Mountain waves, polar stratospheric clouds, and the ozone depletion over Antarctica

We report observations of ozone column and clouds at typically stratospheric altitudes, obtained during the 1987 Airbone Antarctic Experiment from the TIROS Operational Vertical Sounder (TOVS)/High-Resolution Infrared Sounder (HIRS 2) instrument on the National Oceanic and Atmospheric Administration NOAA 10 satellite. Cloud formation occurs mainly along the coast of Antarctica when strong tropospheric winds blow from the ocean to the continent. The period of September 2–9 provides a good example of the formation of localized high-altitude clouds over the Palmer Peninsula and the Weddell Sea. The appearance of these clouds (a subset of the more prevalent polar stratospheric clouds (PSCs)) is consistent with the presence of a strong tropospheric jet over the elevated topography of the peninsula. Mountain waves and their associated high-altitude adiabatic cooling are the driving mechanism for the cloud formation. On the basis of the cloud area coverage and wind analyses, we estimate that in the altitude range 14–18 km the air within the polar vortex has spent 5% of its time inside these clouds from early August to late September. The importance of this observation for springtime ozone depletion mechanisms is discussed. It is also concluded that the TOVS data set recorded during the past decade would be suitable to search for a possible trend in the cloud amount. Such a trend could be relevant to the rate of the Antarctic ozone depletion.

[1]  S. Muller,et al.  Total ozone measurements derived from T.O.V.S. radiances , 1983 .

[2]  M. P. McCormick,et al.  Polar Stratospheric Cloud Sightings by SAM II , 1982 .

[3]  Stanley C. Solomon,et al.  Visible spectroscopy at McMurdo Station, Antarctica: 2. Observations of OClO , 1987 .

[4]  D. Golden,et al.  Reaction of Chlorine Nitrate with Hydrogen Chloride and Water at Antarctic Stratospheric Temperatures , 1987, Science.

[5]  J. Farman,et al.  Large losses of total ozone in Antarctica reveal seasonal ClOx/NOx interaction , 1985, Nature.

[6]  P. Crutzen,et al.  Nitric acid cloud formation in the cold Antarctic stratosphere: a major cause for the springtime ‘ozone hole’ , 1986, Nature.

[7]  R. Turco,et al.  Condensation of HNO3 and HCl in the winter polar stratospheres , 1986 .

[8]  M. McCormick,et al.  SAM II measurements of Antarctic PSC's and aerosols. [Stratospheric Aerosol Measurement satellite - Polar Stratospheric Clouds] , 1986 .

[9]  R. Stolarski,et al.  Nimbus 7 satellite measurements of the springtime Antarctic ozone  decrease , 1986, Nature.

[10]  M. McCormick,et al.  Characteristics of Arctic polar stratospheric clouds and as measured by airborne lidar , 1986 .

[11]  R. Stolarski Nimbus 7 SBUV/TOMS measurements of the springtime Antarctic ozone hole , 1986 .

[12]  M. Patrick McCormick,et al.  Polar stratospheric clouds and the Antarctic ozone hole , 1988 .

[13]  B. Gary Observational results using the microwave temperature profiler during the Airborne Antarctic Ozone Experiment , 1989 .

[14]  S. Wofsy,et al.  Reductions of Antarctic ozone due to synergistic interactions of chlorine and bromine , 1986, Nature.

[15]  A. Chedin,et al.  A Fast Line-by-Line Method for Atmospheric Absorption Computations: The Automatized Atmospheric Absorption Atlas , 1981 .

[16]  S. Solomon,et al.  On the depletion of Antarctic ozone , 1986, Nature.

[17]  John C. Gille,et al.  Implications of the stratospheric water vapor distribution as determined from the Nimbus 7 LIMS experiment. [Limb Infrared Monitor of Stratosphere] , 1984 .

[18]  A. Krueger,et al.  Analysis and comparison of ozone MAPS obtained by TOMS and TOVS during the MAP/GLOBUS 1983 campaign☆ , 1987 .

[19]  G. S. Kent,et al.  Airborne lidar observations of Arctic polar stratospheric clouds , 1986 .

[20]  D. J. Hofmann,et al.  Balloon-borne observations of the development and vertical structure of the Antarctic ozone hole in 1986 , 1987, Nature.

[21]  S. Fels,et al.  Antarctic ozone decreases: A dynamical cause? , 1986 .

[22]  K. Tung,et al.  Are Antarctic ozone variations a manifestation of dynamics or chemistry? , 1986, Nature.

[23]  M. Molina,et al.  Antarctic Stratospheric Chemistry of Chlorine Nitrate, Hydrogen Chloride, and Ice: Release of Active Chlorine , 1987, Science.