecasting , 2016, Water Resources Management.

[2]  Hsiao-Tien Pao,et al.  Forecasting of CO2 emissions, energy consumption and economic growth in China using an improved grey model , 2012 .

[3]  Viktor Pocajt,et al.  A GMDH-type neural network with multi-filter feature selection for the prediction of transition temperatures of bent-core liquid crystals , 2016 .

[4]  D. Antanasijević,et al.  Application of artificial neural networks for estimating Cd, Zn, Pb removal efficiency from wastewater using complexation-microfiltration process , 2017, International Journal of Environmental Science and Technology.

[5]  G. Zeng,et al.  Influence of pH on heavy metal speciation and removal from wastewater using micellar-enhanced ultrafiltration. , 2017, Chemosphere.

[6]  Junghui Chen,et al.  Predicting effect of interparticle interactions on permeate flux decline in CMF of colloidal suspensions: An overlapped type of local neural network , 2008 .

[7]  N. Hankins,et al.  Fouling and cleaning of ultrafiltration membranes: A review , 2014 .

[8]  Mohd Azlan Hussain,et al.  Advanced process control for ultrafiltration membrane water treatment system , 2018 .

[9]  Viktor Pocajt,et al.  A linear and non-linear polynomial neural network modeling of dissolved oxygen content in surface water: Inter- and extrapolation performance with inputs' significance analysis. , 2018, The Science of the total environment.

[10]  Zhan Wang,et al.  Study of dead-end microfiltration features in sequencing batch reactor (SBR) by optimized neural networks , 2011 .

[11]  W. J. Welsh,et al.  Polynomial Neural Network for Linear and Non-linear Model Selection in Quantitative-Structure Activity Relationship Studies on the Internet , 2000, SAR and QSAR in environmental research.

[12]  Durbadal Mandal,et al.  Modeling and optimization of polymer enhanced ultrafiltration using hybrid neural-genetic algorithm based evolutionary approach , 2017, Applied Soft Computing.

[13]  Xiaodong Wang,et al.  Removal of heavy metals from water using polyvinylamine by polymer-enhanced ultrafiltration and flocculation , 2016 .

[14]  Soteris A. Kalogirou,et al.  Artificial intelligence for the modeling and control of combustion processes: a review , 2003 .

[15]  S. Stevanović,et al.  Zinc removal from wastewater by complexation-microfiltration process , 2012 .

[16]  Qi-feng Liu,et al.  Prediction of microfiltration membrane fouling using artificial neural network models , 2009 .

[17]  N. Fatin-Rouge,et al.  Metal removal from aqueous media by polymer-assisted ultrafiltration with chitosan , 2017 .

[18]  A. Malik,et al.  Artificial neural network modeling of the river water quality—A case study , 2009 .

[19]  G. Crini,et al.  Polymer-enhanced ultrafiltration for heavy metal removal: Influence of chitosan and carboxymethyl cellulose on filtration performances , 2018 .

[20]  L. Rink,et al.  The Essential Toxin: Impact of Zinc on Human Health , 2010, International journal of environmental research and public health.

[21]  Fenglian Fu,et al.  Removal of heavy metal ions from wastewaters: a review. , 2011, Journal of environmental management.

[22]  D. Groneberg,et al.  Occupational medicine and toxicology , 2006, Journal of Occupational Medicine and Toxicology (London, England).

[23]  A. Tiwari,et al.  Toxicity of lead: A review with recent updates , 2012, Interdisciplinary toxicology.

[24]  B. Rivas,et al.  Metal ion recovery by polymer-enhanced ultrafiltration using poly(vinyl sulfonic acid): Fouling description and membrane–metal ion interaction , 2009 .

[25]  A. Kim,et al.  Prediction of permeate flux decline in crossflow membrane filtration of colloidal suspension: a radial basis function neural network approach , 2006 .

[26]  D. Groneberg,et al.  Journal of Occupational Medicine and Toxicology the Toxicity of Cadmium and Resulting Hazards for Human Health , 2006 .

[27]  Adewale Giwa,et al.  Experimental investigation and artificial neural networks ANNs modeling of electrically-enhanced membrane bioreactor for wastewater treatment , 2016 .

[28]  Hong-qi Ye,et al.  Application of the hybrid complexation-ultrafiltration process for metal ion removal from aqueous solutions. , 2009, Journal of hazardous materials.

[29]  Fuzhi Li,et al.  Influence of trace cobalt(II) on surfactant fouling of PVDF ultrafiltration membrane , 2017 .

[30]  Yongjun Choi,et al.  Investigation of the filtration characteristics of pilot-scale hollow fiber submerged MF system using cake formation model and artificial neural networks model , 2012 .

[31]  P. Cañizares,et al.  Treatment of copper (II)-loaded aqueous nitrate solutions by polymer enhanced ultrafiltration and electrodeposition , 2010 .

[32]  J. Labanda,et al.  Study of Cr(III) desorption process from a water-soluble polymer by ultrafiltration , 2011 .

[33]  C. Willmott,et al.  A refined index of model performance , 2012 .

[34]  Sung-Kwun Oh,et al.  Polynomial neural networks architecture: analysis and design , 2003, Comput. Electr. Eng..

[35]  P. S. Kumar,et al.  Efficient techniques for the removal of toxic heavy metals from aquatic environment: A review , 2017 .

[36]  H. Tenhu,et al.  Poly(N,N-dimethylaminoethyl methacrylate) for removing chromium (VI) through polymer-enhanced ultrafiltration technique , 2018 .

[37]  Sung-Kwun Oh,et al.  The design of self-organizing Polynomial Neural Networks , 2002, Inf. Sci..

[38]  F. Schmitt,et al.  Development of artificial neural networks to predict membrane fouling in an anoxic-aerobic membrane bioreactor treating domestic wastewater , 2018 .

[39]  S. J. Farlow The GMDH Algorithm of Ivakhnenko , 1981 .

[40]  M. Dhahbi,et al.  Copper and Zinc removal from aqueous solutions by polyacrylic acid assisted-ultrafiltration , 2014 .

[41]  Abdolhamid Salahi,et al.  Experimental investigation, modeling and optimization of membrane separation using artificial neural network and multi-objective optimization using genetic algorithm , 2013 .

[42]  Behrooz Mirza,et al.  Modeling and optimization of cross-flow ultrafiltration using hybrid neural network-genetic algorithm approach , 2014 .

[43]  Xian-she Feng,et al.  Metal sericin complexation and ultrafiltration of heavy metals from aqueous solution , 2014 .

[44]  R. Keiski,et al.  Separation of cadmium and copper from phosphorous rich synthetic waters by micellar-enhanced ultrafiltration , 2011 .

[45]  Wei-hua Wang,et al.  Removal of manganese from waste water by complexation−ultrafiltration using copolymer of maleic acid and acrylic acid , 2014 .

[46]  Jeffrey G. Arnold,et al.  Model Evaluation Guidelines for Systematic Quantification of Accuracy in Watershed Simulations , 2007 .

[47]  Xiaodong Zhang,et al.  Treatment of wastewater containing nickel by complexation- ultrafiltration using sodium polyacrylate and the stability of PAA-Ni complex in the shear field , 2018 .

[48]  M. Barakat,et al.  Polymer-enhanced ultrafiltration process for heavy metals removal from industrial wastewater , 2010 .

[49]  G. Buchner,et al.  Micellar enhanced ultrafiltration (MEUF) of metal cations with oleylethoxycarboxylate , 2015 .

[50]  Ramgopal Uppaluri,et al.  Treatment of oily wastewater using low cost ceramic membrane: Comparative assessment of pore blocking and artificial neural network models , 2010 .

[51]  A. E. Cervera-Padrell,et al.  Modeling of the Flux Decline in a Continuous Ultrafiltration System with Multiblock Partial Least Squares , 2016 .

[52]  Mohd Azlan Hussain,et al.  A practical hybrid modelling approach for the prediction of potential fouling parameters in ultrafiltration membrane water treatment plant , 2017 .

[53]  R. Molinari,et al.  Arsenic removal from water by coupling photocatalysis and complexation-ultrafiltration processes: A preliminary study. , 2017, Water research.

[54]  Oluwaseun O. Ogunbiyi,et al.  Inverted polarity micellar enhanced ultrafiltration for the treatment of heavy metal polluted wastewater , 2005 .

[55]  M. Schwarze Micellar-enhanced ultrafiltration (MEUF) – state of the art , 2017 .

[56]  Alp Yürüm,et al.  High performance ligands for the removal of aqueous boron species by continuous polymer enhanced ultrafiltration , 2013 .

[57]  Yiliang He,et al.  Recovery of nickel from aqueous solutions by complexation-ultrafiltration process with sodium polyacrylate and polyethylenimine. , 2013, Journal of hazardous materials.

[58]  Bashir Rahmanian,et al.  Application of experimental design approach and artificial neural network (ANN) for the determination of potential micellar-enhanced ultrafiltration process. , 2011, Journal of hazardous materials.

[59]  H. Ngo,et al.  A mini-review on membrane fouling. , 2012, Bioresource technology.

[60]  O. Akpor,et al.  Heavy Metal Pollutants in Wastewater Effluents: Sources, Effects and Remediation , 2014 .