论文信息 - CO 2 Capture and Storage

CO 2 Capture and Storage

The CO 2 concentration in the atmosphere has increased due to the combustion of fossil fuels and this is causing concerns of global warming. At present there is no cost effective CO 2 control and capture technologies available at scale for coal-fired plants. The US Department of Energy (DOE) National Energy Technology Laboratory (NETL) has initiated a research and development program to develop advanced CO 2 capture and compression technologies for both existing and new coal-fired power plants. The goal is to achieve 90% CO 2 capture at less than 35% increase in cost of electricity (CCE) at a commercial scale by the year 2020. The time line for developing a system for Carbon Capture and Storage (CCS) is shown in figure. This chapter outlines an overview of the technologies being investigated for CO 2 capture and sequestration in anticipation of future CO 2 emissions legislations. The different elements in developing a CCS is explained with block diagrams throughout the chapter. The success of CCS depends on the ability to measure the amount of CO 2 at a particular site, to confirm the stored CO 2 is not harming the eco-system and the ability to mitigate any impact associated with CO 2 leakage. References for further reading are given.

Bruce G. Miller

[1] Bruce G. Miller,et al. Adsorption separation of carbon dioxide from flue gas of natural gas-fired boiler by a novel nanoporous “molecular basket” adsorbent , 2005 .

[2] A. Scaroni,et al. Influence of Moisture on CO2 Separation from Gas Mixture by a Nanoporous Adsorbent Based on Polyethylenimine-Modified Molecular Sieve MCM-41 , 2005 .

[3] Xiaoliang Ma,et al. "Molecular basket" sorbents for separation of CO(2) and H(2)S from various gas streams. , 2009, Journal of the American Chemical Society.

[4] A L Robinson,et al. Assessment of potential carbon dioxide reductions due to biomass-coal cofiring in the United States. , 2003, Environmental science & technology.

[5] Timothy E. Fout,et al. Advances in CO2 capture technology—The U.S. Department of Energy's Carbon Sequestration Program ☆ , 2008 .

[6] J. Andresen,et al. Preparation and characterization of novel CO2 “molecular basket” adsorbents based on polymer-modified mesoporous molecular sieve MCM-41 , 2003 .

[7] M. Mann,et al. A life cycle assessment of biomass cofiring in a coal-fired power plant , 2001 .

[8] Bruce G. Miller,et al. Novel Polyethylenimine-Modified Mesoporous Molecular Sieve of MCM-41 Type as High-Capacity Adsorbent for CO2 Capture , 2002 .