Parity Broken Chiral Spin Dynamics in Ba 3 NbFe 3 Si 2 O 14

The spin wave excitations emerging from the chiral helically modulated 120 ◦ magnetic order in a langasite Ba 3 NbFe 3 Si 2 O 14 enantiopure crystal were investigated by unpolarized and polarized inelastic neutron scattering. A dynamical fingerprint of the chiral ground state is obtained, sin-gularized by (i) spectral weight asymmetries answerable to the structural chirality and (ii) a full chirality of the spin correlations observed over the whole energy spectrum. The intrinsic chiral nature of the spin waves elementary excitations is shown in absence of macroscopic time reversal symmetry breaking.

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