In searching for solvents that are able to absorb sulfur dioxide and nitric oxide, solvents triethylenetetramine, diethylenetriamine, N-cyclohexyl-2-pyrrolidone and N, N, N', N'-tetraethylethylenediamine have all been tested. It was found that triethylenetetramine and N, N, N', N'-tetraethylethylenediamine absorb nitric oxide, while this gas is not absorbed by N-cyclohexyl-2-pyrrolidone and diethylenetriamine. Sulfur dioxide, besides being absorbed by triethylenetetramine, is also absorbed by diethylenetriamine and N-cyclohexyl-2-pyrrolidone.
The Henry's law constants and activity coefficients at infinite dilution of the gases in the absorbing solvents were determined by gas-liquid chromatography.
La recherche de solvants capables d'absorber l'anhydride sulfureux et l'oxyde nitrique, nous a amene a tester les solvants triethylenetetramine, diethylenetriamine, N-cyclohexyl-2-pyrrolidone et N, N, N', N'-tetraethylethylenediamine. On a trouve que la triethylenetetramine et la N, N, N', N'-tetraethylehylenediamine absorbent l'oxyde nitrique qui n'est par ailleurs pas absorbe par la N-cyclohexyl-2-pyrrolidone ni la diethylenetriamine. L'anhydride sulfureux, en plus d'etre absorbe par la triethylenetetramine, est egalement absorbe par la diethylenetriamine et la N-cyclohexyl-2-pyrrolidone.
Les constantes de la loi de Henry et les coefficients d'activite a dilution infinie des gaz dans les solvants utilisables, ont ete determinees par chromatographic gaz-liquide.
[1]
G. Klinzing,et al.
Solubility of SO2 in 1-methyl-2-pyrrolidinone and tri-n-butyl phosphate
,
1984
.
[2]
G. Klinzing,et al.
Absorption of nitrogen dioxide and sulfur dioxide in methanol
,
1984
.
[3]
Ichibei Kudo,et al.
Individual and Simultaneous Absorption of Dilute NO and SO2 in Aqueous Slurries of MgSO3 with FeII-EDTA
,
1980
.
[4]
C. Hussey,et al.
Specific retention volumes and limiting activity coefficients of C4-C8 alkane solutes in C22-C36 n-alkane solvents
,
1975
.
[5]
J. Janák,et al.
A study on the reliability of the excess enthalpies calculated from gas-liquid chromatographic retention data
,
1972
.
[6]
H. G. Harris,et al.
Henry's constants for methane, ethane, ethylene, propane, and propylene in octadecane, eicosane, and docosane
,
1969
.
[7]
D. Ambrose,et al.
Presentation of Gas-Liquid Chromatographic Retention Data
,
1958
.