Abstract Neutron resonance absorption spectroscopy (N-RAS) using a pulsed neutron source can be applied to time-of-flight (TOF) radiography, and the obtained parameters from the peak shape analysis can be reconstructed as the tomograms of nuclide distributions using computed tomography (CT). The problem is that the available spatial resolution is not sufficient for radiography imaging. In this study, we combined neutron and X-ray radiographies to improve the quantitative reconstruction of the neutron tomogram. The accelerator-based neutron source emits X-rays (or gamma-rays) at the same time the neutron pulse is emitted. We utilized the X-ray beam from the neutron source to obtain X-ray radiogram on the same beam line with neutron radiography and then reconstructed the neutron tomogram quantitatively with the help of a detailed sample internal structure obtained from the X-ray radiogram. We calculated the nuclide number density distribution tomogram using a statistical reconstruction procedure, which was easy to include in the structure model during the reconstruction. The obtained result of nuclide number density distribution showed good coincidence with the original object number density.
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