Effect of direct exchange on spin current scattering in Pd and Pt

Ultrathin films of the heavy elements Pd and Pt are widely used in spintronics as converters between charge and spin currents and vice versa. One open question has been whether the strongly paramagnetic nature of these elements influences the interconversion process. The authors show, using a combination of ferromagnetic resonance and x-ray magnetic circular dichroism measurements, that a related spin current absorption process (spin pumping damping) responds to the presence of ferromagnetic order in the polarizable Pd and Pt layers. They observe a change in the thickness dependence of spin current absorption when the Pd and Pt layers are in direct contact with a ferromagnet, compared with when they are in indirect contact. This change correlates with the presence of induced magnetic moments in Pd and Pt as revealed by element-specific x-ray magnetic circular dichroism magnetometry. The results show that the decoherence process for spin current in such layers is not independent of geometry, but rather is influenced by the presence of induced ferromagnetic order.