The simulation of aerosol transport over East Asia region

Abstract This study was carried out to understand the contribution of PM10 from China emission to Seoul Metropolitan Area (SMA) during high concentration period in January, 2007. The hourly PM10 concentration in Seoul Metropolitan Area had reached up to over 150 μg/m3 on 17th and 23rd of January in 2007. The aerosol transports from China along the Northwestern wind becomes the background concentrations in Korea and the assessment of the amount of contribution from China is very important in managing the air quality improvement plan in SMA. The U.S. EPA's Models-3/CMAQ (Community Multiscale Air Quality) was used to simulate PM10 concentration. The CMAQ performance was evaluated by comparing with the measurements in SMA for the episode period. The predictions were relatively in a good agreement with the measurements. The results show that the PM10 transport from China to Korea is significant and its contribution reaches up to 80% in the episode period. In order to assess more extensively the aerosol transport in East Asia region, the study to run the model in full year with speciated PM component measurements in super site is underway.

[1]  Christian Seigneur,et al.  Evaluation of three probing techniques in a three-dimensional air quality model , 2005 .

[2]  Yongtao Hu,et al.  Decoupled direct 3D sensitivity analysis for particulate matter (DDM-3D/PM) , 2006 .

[3]  H. Tanimoto,et al.  Analysis of the seasonal variation of ozone in the boundary layer in East Asia using the Community Multi-scale Air Quality model: What controls surface ozone levels over Japan? , 2006 .

[4]  C. N. Hewitt,et al.  A global model of natural volatile organic compound emissions , 1995 .

[5]  Henry E. Fuelberg,et al.  Uptake of nitrate and sulfate on dust aerosols during TRACE‐P , 2003 .

[6]  Michael Q. Wang,et al.  An inventory of gaseous and primary aerosol emissions in Asia in the year 2000 , 2003 .

[7]  Ki‐Hyun Kim,et al.  Temporal variation and cause of acidic precipitation from a monitoring network in Korea , 1996 .

[8]  William P. L. Carter,et al.  Condensed atmospheric photooxidation mechanisms for isoprene , 1996 .

[9]  O. Cooper,et al.  The 2001 Asian dust events: Transport and impact on surface aerosol concentrations in the U.S. , 2003 .

[10]  D. Reible,et al.  Flow and transport modeling in the sea-breeze. Part I: A modifiedE — ∈ model with a non-equilibrium level 2.5 closure , 1995 .

[11]  D. Reible,et al.  Flow and transport modeling in the sea-breeze part II: Flow model application and pollutant transport , 1995 .

[12]  T. Kitada,et al.  Simulated Semi-Global Scale Transport of SO 2 and SO 4 = from East Asia to the Northern Pacific in Spring Season: The Role of Low and High Pressure Systems , 1992 .

[13]  H. Dop Air pollution modeling and its application VI. , 1988 .

[14]  M. C. Dodge,et al.  A photochemical kinetics mechanism for urban and regional scale computer modeling , 1989 .

[15]  D. Byun Science algorithms of the EPA Models-3 community multi-scale air quality (CMAQ) modeling system , 1999 .

[16]  G. Grell,et al.  A description of the fifth-generation Penn State/NCAR Mesoscale Model (MM5) , 1994 .

[17]  M. C. Dodge A comparison of three photochemical oxidant mechanisms , 1989 .

[18]  Young-Joon Kim,et al.  An overview of ACE‐Asia: Strategies for quantifying the relationships between Asian aerosols and their climatic impacts , 2003 .

[19]  Hajime Akimoto,et al.  Intercontinental transport of ozone and its precursors in a three-dimensional global CTM , 2001 .