Impacts of Cloud Droplet-Nucleating Aerosols on Shallow Tropical Convection

Low-level warm-phase clouds cover a substantial portion of Earth’s oceans and play an important role in the global water and energy budgets. The characteristics of these clouds are controlled by the large-scale environment, boundary layer conditions, and cloud microphysics. Variability in the concentration of aerosols can alter cloud microphysical and precipitation processes that subsequently impact the system dynamics and thermodynamics and thereby create aerosol–cloud dynamic–thermodynamic feedback effects. In this study, three distinct cloud regimes were simulated, including stratocumulus, low-level cumulus (cumulus under stratocumulus), and deeper cumulus clouds. The simulations were conducted without environmental largescale forcing, thereby allowing all three cloud types to freely interact with the environmental state in an undamped fashion. Increases in aerosol concentration in these unforced, warm-phase, tropical cloud simulations lead to the production of fewer low-level cumuli; thinning and erosion of the widespread stratocumuluslayer;andthedevelopmentofdeeper,inversion-penetratingcumuli.Themechanismsforthesechanges are explored. Despite the development of deeper, more heavily precipitating cumuli, the reduction of the widespread moderately precipitating stratocumulus clouds leads to an overall reduction in domainwide accumulated precipitation when aerosol concentrations are enhanced.

[1]  R. Shaw,et al.  Measurements of Turbulent Mixing and Subsiding Shells in Trade Wind Cumuli , 2014 .

[2]  S. C. Heever,et al.  Developments in the CSU-RAMS Aerosol Model: Emissions, Nucleation, Regeneration, Deposition, and Radiation , 2013 .

[3]  S. C. Heever,et al.  Microphysical Processes Evident in Aerosol Forcing of Tropical Deep Convective Clouds , 2013 .

[4]  G. Stephens,et al.  Aerosol Indirect Effects on Tropical Convection Characteristics under Conditions of Radiative-Convective Equilibrium , 2011 .

[5]  T. L’Ecuyer,et al.  Impact of Cloud-Nucleating Aerosols in Cloud-Resolving Model Simulations of Warm-Rain Precipitation in the East China Sea , 2010 .

[6]  B. Khouider,et al.  The Deepening of Tropical Convection by Congestus Preconditioning , 2010 .

[7]  G. Stephens,et al.  Modeling Aerosol Impacts on Convective Storms in Different Environments , 2009 .

[8]  T. Takemura,et al.  Global observations of aerosol impacts on precipitation occurrence in warm maritime clouds , 2009 .

[9]  W. Cotton,et al.  Influence of cloud condensation and giant cloud condensation nuclei on the development of precipitating trade wind cumuli in a large eddy simulation , 2009 .

[10]  J. Penner,et al.  Aerosol effects on liquid‐water path of thin stratocumulus clouds , 2009 .

[11]  Guy N. Pearson,et al.  Vertical velocity variance and skewness in clear and cloud‐topped boundary layers as revealed by Doppler lidar , 2009 .

[12]  Christian D. Kummerow,et al.  Multisensor satellite observations of aerosol effects on warm clouds , 2008 .

[13]  Susan C. van den Heever,et al.  Evidence for the impact of aerosols on the onset and microphysical properties of rainfall from a combination of satellite observations and cloud‐resolving model simulations , 2008 .

[14]  A. Pokrovsky,et al.  Factors Determining the Impact of Aerosols on Surface Precipitation from Clouds: An Attempt at Classification , 2008 .

[15]  B. Stevens,et al.  The Structure and Mesoscale Organization of Precipitating Stratocumulus , 2008 .

[16]  Thijs Heus,et al.  A refined view of vertical mass transport by cumulus convection , 2008 .

[17]  B. Stevens,et al.  Aerosol effects on clouds, precipitation, and the organization of shallow cumulus convection , 2008 .

[18]  Kenneth Sassen,et al.  Classifying clouds around the globe with the CloudSat radar: 1‐year of results , 2008 .

[19]  A. Kostinski,et al.  Aerosols' influence on the interplay between condensation, evaporation and rain in warm cumulus cloud , 2007 .

[20]  Shepard A. Clough,et al.  Thin Liquid Water Clouds: Their Importance and Our Challenge , 2007 .

[21]  G. Feingold,et al.  Large-Eddy Simulations of Trade Wind Cumuli: Investigation of Aerosol Indirect Effects , 2006 .

[22]  Christian D. Kummerow,et al.  Rainfall Climate Regimes: The Relationship of Regional TRMM Rainfall Biases to the Environment , 2006 .

[23]  K. D. Beheng,et al.  A two-moment cloud microphysics parameterization for mixed-phase clouds. Part 2: Maritime vs. continental deep convective storms , 2006 .

[24]  Hongli Jiang,et al.  Effect of aerosol on warm convective clouds: Aerosol‐cloud‐surface flux feedbacks in a new coupled large eddy model , 2006 .

[25]  W. Cotton,et al.  A Large-Droplet Mode and Prognostic Number Concentration of Cloud Droplets in the Colorado State University Regional Atmospheric Modeling System (RAMS). Part II: Sensitivity to a Colorado Winter Snowfall Event , 2005 .

[26]  Ilan Koren,et al.  The effect of smoke, dust, and pollution aerosol on shallow cloud development over the Atlantic Ocean. , 2005, Proceedings of the National Academy of Sciences of the United States of America.

[27]  Y. Kaufman,et al.  Aerosol invigoration and restructuring of Atlantic convective clouds , 2005 .

[28]  Ming Zhao,et al.  Life Cycle of Numerically Simulated Shallow Cumulus Clouds. Part I: Transport , 2005 .

[29]  M. Kirkpatrick,et al.  The impact of humidity above stratiform clouds on indirect aerosol climate forcing , 2004, Nature.

[30]  Roger A. Pielke,et al.  Impact of aerosols and atmospheric thermodynamics on cloud properties within the climate system , 2004 .

[31]  Sonoyo Mukai,et al.  A study of the direct and indirect effects of aerosols using global satellite data sets of aerosol and cloud parameters , 2003 .

[32]  W. Cotton,et al.  Simulations of aerosol-cloud-dynamical feedbacks resulting from entrainment of aerosol into the marine boundary layer during the Atlantic Stratocumulus Transition Experiment , 2002 .

[33]  Ilan Levy,et al.  Relationship between synoptic‐scale atmospheric circulation and ozone concentrations over Israel , 2002 .

[34]  K.,et al.  Simulations of Trade Wind Cumuli under a Strong Inversion , 2001 .

[35]  Roger A. Pielke,et al.  Coupled Atmosphere–Biophysics–Hydrology Models for Environmental Modeling , 2000 .

[36]  B. Stevens,et al.  Efficient computation of vapor and heat diffusion between hydrometeors in a numerical model , 2000 .

[37]  W. Rossow,et al.  Advances in understanding clouds from ISCCP , 1999 .

[38]  B. Stevens,et al.  Large-Eddy Simulations of Strongly Precipitating, Shallow, Stratocumulus-Topped Boundary Layers , 1998 .

[39]  B. Stevens,et al.  Simulations of marine stratocumulus using a new microphysical parameterization scheme , 1998 .

[40]  William R. Cotton,et al.  New RAMS cloud microphysics parameterization. Part II: The two-moment scheme , 1997 .

[41]  W. Cotton,et al.  The Relationship between Drop In-Cloud Residence Time and Drizzle Production in Numerically Simulated Stratocumulus Clouds , 1996 .

[42]  D. Hartmann,et al.  The Effect of Cloud Type on Earth's Energy Balance: Global Analysis , 1992 .

[43]  D. Lenschow,et al.  Stratiform cloud formation in the marine boundary layer , 1991 .

[44]  R. Rotunno,et al.  Vertical-Velocity Skewness in the Buoyancy-Driven Boundary Layer , 1990 .

[45]  B. Albrecht Aerosols, Cloud Microphysics, and Fractional Cloudiness , 1989, Science.

[46]  Jorgen B. Jensen,et al.  A Study of the Source of Entrained Air in Montana Cumuli , 1988 .

[47]  G. Feingold,et al.  An Efficient Numerical Solution to the Stochastic Collection Equation , 1987 .

[48]  S. Twomey The Influence of Pollution on the Shortwave Albedo of Clouds , 1977 .

[49]  S. Twomey Pollution and the Planetary Albedo , 1974 .

[50]  E. Augstein,et al.  The vertical structure of the atmospheric planetary boundary layer in undisturbed trade winds over the Atlantic Ocean , 1974 .

[51]  H. Riehl,et al.  Mass and Energy Transports in an Undisturbed Atlantic Trade-Wind Flow , 1973 .

[52]  J. Smagorinsky,et al.  GENERAL CIRCULATION EXPERIMENTS WITH THE PRIMITIVE EQUATIONS , 1963 .

[53]  R. Wood,et al.  REVIEW Stratocumulus Clouds , 2012 .

[54]  Stephen G. Warren,et al.  A GRIDDED CLIMATOLOGY OF CLOUDS OVER LAND (1971-96) AND OCEAN (1954-97) FROM SURFACE OBSERVATIONS WORLDWIDE , 2007 .

[55]  William R. Cotton,et al.  A Large-Droplet Mode and Prognostic Number Concentration of Cloud Droplets in the Colorado State University Regional Atmospheric Modeling System (RAMS). Part I: Module Descriptions and Supercell Test Simulations , 2004 .

[56]  W. Cotton,et al.  RAMS 2001: Current status and future directions , 2003 .

[57]  J. Harrington,et al.  The effects of radiative and microphysical processes on simulated warm and transition season arctic stratus , 1997 .

[58]  Bruce A. Albrecht,et al.  A Model of the Thermodynamic Structure of the Trade-Wind Boundary Layer: Part II. Applications , 1979 .

[59]  H. Riehl,et al.  On the low-level wind structure in the Atlantic trade , 1974 .

[60]  H. Riehl,et al.  On the heat balance and maintenance of circulation in the trades , 1957 .