Resonant femtosecond laser pulse dynamics in metal nanorod-based hyperbolic metamaterials in epsilon-near-zero regime

Wealth of fascinating phenomena provided by artificial photonic structures sparks extensive research efforts in the studies of metamaterials, a special and perspective class of them being the hyperbolic metamaterials (HMMs). Strong HMMs optical anisotropy attained by the combination of metal and dielectric constituents underpins unusual hyperbolic dispersion of light in these artificial media, which marvels plethora of far-reaching applications in photonics. However the dynamics of ultrashort optical pulses in HMMs remains almost unexplored. In this work we experimentally investigate the interaction of femtosecond laser pulses with metal-nanorod based HMMs exhibiting the epsilon-near-zero (ENZ) spectral point, when extraordinary dielectric permittivity goes to zero yielding transition between topologically distinct elliptic and hyperbolic light HMM dispersion. We demonstrate a pronounced superluminal and slow propagation of laser pulses in the HMM, with the transition between these regimes and resonant character of these phenomena in the spectral vicinity of the ENZ point. We put forward a theoretical model of the superluminality and slow light, which leverages unusual case of laser pulse with spectral components in elliptic and hyperbolic dispersion at once. We believe our findings bring to life superior applications for future linear and nonlinear ultrafast photonics of HMMs harnessing of revealed exotic dynamics of optical field in these media.

[1]  F. R. Faxvog,et al.  MEASURED PULSE VELOCITY GREATER THAN c IN A NEON ABSORPTION CELL , 1970 .

[2]  L. J. Wang,et al.  Transparent anomalous dispersion and superluminal light-pulse propagation at a negative group velocity , 2001 .

[3]  Zhaowei Liu,et al.  Far-Field Optical Hyperlens Magnifying Sub-Diffraction-Limited Objects , 2007, Science.

[4]  Robert W. Boyd,et al.  Superluminal and Slow Light Propagation in a Room-Temperature Solid , 2003, Science.

[5]  L. J. Wang,et al.  Gain-assisted superluminal light propagation , 2000, Nature.

[6]  David R. Smith,et al.  Partial focusing of radiation by a slab of indefinite media , 2004 .

[7]  Frank H. L. Koppens,et al.  Direct observation of ultraslow hyperbolic polariton propagation with negative phase velocity , 2015, Nature Photonics.

[8]  P. Kelly,et al.  Adaptive pre-shaping for ultrashort pulse control during propagation in AZO/ZnO multilayered metamaterial at the epsilon-near-zero spectral point , 2020 .

[9]  G. Wurtz,et al.  Superluminal and stopped light due to mode coupling in confined hyperbolic metamaterial waveguides , 2015, Scientific Reports.

[10]  G. Wurtz,et al.  Anisotropic optical properties of arrays of gold nanorods embedded in alumina , 2006 .

[11]  Robert W Boyd,et al.  Observation of Backward Pulse Propagation Through a Medium with a Negative Group Velocity , 2006, Science.

[12]  P. Kelly,et al.  Pulse shaping in the presence of enormous second-order dispersion in Al:ZnO/ZnO epsilon-near-zero metamaterial , 2018 .

[13]  I. Kolmychek,et al.  Second-harmonic generation spectroscopy in gold nanorod-based epsilon-near-zero metamaterials. , 2020, Optics letters.

[14]  I. Kolmychek,et al.  Phase-matched optical second harmonic generation in a hyperbolic metamaterial based on silver nanorods , 2020 .

[15]  P. Kelly,et al.  Pump-probe ultrashort pulse modulation in an AZO/ZnO metamaterial at the epsilon near zero spectral point , 2020 .

[16]  Jean-Luc Brédas,et al.  The speed of information in a ‘ fast-light ’ optical medium , 2022 .

[17]  M. A. Vincenti,et al.  Singularity-driven second- and third-harmonic generation at -near-zero crossing points , 2011 .

[18]  Zubin Jacob,et al.  Broadband super-planckian thermal emission from hyperbolic metamaterials , 2013, CLEO: 2013.

[19]  Steven Chu,et al.  Linear Pulse Propagation in an Absorbing Medium , 1982 .

[20]  Igor Krois,et al.  Ultra-broadband simultaneous superluminal phase and group velocities in non-Foster epsilon-near-zero metamaterial , 2013 .

[21]  Michael Scalora,et al.  Second-harmonic generation in longitudinal epsilon-near-zero materials , 2017 .

[22]  Leonid Alekseyev,et al.  Supplementary Information for “ Negative refraction in semiconductor metamaterials ” , 2007 .

[23]  M. Wegener,et al.  Simultaneous Negative Phase and Group Velocity of Light in a Metamaterial , 2006, Science.

[24]  B. Segard,et al.  Observation of negative velocity pulse propagation , 1985 .

[25]  Wayne Dickson,et al.  Eliminating material constraints for nonlinearity with plasmonic metamaterials , 2015, Nature Communications.

[26]  A. Cimmino,et al.  Negative group velocity of a light pulse in cesium vapour , 2002 .