Optimization of plasmon nano-focusing in tapered metal rods

Analysis of adiabatic and non-adiabatic nano-focusing in tapered metal nano- rods leads to the determination of optimal taper angles and rod lengths as functions of material parameters (for gold, silver, and aluminum) at frequencies from the optical and near infra-red ranges. The considered nano-focusing structures appear to be highly toler- ant to such structural and fabrication imperfections as variations of length of the rod and taper angle around their optimal values. However, the major parameter that tends to sig- nificantly affect the nano-focusing capabilities of the rods is the radius of the tip, and this is the parameter that should be carefully reproduced in the experiments. Comparison of the numerical results with the adiabatic theory of nano-focusing for different metals and different wavelengths demonstrates the validity of the adiabatic theory in a much wider range of taper angles (up to tens of degrees) than it was previously expected. Major pre- dicted local field enhancements of up to ~ 2,500 times in the considered structures within nano-scale regions as small as a few nanometers will make tapered metal rods highly promising for single molecule detection and development of a new generation of sensors, measurement and nano-manipulation techniques.

[1]  M. Stockman,et al.  Nanofocusing of optical energy in tapered plasmonic waveguides. , 2004, Physical review letters.

[2]  David J. Bergman,et al.  Enhanced second harmonic generation in a self-similar chain of metal nanospheres , 2005 .

[3]  Dmitri K. Gramotnev,et al.  Adiabatic nanofocusing of plasmons by a sharp metal wedge on a dielectric substrate , 2007 .

[4]  A. Kisliuk,et al.  Optical properties and enhancement factors of the tips for apertureless near-field optics , 2006 .

[5]  Lukas Novotny,et al.  Light confinement in scanning near-field optical microscopy , 1995 .

[6]  Reinhard Guckenberger,et al.  Fluorescence near metal tips: The roles of energy transfer and surface plasmon polaritons. , 2007, Optics express.

[7]  W. Denk,et al.  Optical stethoscopy: Image recording with resolution λ/20 , 1984 .

[8]  Kh. V. Nerkararyan,et al.  Superfocusing of surface polaritons in the conical structure , 2000 .

[9]  Mark I. Stockman,et al.  Optimized nonadiabatic nanofocusing of plasmons by tapered metal rods , 2008 .

[10]  Novotny,et al.  Light propagation in a cylindrical waveguide with a complex, metallic, dielectric function. , 1994, Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics.

[11]  Nader A. Issa,et al.  Optical Nanofocusing on Tapered Metallic Waveguides , 2007 .

[12]  Dmitri K. Gramotnev,et al.  Adiabatic and nonadiabatic nanofocusing of plasmons by tapered gap plasmon waveguides , 2006 .

[13]  Maxim Durach,et al.  Toward full spatiotemporal control on the nanoscale. , 2007, Nano letters.

[14]  Neil A. Anderson,et al.  Institute of Physics Publishing Journal of Optics A: Pure and Applied Optics Optimal Configurations for Imaging Polarimeters: Impact of Image Noise and Systematic Errors , 2006 .

[15]  E. Palik Handbook of Optical Constants of Solids , 1997 .

[16]  A. Bouhelier,et al.  Plasmon‐coupled tip‐enhanced near‐field optical microscopy , 2003, Journal of microscopy.

[17]  T. Elsaesser,et al.  Grating-coupling of surface plasmons onto metallic tips: a nanoconfined light source. , 2007, Nano letters.

[18]  D. Bergman,et al.  Self-similar chain of metal nanospheres as efficient nanolens , 2003, InternationalQuantum Electronics Conference, 2004. (IQEC)..

[19]  E. Janunts,et al.  Excitation and propagation of surface plasmon polaritons on the gold covered conical tip , 2006 .

[20]  Dmitri K. Gramotnev,et al.  Adiabatic nano-focusing of plasmons by sharp metallic wedges , 2006 .

[21]  Pavel Ginzburg,et al.  Gap plasmon polariton structure for very efficient microscale-to-nanoscale interfacing. , 2006, Optics letters.

[22]  S. Kawata Near-Field Optics and Surface Plasmon Polaritons , 2001 .

[23]  Xiang Zhang,et al.  Local electric field enhancement during nanofocusing of plasmons by a tapered gap , 2007 .

[24]  Ewold Verhagen,et al.  Enhanced nonlinear optical effects with a tapered plasmonic waveguide. , 2007, Nano letters.

[25]  Dmitri K. Gramotnev,et al.  Adiabatic nanofocusing of plasmons by sharp metallic grooves: Geometrical optics approach , 2005 .

[26]  Dmitri K. Gramotnev,et al.  Adiabatic nano-focusing of plasmons by metallic tapered rods in the presence of dissipation , 2007 .