Satellite derived trends in NO2 over the major global hotspot regions during the past decade and their inter-comparison.

We assessed satellite derived tropospheric NO(2) distribution on a global scale and identified the major NO(2) hotspot regions. Combined GOME and SCIAMACHY measurements for the period 1996-2006 have been used to compute the trends over these regions. Our analysis shows that tropospheric NO(2) column amounts have increased over the newly and rapidly developing regions like China (11+/-2.6%/year), south Asia (1.76+/-1.1%/year), Middle East (2.3+/-1%/year) and South Africa (2.4+/-2.2%/year). Tropospheric NO(2) column amounts show some decrease over the eastern US (-2+/-1.5%/year) and Europe (0.9+/-2.1%/year). We found that although tropospheric NO(2) column amounts decreased over the major developed regions in the past decade, the present tropospheric NO(2) column amounts over these regions are still significantly higher than those observed over newly and rapidly developing regions (except China). Tropospheric NO(2) column amounts show some decrease over South America and Central Africa, which are major biomass burning regions in the Southern Hemisphere.

[1]  Johannes W. Kaiser,et al.  Comparison of GOME tropospheric NO 2 columns with NO 2 profiles deduced from ground-based in situ measurements , 2006 .

[2]  J. Ziemke,et al.  Dynamical proxies of column ozone with applications to global trend models , 1997 .

[3]  M. Coyle,et al.  The atmospheric budget of oxidized nitrogen and its role in ozone formation and deposition , 1998 .

[4]  H. Akimoto Global Air Quality and Pollution , 2003, Science.

[5]  Bernd Jähne,et al.  Quantitative analysis of NO x emissions from Global Ozone Monitoring Experiment satellite image sequences , 2001 .

[6]  Steffen Beirle,et al.  Weekly cycle of NO 2 by GOME measurements: a signature of anthropogenic sources , 2003 .

[7]  Zhiliang Yao,et al.  NOx emission trends for China, 1995–2004: The view from the ground and the view from space , 2007 .

[8]  Steffen Beirle,et al.  Global distribution pattern of anthropogenic nitrogen oxide emissions: Correlation analysis of satellite measurements and model calculations , 2006 .

[9]  G. Beig,et al.  Detection of surface emission hot spots, trends, and seasonal cycle from satellite-retrieved NO2 over India , 2008 .

[10]  Henk Eskes,et al.  Estimates of lightning NO x production from GOME satellite observations , 2005 .

[11]  R. Martin,et al.  Space‐based constraints on the production of nitric oxide by lightning , 2007 .

[12]  K. Boersma,et al.  Trends, seasonal variability and dominant NOx source derived from a ten year record of NO2 measured from space , 2008 .

[13]  John P. Burrows,et al.  TROPOSPHERIC NO2 FROM GOME MEASUREMENTS , 2002 .

[14]  Ari Laaksonen,et al.  Organic aerosol formation via sulphate cluster activation , 2004 .

[15]  Daniele Bortoli,et al.  First comparison between ground-based and satellite-borne measurements of tropospheric nitrogen dioxide in the Po basin , 2004 .

[16]  Michael Q. Wang,et al.  An inventory of gaseous and primary aerosol emissions in Asia in the year 2000 , 2003 .

[17]  Henk Eskes,et al.  Intercomparison of SCIAMACHY nitrogen dioxide observations, in situ measurements and air quality modeling results over Western Europe , 2007 .

[18]  Aaron L. Swanson,et al.  Effects of changing power plant NOx emissions on ozone in the eastern United States: Proof of concept , 2006 .

[19]  John P. Burrows,et al.  Satellite‐observed U.S. power plant NOx emission reductions and their impact on air quality , 2006 .

[20]  Kelly Chance,et al.  Global partitioning of NOx sources using satellite observations: relative roles of fossil fuel combustion, biomass burning and soil emissions. , 2005, Faraday discussions.

[21]  Amit Garg,et al.  Large point source (LPS) emissions from India: regional and sectoral analysis , 2002 .

[22]  R. Martin,et al.  Interannual and seasonal variability of biomass burning emissions constrained by satellite observations , 2003 .

[23]  Michael H. Kutner Applied Linear Statistical Models , 1974 .

[24]  R. Martin,et al.  Global and regional decreases in tropospheric oxidants from photochemical effects of aerosols , 2003 .

[25]  J. Burrows,et al.  Increase in tropospheric nitrogen dioxide over China observed from space , 2005, Nature.

[26]  Henk Eskes,et al.  Error analysis for tropospheric NO2 retrieval from space , 2004 .

[27]  Sanford Sillman,et al.  The sensitivity of ozone to nitrogen oxides and hydrocarbons in regional ozone episodes , 1990 .

[28]  Henk Eskes,et al.  Detection of the trend and seasonal variation in tropospheric NO2 over China , 2006 .

[29]  Bernd Jähne,et al.  Quantitative analysis of NOx emissions from GOME-satellite image sequences , 2001 .

[30]  F. Achard,et al.  Determination of Deforestation Rates of the World's Humid Tropical Forests , 2002, Science.