Identification of storage years of black tea using near-infrared hyperspectral imaging with deep learning methods

Abstract Black tea stored for years might be adulterated as fresh tea for sell. Near-infrared hyperspectral imaging coupled with machine learning methods was applied for rapid detection of black tea storage years. Black tea samples produced in the years of 2016, 2017, 2018 and 2019 (storage for 3, 2, 1 and 0 years) were studied. Principal component analysis (PCA) was used to form score images to qualitatively visualize the differences of tea samples stored for different years. Loadings of each principal component were used to identify optimal wavelengths. Based on the full range spectra and the optimal wavelengths, conventional machine learning methods (logistic regression (LR), support vector machine (SVM)) and deep learning methods (convolutional neural network (CNN), long short-term memory (LSTM) and CNN-LSTM) were used to establish classification models. Classification models using full spectra and optimal wavelengths obtained close results. Deep learning methods obtain better results. Black tea samples stored for 1 and 2 years were more likely to be misclassified. Fresh tea samples can be well identified from the stored samples. The overall results illustrated the feasibility to identify the storage year of black tea with machine learning methods, proving an efficient alternative for black tea quality inspection.

[1]  Ioannis E. Livieris,et al.  A CNN–LSTM model for gold price time-series forecasting , 2020, Neural Computing and Applications.

[2]  J. Rufián‐Henares,et al.  Antioxidant capacity, total phenols and color profile during the storage of selected plants used for infusion. , 2016, Food chemistry.

[3]  Dong Liang,et al.  Nondestructive detection of storage time of strawberries using visible/near-infrared hyperspectral imaging , 2020 .

[4]  Young-Boong Kim,et al.  Changes in major polyphenolic compounds of tea (Camellia sinensis) leaves during the production of black tea , 2016, Food Science and Biotechnology.

[5]  Chu Zhang,et al.  Identification of coffee bean varieties using hyperspectral imaging: influence of preprocessing methods and pixel-wise spectra analysis , 2018, Scientific Reports.

[6]  Chen Yuanyuan,et al.  Quantitative analysis modeling of infrared spectroscopy based on ensemble convolutional neural networks , 2018, Chemometrics and Intelligent Laboratory Systems.

[7]  Yun Yang,et al.  Improved Deep Hybrid Networks for Urban Traffic Flow Prediction Using Trajectory Data , 2018, IEEE Access.

[8]  Asifullah Khan,et al.  A survey of the recent architectures of deep convolutional neural networks , 2019, Artificial Intelligence Review.

[9]  Tian Ding,et al.  Identification of bitter compounds from dried fruit of Ziziphus jujuba cv. Junzao , 2017 .

[10]  Ba Tuan Le,et al.  Coal analysis based on visible-infrared spectroscopy and a deep neural network , 2018, Infrared Physics & Technology.

[11]  Antonietta Baiano,et al.  Applications of hyperspectral imaging for quality assessment of liquid based and semi-liquid food products: A review , 2017 .

[12]  Yong He,et al.  Rapid and Nondestructive Discrimination of Geographical Origins of Longjing Tea using Hyperspectral Imaging at Two Spectral Ranges Coupled with Machine Learning Methods , 2020, Applied Sciences.

[13]  Jingming Ning,et al.  Hyperspectral imaging for discrimination of Keemun black tea quality categories: Multivariate calibration analysis and data fusion , 2020 .

[14]  J. Stoltzfus,et al.  Logistic regression: a brief primer. , 2011, Academic emergency medicine : official journal of the Society for Academic Emergency Medicine.

[15]  Lei Yu,et al.  A 6-DOFs event-based camera relocalization system by CNN-LSTM and image denoising , 2021, Expert Syst. Appl..

[16]  Li Zhengquan,et al.  Effect of 1–20 years storage on volatiles and aroma of Keemun congou black tea by solvent extraction-solid phase extraction-gas chromatography-mass spectrometry , 2021 .

[17]  C. Sengupta,et al.  Temporal depletion of packaged tea antioxidant quality under commercial storage condition , 2020, Journal of Food Science and Technology.

[18]  A. Gowen,et al.  Use of hyperspectral imaging for evaluation of the shelf-life of fresh white button mushrooms (Agaricus bisporus) stored in different packaging films , 2010 .

[19]  Zheng-Zhu Zhang,et al.  Rapid detection of quality index of postharvest fresh tea leaves using hyperspectral imaging. , 2020, Journal of the science of food and agriculture.

[20]  Thomas Arnold,et al.  Hyperspectral imaging: a novel approach for plant root phenotyping , 2018, Plant Methods.

[21]  Baohua Yang,et al.  A Model for Yellow Tea Polyphenols Content Estimation Based on Multi-Feature Fusion , 2019, IEEE Access.

[22]  Jingming Ning,et al.  Classification of five Chinese tea categories with different fermentation degrees using visible and near-infrared hyperspectral imaging , 2016 .

[23]  Martin Pelikan,et al.  Hierarchical Bayesian optimization algorithm: toward a new generation of evolutionary algorithms , 2010, SICE 2003 Annual Conference (IEEE Cat. No.03TH8734).

[24]  Han Cao,et al.  Prediction for Tourism Flow based on LSTM Neural Network , 2017, IIKI.

[25]  Bolin Shi,et al.  Study of wavelet denoising in apple's charge-coupled device near-infrared spectroscopy. , 2007, Journal of agricultural and food chemistry.

[26]  Yuzhen Lu,et al.  Hyperspectral imaging technology for quality and safety evaluation of horticultural products: A review and celebration of the past 20-year progress , 2020 .

[27]  Wang Jing,et al.  Differentiation of storage time of wheat seed based on near infrared hyperspectral imaging , 2017 .

[28]  A. Sharangi Medicinal and therapeutic potentialities of tea (Camellia sinensis L.) - a review. , 2009 .

[29]  Dong Yang,et al.  Combination of spectral and textural information of hyperspectral imaging for the prediction of the moisture content and storage time of cooked beef , 2017 .

[30]  R. Senthilkumar,et al.  Induction of γ irradiation for decontamination and to increase the storage stability of black teas , 2008 .

[31]  Chu Zhang,et al.  Non-Destructive and Rapid Variety Discrimination and Visualization of Single Grape Seed Using Near-Infrared Hyperspectral Imaging Technique and Multivariate Analysis , 2018, Molecules.

[32]  Christopher J. C. Burges,et al.  A Tutorial on Support Vector Machines for Pattern Recognition , 1998, Data Mining and Knowledge Discovery.

[33]  Stephen Marshall,et al.  Near-infrared hyperspectral imaging for non-destructive classification of commercial tea products , 2018, Journal of Food Engineering.

[34]  Jingming Ning,et al.  Using near-infrared hyperspectral imaging with multiple decision tree methods to delineate black tea quality. , 2020, Spectrochimica acta. Part A, Molecular and biomolecular spectroscopy.