Concentration fluctuation measurements in tracer plumes using high and low frequency response detectors

A set of tracer experiments designed to compare two concentration fluctuation detectors and measure fluctuation statistics at high frequencies is described. A detector which has been used in several previous fluctuation experiments (the TIP photoionisation detector manufactured by Photovac of Canada) is compared with another with a much higher frequency response (the flame ionisation detector — FID — made by Cambustion of the UK). Good agreement is found and results show that the signal optimization system used in previous work with the TIP provides an accurate enhancement of the instrument output, thus improving confidence in the results of previous papers. They also confirm that the TIP detector is able to resolve most of the concentration variance in most situations of interest, but not at very short range. Measurements of the high frequency end of the fluctuation spectrum using the FID show inertial-convective subrange behaviour at frequencies not resolved by the TIP, supporting earlier work. Fluctuation spectra measured very close to the source are also shown to have a characteristic +2/3 power law behaviour (when nSc (n) is plotted against n) at lower frequencies, in agreement with theoretical predictions.

[1]  C. Jones On the structure of instantaneous plumes in the atmosphere , 1983 .

[2]  Eugene Yee,et al.  The shape of the probability density function of short-term concentration fluctuations of plumes in the atmospheric boundary layer , 1990 .

[3]  Richard J. Perkins,et al.  Plume dispersion through large groups of obstacles – a field investigation , 1995 .

[4]  M. Davidson,et al.  Concentration Fluctuation Experiments in Stable Conditions and in a Pseudo-Urban Environment , 1992 .

[5]  D. Thomson The second-order moment structure of dispersing plumes and puffs , 1996, Journal of Fluid Mechanics.

[6]  Steven R. Hanna The exponential probability density function and concentration fluctuations in smoke plumes , 1984 .

[7]  B. Lamb,et al.  A Fast Response Continuous Analyzer for Halogenated Atmospheric Tracers , 1985 .

[8]  K. Mylne The PDF of concentration fluctuations — Comments on YEE (1990) and YEE (1991) , 1992 .

[9]  K. Mylne,et al.  Concentration fluctuation measurements in a plume dispersing in a stable surface layer , 1992 .

[10]  Eugene Yee,et al.  Concentration fluctuation measurements in clouds released from a quasi-instantaneous point source in the atmospheric surface layer , 1994 .

[11]  A wind tunnel study of mean and fluctuating concentrations in a plume dispersing over a two-dimensional hill , 1993 .

[12]  P. J. Mason,et al.  Concentration fluctuation measurements in a dispersing plume at a range of up to 1000 m , 1991 .

[13]  J. Fackrell,et al.  A flame ionisation detector for measuring fluctuating concentration , 1980 .

[14]  E. Yee Reply to the ‘comments on: The PDF of concentration fluctuations’ by Kenneth R. Mylne , 1992 .

[15]  D. J. Hall,et al.  Avoiding aerosol sampling problems in fast response flame ionisation detectors , 1991 .

[16]  P. C. Chatwin,et al.  The treatment of atmospheric dispersion data in the presence of noise and baseline drift , 1995 .

[17]  M. Kleiman,et al.  Characterization of concentration fluctuations of a surface plume in a neutral boundary layer , 1988 .

[18]  B. Sawford Conditional concentration statistics for surface plumes in the atmospheric boundary layer , 1987 .

[19]  Eugene Yee,et al.  Experimental Measurements of Concentration Fluctuations and Scales in a Dispersing Plume in the Atmospheric Surface Layer Obtained Using a Very Fast Response Concentration Detector , 1994 .

[20]  Eugene Yee,et al.  Statistical characteristics of concentration fluctuations in dispersing plumes in the atmospheric surface layer , 1993 .

[21]  B. Sawford,et al.  Atmospheric boundary-layer measurements of concentration statistics from isolated and multiple sources , 1985 .

[22]  K. Mylne,et al.  The vertical profile of concentration fluctuations in near-surface plumes , 1993 .

[23]  A. Robins,et al.  Concentration fluctuations and fluxes in plumes from point sources in a turbulent boundary layer , 1982, Journal of Fluid Mechanics.

[24]  Application of nonlinear dynamical systems analysis to conditionally sampled concentration fluctuations of a passive scalar in the atmospheric boundary layer , 1991 .

[25]  David J. Thomson,et al.  A stochastic model for the motion of particle pairs in isotropic high-Reynolds-number turbulence, and its application to the problem of concentration variance , 1990, Journal of Fluid Mechanics.

[26]  Recurrence statistics of concentration fluctuations in plumes within a near-neutral atmospheric surface layer , 1993 .