Two-photon excited whispering-gallery mode ultraviolet laser from an individual ZnO microneedle

Wurtzite structural ZnO microneedles with hexagonal cross section were fabricated by vapor-phase transport method and an individual microneedle was employed as a lasing microcavity. Under excitation of a femtosecond pulse laser with 800 nm wavelength, the ultraviolet (UV) laser emission was obtained, which presented narrow linewidth and high Q value. The UV emission, resonant mechanism, and laser mode characteristics were discussed in detail. The results demonstrated that the UV laser originated from the whispering-gallery mode induced by two-photon absorption assisted by Rabi oscillation.

[1]  Jun Wang,et al.  Femtosecond pulse excited two-photon photoluminescence and second harmonic generation in ZnO nanowires , 2006 .

[2]  V. L. Velichansky,et al.  Diode laser coupled to a high-Q microcavity via a GRIN lens , 2003 .

[3]  Thomas Halfmann,et al.  Efficient adiabatic population transfer by two-photon excitation assisted by a laser-induced Stark shift , 2000 .

[4]  Larry R. Dalton,et al.  Polymer micro-ring filters and modulators , 2002 .

[5]  A. Huston,et al.  Strain-sensitive elastic scattering from cylinders. , 1993, Optics letters.

[6]  Masashi Kawasaki,et al.  Room-temperature ultraviolet laser emission from self-assembled ZnO microcrystallite thin films , 1998 .

[7]  Masashi Kawasaki,et al.  Self-assembled ZnO nano-crystals and exciton lasing at room temperature , 2006 .

[8]  Ruibin Liu,et al.  Lasing mechanism of ZnO nanowires/nanobelts at room temperature. , 2006, The journal of physical chemistry. B.

[9]  Robert P. H. Chang,et al.  Random laser action in semiconductor powder , 1999 .

[10]  A. Bhowmik Polygonal optical cavities. , 2000, Applied optics.

[11]  M. Bozack,et al.  Lasing in whispering gallery mode in ZnO nanonails , 2006 .

[12]  Marius Grundmann,et al.  Whispering gallery mode lasing in zinc oxide microwires , 2008 .

[13]  W. Denk,et al.  Two-photon laser scanning fluorescence microscopy. , 1990, Science.

[14]  Nikita M. Bityurin,et al.  Two-photon pumped random laser in nanocrystalline ZnO , 2006 .

[15]  X. W. Sun,et al.  Field emission from gallium-doped zinc oxide nanofiber array , 2004 .

[16]  Kelly P. Knutsen,et al.  Single gallium nitride nanowire lasers , 2002, Nature materials.

[17]  M. Zhang,et al.  Structural and lasing characteristics of ultrathin hexagonal ZnO nanodisks grown vertically on silicon-on-insulator substrates , 2007 .

[18]  S. Yu,et al.  Room-Temperature Ultraviolet Lasing from Zinc Oxide Microtubes , 2003 .

[19]  Chunfeng Zhang,et al.  Multiphoton absorption pumped ultraviolet stimulated emission from ZnO microtubes , 2007 .

[20]  S. Ho,et al.  Optically-pumped ultraviolet microdisk laser on a silicon substrate , 2004, Conference on Lasers and Electro-Optics, 2004. (CLEO)..

[21]  J. Wiersig Hexagonal dielectric resonators and microcrystal lasers , 2002, physics/0210052.

[22]  Yiying Wu,et al.  Room-Temperature Ultraviolet Nanowire Nanolasers , 2001, Science.

[23]  M. Grundmann,et al.  Low-order optical whispering-gallery modes in hexagonal nanocavities (11 pages) , 2005 .

[24]  D A Parthenopoulos,et al.  Three-Dimensional Optical Storage Memory , 1989, Science.

[25]  Li Yang,et al.  Observation of two-photon-induced photoluminescence in ZnO microtubes , 2005 .

[26]  B. Su,et al.  Random laser action of ZnO@mesoporous silicas , 2008, Nanotechnology.