Treatment of coal gasification wastewater by a two-continuous UASB system with step-feed for COD and phenols removal.

A two-continuous mesophilic (37 ± 2°C) UASB system with step-feed was investigated as an attractive optimization strategy for enhancing COD and total phenols removal of the system and improving aerobic biodegradability of real coal gasification wastewater. Through the step-feed period, the maximum removal efficiencies of COD and total phenols reached 55-60% and 58-63% respectively in the system, at an influent flow distribution ratio of 0.2 and influent COD concentration of 2500 mg/L; the corresponding efficiencies were at low levels of 45-50% and 43-50% respectively at total HRT of 48 h during the single-feed period. The maximum specific methanogenic activity and substrate utilization rate were 592 ± 16 mg COD-CH(4)/(g VSS d) and 89 ± 12 mg phenol/(g VSS d) during the step-feed operation. After the anaerobic digestion with step-feed, the aerobic effluent COD concentration decreased from 270 ± 9 to 215 ± 10 mg/L. The results suggested that step-feed enhanced the degradation of refractory organics in the second reactor.

[1]  M. Suidan,et al.  Control of anaerobic GAC reactors treating inhibitory wastewaters. , 1990 .

[2]  J. Rodríguez,et al.  Treatment of coke wastewater in a sequential batch reactor (SBR) at pilot plant scale. , 2008, Bioresource technology.

[3]  K. S. Creamer,et al.  Inhibition of anaerobic digestion process: a review. , 2008, Bioresource technology.

[4]  Shunni Zhu,et al.  Treatment of coking wastewater by a UBF-BAF combined process , 2008 .

[5]  M. Suidan,et al.  Anaerobic filters for the treatment of coal gasification wastewater , 1983, Biotechnology and bioengineering.

[6]  Boubaker Fezzani,et al.  Two-phase anaerobic co-digestion of olive mill wastes in semi-continuous digesters at mesophilic temperature. , 2010, Bioresource technology.

[7]  Vasileios Diamantis,et al.  Comparison of single- and two-stage UASB reactors used for anaerobic treatment of synthetic fruit wastewater , 2007 .

[8]  H. Tsuno,et al.  Comparison of thermophilic anaerobic digestion characteristics between single-phase and two-phase systems for kitchen garbage treatment. , 2008, Journal of bioscience and bioengineering.

[9]  A. E. Greenberg,et al.  Standard methods for the examination of water and wastewater : supplement to the sixteenth edition , 1988 .

[10]  J. Bandy,et al.  Hybrid Expanded‐Bed GAC Reactor for Treating Inhibitory Wastewaters , 1990 .

[11]  Su Lin,et al.  Adsorption of phenol and its derivatives from water using synthetic resins and low-cost natural adsorbents: a review. , 2009, Journal of environmental management.

[12]  W. Jianlong,et al.  Bioaugmentation as a tool to enhance the removal of refractory compound in coke plant wastewater , 2002 .

[13]  S. Mudliar,et al.  Heterocyclic nitrogenous pollutants in the environment and their treatment options--an overview. , 2008, Bioresource technology.

[14]  M. Kästner,et al.  Batch methanogenic fermentation experiments of wastewater from a brown coal low-temperature coke plant. , 2010, Journal of environmental sciences.

[15]  Andrzej Kraslawski,et al.  Conceptual design and retrofitting of the coal-gasification wastewater treatment process , 2008 .

[16]  T. Felföldi,et al.  Polyphasic bacterial community analysis of an aerobic activated sludge removing phenols and thiocyanate from coke plant effluent. , 2010, Bioresource technology.

[17]  D. Sales,et al.  Anaerobic thermophilic digestion of cutting oil wastewater: Effect of co-substrate , 2006 .

[18]  G. K. Anderson,et al.  Determination of bicarbonate and total volatile acid concentration in anaerobic digesters using a simple titration , 1992 .

[19]  Anushuya Ramakrishnan,et al.  Effect of effluent recycling and shock loading on the biodegradation of complex phenolic mixture in hybrid UASB reactors. , 2008, Bioresource technology.

[20]  Alfons J. M. Stams,et al.  Enhanced biodegradation of aromatic pollutants in cocultures of anaerobic and aerobic bacterial consortia , 2004, Antonie van Leeuwenhoek.

[21]  Xia Huang,et al.  Fouling characteristics in a membrane bioreactor coupled with anaerobic-anoxic-oxic process for coke wastewater treatment. , 2010, Bioresource technology.

[22]  M. Ahmaruzzaman Adsorption of phenolic compounds on low-cost adsorbents: A review. , 2008, Advances in colloid and interface science.

[23]  D. Lee,et al.  Effect of HRT on the biological pre-denitrification process for the simultaneous removal of toxic pollutants from cokes wastewater. , 2008, Bioresource technology.

[24]  S. Gupta,et al.  Anaerobic biogranulation in a hybrid reactor treating phenolic waste. , 2006, Journal of hazardous materials.

[25]  J. Ni,et al.  Assessing the effectiveness of treating coking effluents using anaerobic and aerobic biofilms , 2008 .

[26]  Wei Wang,et al.  Enhanced anaerobic biodegradability of real coal gasification wastewater with methanol addition. , 2010, Journal of environmental sciences.

[27]  H. Carrère,et al.  PAH fate during the anaerobic digestion of contaminated sludge: Do bioavailability and/or cometabolism limit their biodegradation? , 2010, Water research.

[28]  B. Fernández,et al.  Long-chain fatty acids inhibition and adaptation process in anaerobic thermophilic digestion: batch tests, microbial community structure and mathematical modelling. , 2010, Bioresource technology.

[29]  F. Omil,et al.  Continuous anaerobic treatment of wastewaters containing formaldehyde and urea , 1999 .

[30]  Yun Chen,et al.  Process Development, Simulation, and Industrial Implementation of a New Coal-Gasification Wastewater Treatment Installation for Phenol and Ammonia Removal , 2010 .