Emission inventories of primary particles and pollutant gases for China

Detailed high-resolution emission inventories of primary particles (PM2.5, BC and OC) and pollutant gases (SO2, NOx, NH3, CO and VOCs) for China in 2007 were constructed on the basis of the latest fuel consumption data, mostly at the county level, and from socio-economic statistics and data on fossil and biomass fuels obtained from government agencies. New emission factors reflecting local features were also used. The calculated emissions were 13.212 Mt PM2.5, 1.4 Mt BC, 2.946 Mt OC, 31.584 Mt SO2, 23.248 Mt NOx, 16.017 Mt NH3, 164.856 Mt CO and 35.464 Mt VOCs. The national and regional emissions were gridded with 0.5° × 0.5° resolution for use in air quality models. Larger emissions were found in eastern and central China than in western China. The emissions estimated here are roughly equal to those obtained in previous studies, but with different contributions from because of seasonal changes in residential heating and biomass combustion. Finally, uncertainties in inventories were analyzed.

[1]  David G. Streets,et al.  Anthropogenic emissions of non-methane volatile organic compounds in China , 2002 .

[2]  K. Lam,et al.  A modeling study on acid rain and recommended emission control strategies in China , 2000 .

[3]  Tami C. Bond,et al.  On the future of carbonaceous aerosol emissions , 2004 .

[4]  Yongliang Ma,et al.  Greenhouse Gases and other Airborne Pollutants from Household Stoves in China: a Database for Emission Factors , 2000 .

[5]  David G. Streets,et al.  Sulfur dioxide emissions and sectorial contributions to sulfur deposition in Asia , 1997 .

[6]  D. Ward,et al.  Fuel biomass and combustion factors associated with fires in savanna ecosystems of South Africa and Zambia , 1996 .

[7]  Tian Xiao,et al.  Direct Carbon Emissions from Chinese Forest Fires, 1991～2000 , 2003 .

[8]  J. Hao,et al.  [VOC emission situation and control measures of gas station in China]. , 2006, Huan jing ke xue= Huanjing kexue.

[9]  M. Jacobson,et al.  Strong radiative heating due to the mixing state of black carbon in atmospheric aerosols , 2022 .

[10]  D. Streets,et al.  A technology‐based global inventory of black and organic carbon emissions from combustion , 2004 .

[11]  Yanli Feng,et al.  Emission factors for carbonaceous particles and polycyclic aromatic hydrocarbons from residential coal combustion in China. , 2005, Environmental science & technology.

[12]  Zhang Xiao-ye.  Aerosol over China and Their Climate Effect , 2007 .

[13]  G. Cao,et al.  Inventory of black carbon and organic carbon emissions from China , 2006 .

[14]  M. Jacobson.  Control of fossil‐fuel particulate black carbon and organic matter, possibly the most effective method of slowing global warming , 2002 .

[15]  Michael Q. Wang,et al.  Black carbon emissions in China , 2001 .

[16]  J. Hansen,et al.  Climate Effects of Black Carbon Aerosols in China and India , 2002, Science.

[17]  Zhu Song-li.  Study on emission factors of GHG and pollutants from rural stoves in developing countries , 2004 .

[18]  Xiaobin Xu,et al.  Characteristics of gaseous pollutants at Gucheng, a rural site southwest of Beijing , 2009 .

[19]  C. Venkataraman,et al.  Inventory of aerosol and sulphur dioxide emissions from India: I—Fossil fuel combustion , 2002 .

[20]  E. Larson,et al.  A high-resolution emission inventory for eastern China in 2000 and three scenarios for 2020 , 2005 .

[21]  David G. Streets,et al.  Present and future emissions of air pollutants in China:: SO2, NOx, and CO , 2000 .

[22]  M. Andreae,et al.  Emission of trace gases and aerosols from biomass burning , 2001 .

[23]  W. Jo,et al.  Analysis of Operation Parameters of Pilot-Scale Packed-Absorption System for Airborne Methyl Ethyl Ketone Control , 2011 .

[24]  G. Carmichael,et al.  Asian emissions in 2006 for the NASA INTEX-B mission , 2009 .

[25]  C. Liousse,et al.  Construction of a 1° × 1° fossil fuel emission data set for carbonaceous aerosol and implementation and radiative impact in the ECHAM4 model , 1999 .

[26]  David G. Streets,et al.  Anthropogenic NOx emissions in Asia in the period 1990–2020 , 1999 .

[27]  J. Hao,et al.  Inventories and distribution characteristics of NOx emissions in China , 2001 .

[28]  Zhang Xiaoye,et al.  Estimating the Quantity of Crop Residues Burnt in Open Field in China , 2006 .

[29]  Zhao Dianwu,et al.  ESTIMATION OF ANTHROPOGENIC AMMONIA EMISSIONS IN ASIA , 1994 .

[30]  Guoliang Cao,et al.  Investigation on emission factors of particulate matter and gaseous pollutants from crop residue burning. , 2008, Journal of environmental sciences.

[31]  Kenji Satake,et al.  The 1964 Prince William Sound earthquake: Joint inversion of tsunami and geodetic data , 1996 .

[32]  Li Wei,et al.  Emission Inventory of 10 Kinds of Air Pollutants for Road Traffic Vehicles in China , 2003 .

[33]  David G. Streets,et al.  Sulfur dioxide emissions in Asia in the period 1985–1997 , 2000 .

[34]  H. Akimoto,et al.  An Asian emission inventory of anthropogenic emission sources for the period 1980-2020 , 2007 .

[35]  Trend of acid rain and neutralization by yellow sand in east Asia—a numerical study , 2002 .

[36]  Xiaoye Zhang,et al.  Carbonaceous aerosol composition over various regions of China during 2006 , 2008 .

[37]  J. Penner,et al.  A global three‐dimensional model study of carbonaceous aerosols , 1996 .

[38]  A. Bouwman,et al.  A global high‐resolution emission inventory for ammonia , 1997 .

[39]  David G. Streets,et al.  Sulfur dioxide emissions in China and sulfur trends in East Asia since 2000 , 2010 .

[40]  Yutaka Tonooka,et al.  NMVOCs and CO Emission Inventory in East Asia , 2001 .

[41]  Z. Klimont,et al.  Emission and speciation of non-methane volatile organic compounds from anthropogenic sources in China , 2008 .

[42]  Zhong Liu-ju,et al.  Quantitative Uncertainty Analysis in Air Pollutant Emission Inventories: Methodology and Case Study , 2007 .

[43]  S. A. Whalen,et al.  Elemental characterization of particulate matter emitted from biomass burning: Wind tunnel derived source profiles for herbaceous and wood fuels , 1997 .

[44]  Du Qing.  The Study of Vehicle Emission Properties on Real-Road Condition and the Influence of Some Important Factors , 2002 .

[45]  D. Streets,et al.  An Evaluation of TRACE-P Emission Inventories From China Using a Regional Model and Chemical Measurements At a Rural Site in China , 2004 .

[46]  Michael Q. Wang,et al.  An inventory of gaseous and primary aerosol emissions in Asia in the year 2000 , 2003 .

[47]  中華人民共和国国家統計局.  China statistical yearbook , 1988 .

[48]  Young-Joon Kim,et al.  An overview of ACE‐Asia: Strategies for quantifying the relationships between Asian aerosols and their climatic impacts , 2003 .

[49]  P. Purohit,et al.  Projections of SO2, NOx and carbonaceous aerosols emissions in Asia , 2009 .

[50]  Nobuo Kato,et al.  Anthropogenic emissions of SO2 and NOx in Asia : emission inventories , 1992 .