Global-scale atmosphere monitoring by in-service aircraft – current achievements and future prospects of the European Research Infrastructure IAGOS

The European Research Infrastructure IAGOS (In-service Aircraft for a Global Observing System) operates a global-scale monitoring system for atmospheric trace gases, aerosols and clouds utilising the existing global civil aircraft. This new monitoring infrastructure builds on the heritage of the former research projects MOZAIC (Measurement of Ozone and Water Vapour on Airbus In-service Aircraft) and CARIBIC (Civil Aircraft for the Regular Investigation of the Atmosphere Based on an Instrument Container). CARIBIC continues within IAGOS and acts as an important airborne measurement reference standard within the wider IAGOS fleet. IAGOS is a major contributor to the in-situ component of the Copernicus Atmosphere Monitoring Service (CAMS), the successor to the Global Monitoring for the Environment and Security – Atmospheric Service, and is providing data for users in science, weather services and atmospherically relevant policy. IAGOS is unique in collecting regular in-situ observations of reactive gases, greenhouse gases and aerosol concentrations in the upper troposphere and lowermost stratosphere (UTLS) at high spatial resolution. It also provides routine vertical profiles of these species in the troposphere over continental sites or regions, many of which are undersampled by other networks or sampling studies, particularly in Africa, Southeast Asia and South America. In combination with MOZAIC and CARIBIC, IAGOS has provided long-term observations of atmospheric chemical composition in the UTLS since 1994. The longest time series are 20 yr of temperature, H2O and O3, and 9–15 yr of aerosols, CO, NO y , CO2, CH4, N2O, SF6, Hg, acetone, ~30 HFCs and ~20 non-methane hydrocarbons. Among the scientific highlights which have emerged from these data sets are observations of extreme concentrations of O3 and CO over the Pacific basin that have never or rarely been recorded over the Atlantic region for the past 12 yr; detailed information on the temporal and regional distributions of O3, CO, H2O, NO y and aerosol particles in the UTLS, including the impacts of cross-tropopause transport, deep convection and lightning on the distribution of these species; characterisation of ice-supersaturated regions in the UTLS; and finally, improved understanding of the spatial distribution of upper tropospheric humidity including the finding that the UTLS is much more humid than previously assumed.

[1]  U. Schumann,et al.  Determination of humidity and temperature fluctuations based on MOZAIC data and parametrisation of persistent contrail coverage for general circulation models , 1997 .

[2]  John A. Pyle,et al.  Measurement of ozone and water vapor by Airbus in-service aircraft: The MOZAIC airborne program, an overview , 1998 .

[3]  D. Kley,et al.  Calibration and performance of automatic compact instrumentation for the measurement of relative humidity from passenger aircraft , 1998 .

[4]  Valerie Thouret,et al.  Comparisons of ozone measurements from the MOZAIC airborne program and the ozone sounding network at eight locations , 1998 .

[5]  Klaus Gierens,et al.  A distribution law for relative humidity in the upper troposphere and lower stratosphere derived from three years of MOZAIC measurements , 1999 .

[6]  Paul J. Crutzen,et al.  CARIBIC—Civil Aircraft for Global Measurement of Trace Gases and Aerosols in the Tropopause Region , 1999 .

[7]  Klaus Gierens,et al.  On the size distribution of ice-supersaturated regions in the upper troposphere and lowermost stratosphere , 2000 .

[8]  H. Schlager,et al.  Distributions of NO, NO x , and NO y in the upper troposphere and lower stratosphere between 28° and 61°N during POLINAT 2 , 2000 .

[9]  B. Doddridge,et al.  A tropical Atlantic Paradox: Shipboard and satellite views of a tropospheric ozone maximum and wave‐one in January–February 1999 , 2000 .

[10]  Paul J. Crutzen,et al.  Comparison between global chemistry transport model results and Measurement of Ozone and Water Vapor by Airbus In‐Service Aircraft (MOZAIC) data , 2000 .

[11]  A. Wiedensohler,et al.  Counting efficiency of condensation particle counters at low-pressures with illustrative data from the upper troposphere , 2001 .

[12]  J. Palutikof,et al.  Climate change 2007 : impacts, adaptation and vulnerability , 2001 .

[13]  Paul J. Crutzen,et al.  Budgets of O3 and CO in the upper troposphere: CARIBIC passenger aircraft results 1997–2001 , 2002 .

[14]  J. Heintzenberg,et al.  Meridional distributions of aerosol particle number concentrations in the upper troposphere and lower stratosphere obtained by Civil Aircraft for Regular Investigation of the Atmosphere Based on an Instrument Container (CARIBIC) flights , 2003 .

[15]  Frank Arnold,et al.  A Backward Modeling Study of Intercontinental Pollution Transport using Aircraft Measurements , 2003 .

[16]  Jean-Pierre Cammas,et al.  c ○ European Geosciences Union 2003 Atmospheric Chemistry and Physics Discussions , 2003 .

[17]  J. Gayet,et al.  On the distribution of relative humidity in cirrus clouds , 2004 .

[18]  A. Volz-Thomas,et al.  Measurements of total odd nitrogen (NO y ) aboard MOZAIC in-service aircraft: instrument design, operation and performance , 2004 .

[19]  V. Thouret,et al.  Tropospheric ozone over Equatorial Africa: regional aspects from the MOZAIC data , 2004 .

[20]  A. Stohl,et al.  Extreme CO concentrations in the upper troposphere over northeast Asia in June 2003 from the in situ MOZAIC aircraft data , 2005 .

[21]  Jean-Pierre Cammas,et al.  Mid-latitude tropospheric ozone columns from the MOZAIC program: climatology and interannual variability , 2005 .

[22]  V. Thouret,et al.  Tropopause referenced ozone climatology and inter-annual variability (1994–2003) from the MOZAIC programme , 2005 .

[23]  Hung N. Nguyen,et al.  Characteristics and origin of lowermost stratospheric aerosol at northern midlatitudes under volcanically quiescent conditions based on CARIBIC observations , 2005 .

[24]  V. Thouret,et al.  Enhanced view of the “tropical Atlantic ozone paradox” and “zonal wave one” from the in situ MOZAIC and SHADOZ data , 2006 .

[25]  H. Fischer,et al.  In-situ comparison of the NOy instruments flown in MOZAIC and SPURT , 2006 .

[26]  Hung N. Nguyen,et al.  Design and Calibration of a Multi-Channel Aerosol Sampler for Tropopause Region Studies from the CARIBIC Platform , 2006 .

[27]  Axel Lauer,et al.  Single‐particle measurements of midlatitude black carbon and light‐scattering aerosols from the boundary layer to the lower stratosphere , 2006 .

[28]  Paul J. Crutzen,et al.  Civil Aircraft for the regular investigation of the atmosphere based on an instrumented container: The new CARIBIC system , 2007 .

[29]  V. Thouret,et al.  Medium-range mid-tropospheric transport of ozone and precursors over Africa: two numerical case studies in dry and wet seasons , 2007 .

[30]  Klaus Gierens,et al.  Ice supersaturation in the ECMWF integrated forecast system , 2007 .

[31]  Hung N. Nguyen,et al.  The CARIBIC aircraft system for detailed, long-term, global-scale measurement of trace gases and aerosol in a changing atmosphere , 2007 .

[32]  S. Solomon The Physical Science Basis : Contribution of Working Group I to the Fourth Assessment Report of the Intergovernmental Panel on Climate Change , 2007 .

[33]  Herman G. J. Smit,et al.  Tropical Atlantic convection as revealed by ozone and relative humidity measurements , 2007 .

[34]  P. V. Velthoven,et al.  Influence of clouds on aerosol particle number concentrations in the upper troposphere , 2009 .

[35]  B. Martinsson,et al.  Analysis of C, N and O in aerosol collected on an organic backing using internal blank measurements and variable beam size , 2007 .

[36]  Richard H. Johnson,et al.  Ten Years of Measurements of Tropical Upper-Tropospheric Water Vapor by MOZAIC. Part I: Climatology, Variability, Transport, and Relation to Deep Convection , 2007 .

[37]  O. Cooper,et al.  Characterization of the composition, structure, and seasonal variation of the mixing layer above the extratropical tropopause as revealed by MOZAIC measurements , 2008 .

[38]  H. Smit,et al.  Statistical analysis of water vapour and ozone in the UT/LS observed during SPURT and MOZAIC , 2008 .

[39]  F. Slemr,et al.  Gaseous mercury distribution in the upper troposphere and lower stratosphere observed onboard the CARIBIC passenger aircraft , 2008 .

[40]  A. Stohl,et al.  Injection in the lower stratosphere of biomass fire emissions followed by long-range transport: a MOZAIC case study , 2008 .

[41]  Michaela I. Hegglin,et al.  A global view of the extratropical tropopause transition layer from Atmospheric Chemistry Experiment Fourier Transform Spectrometer O3, H2O, and CO , 2009 .

[42]  Franz Slemr,et al.  Greenhouse gas analysis of air samples collected onboard the CARIBIC passenger aircraft , 2009 .

[43]  D. C. Snyder,et al.  Single-Particle Measurements in Dearborn, Michigan , 2009 .

[44]  M. Saunois,et al.  An overview of two years of ozone radio soundings over Cotonou as part of AMMA , 2009 .

[45]  F. Slemr,et al.  Analysis of non-methane hydrocarbons in air samples collected aboard the CARIBIC passenger aircraft , 2009 .

[46]  S. Sherwood,et al.  A Matter of Humidity , 2009, Science.

[47]  B. Dix,et al.  Airborne multi-axis DOAS measurements of atmospheric trace gases on CARIBIC long-distance flights , 2009 .

[48]  Colm Sweeney,et al.  Civil Aviation Monitors Air Quality and Climate , 2009 .

[49]  V. Thouret,et al.  Lightning NOx influence on large-scale NOy and O3 plumes observed over the northern mid-latitudes , 2010 .

[50]  A. Stohl,et al.  Current status of the ability of the GEMS/MACC models to reproduce the tropospheric CO vertical distribution as measured by MOZAIC , 2010 .

[51]  A. Kunz Observation- and model-based study of the extratropical UT/LS , 2010 .

[52]  Andrew A. Lacis,et al.  Atmospheric CO2: Principal Control Knob Governing Earth’s Temperature , 2010, Science.

[53]  I. S. McDermid,et al.  Increasing springtime ozone mixing ratios in the free troposphere over western North America , 2010, Nature.

[54]  Christoph Weder,et al.  Atmospheric CO 2 : Principal Control Knob Governing Earth's Temperature , 2010 .

[55]  Characterization of non-methane hydrocarbons in Asian summer monsoon outflow observed by the CARIBIC aircraft , 2010 .

[56]  Louisa Emmons,et al.  Asian Monsoon Transport of Pollution to the Stratosphere , 2010, Science.

[57]  S. Solomon,et al.  Contributions of Stratospheric Water Vapor to Decadal Changes in the Rate of Global Warming , 2010, Science.

[58]  D. E. Harrison,et al.  Implementation Plan for the Global Observing System for Climate in Support of the UNFCCC (2010 Update) , 2010 .

[59]  A. Zahn,et al.  Acetone in the upper troposphere/lowermost stratosphere measured by the CARIBIC passenger aircraft: Distribution, seasonal cycle, and variability , 2010 .

[60]  S. Meunier,et al.  Comparison between global loudness and loudness change ratings for increasing sounds , 2010 .

[61]  Andrew Gettelman,et al.  THE EXTRATROPICAL UPPER TROPOSPHERE AND LOWER STRATOSPHERE , 2011 .

[62]  K. Schlote-Holubek,et al.  A fast and precise chemiluminescence ozone detector for eddy flux and airborne application , 2011 .

[63]  M. Saunois,et al.  Atmospheric composition of West Africa: highlights from the AMMA international program , 2011 .

[64]  P. V. Velthoven,et al.  Near-global aerosol mapping in the upper troposphere and lowermost stratosphere with data from the CARIBIC project , 2011 .

[65]  C. Brenninkmeijer,et al.  Investigation of chlorine radical chemistry in the Eyjafjallajökull volcanic plume using observed depletions in non‐methane hydrocarbons , 2011 .

[66]  F. Slemr,et al.  Carbon monoxide measurements onboard the CARIBIC passenger aircraft using UV resonance fluorescence , 2012 .

[67]  Sub‐micrometer aerosol particles in the upper troposphere/lowermost stratosphere as measured by CARIBIC and modeled using the MIT‐CAM3 global climate model , 2012 .

[68]  Martin Riese,et al.  Impact of uncertainties in atmospheric mixing on simulated UTLS composition and related radiative effects , 2012 .

[69]  Bengt G. Martinsson,et al.  Composition and evolution of volcanic aerosol from eruptions of Kasatochi, Sarychev and Eyjafjallajökull in 2008-2010 based on CARIBIC observations , 2012 .

[70]  J. Staehelin,et al.  Changes in ozone over Europe: Analysis of ozone measurements from sondes, regular aircraft (MOZAIC) and alpine surface sites , 2012 .

[71]  K. Rosenlof,et al.  Stratospheric water vapor feedback , 2013, Proceedings of the National Academy of Sciences.

[72]  M. Gallagher,et al.  The backscatter cloud probe – a compact low-profile autonomous optical spectrometer , 2013 .

[73]  Rebecca Reid,et al.  Cost-benefit studies for observing systems , 2014 .

[74]  M. Hermann,et al.  Sources of increase in lowermost stratospheric sulphurous and carbonaceous aerosol background concentrations during 1999–2008 derived from CARIBIC flights , 2014 .

[75]  A. Petzold,et al.  Technical Note: Reanalysis of upper troposphere humidity data from the MOZAIC programme for the period 1994 to 2009 , 2014 .

[76]  P. V. Velthoven,et al.  Pollution patterns in the upper troposphere over Europe and Asia observed by CARIBIC , 2014 .

[77]  J. Landgraf,et al.  Validation of nine years of MOPITT V5 NIR using MOZAIC/IAGOS measurements: biases and long-term stability , 2014 .

[78]  A. Petzold,et al.  Evaluation of the MOZAIC Capacitive Hygrometer during the airborne field study CIRRUS-III , 2014 .

[79]  C. Brenninkmeijer,et al.  Processes controlling water vapor in the upper troposphere/lowermost stratosphere: An analysis of 8 years of monthly measurements by the IAGOS‐CARIBIC observatory , 2014 .

[80]  A. Simmons,et al.  The Concept of Essential Climate Variables in Support of Climate Research, Applications, and Policy , 2014 .

[81]  Analysis of tropospheric ozone and carbon monoxide profiles over South America based on MOZAIC/IAGOS database and model simulations , 2015 .

[82]  Damien Boulanger,et al.  Instrumentation on commercial aircraft for monitoring the atmospheric composition on a global scale: the IAGOS system, technical overview of ozone and carbon monoxide measurements , 2015 .

[83]  J. Flaud,et al.  The first regular measurements of ozone, carbon monoxide and water vapour in the Pacific UTLS by IAGOS , 2015 .

[84]  H. Tanimoto,et al.  Consistency of tropospheric ozone observations made by different platforms and techniques in the global databases , 2015 .

[85]  H. Eskes,et al.  On the use of MOZAIC-IAGOS data to assess the ability of the MACC reanalysis to reproduce the distribution of ozone and CO in the UTLS over Europe , 2015 .

[86]  C. Mari,et al.  An upper tropospheric ‘ozone river’ from Africa to India during the 2008 Asian post-monsoon season , 2015 .

[87]  Volker Ebert,et al.  Quality assessment of MOZAIC and IAGOS capacitive hygrometers: insights from airborne field studies , 2015 .

[88]  M. Hermann,et al.  Influence of volcanic eruptions on midlatitude upper tropospheric aerosol and consequences for cirrus clouds , 2015 .

[89]  David W. Fahey,et al.  Challenges of a lowered U.S. ozone standard , 2015, Science.

[90]  T. Shaw,et al.  Circulation response to warming shaped by radiative changes of clouds and water vapour , 2015 .

[91]  V. Thouret,et al.  Climatology of NOy in the troposphere and UT/LS from measurements made in MOZAIC , 2015 .

[92]  A. Petzold,et al.  The IAGOS-CORE aerosol package: instrument design, operation and performance for continuous measurement aboard in-service aircraft , 2015 .

[93]  Patrick Minnis,et al.  Properties of small cirrus ice crystals from commercial aircraft measurements and implications for flight operations , 2015 .

[94]  V. Thouret,et al.  Characterizing tropospheric ozone and CO around Frankfurt between 1994–2012 based on MOZAIC-IAGOS aircraft measurements , 2015 .

[95]  C. Gerbig,et al.  The IAGOS-core greenhouse gas package: a measurement system for continuous airborne observations of CO2, CH4, H2O and CO , 2015 .

[96]  R. Forbes,et al.  Comparison of ECMWF analysis and forecast humidity data with CARIBIC upper troposphere and lower stratosphere observations , 2015 .

[97]  J. Vernier,et al.  Significant radiative impact of volcanic aerosol in the lowermost stratosphere , 2015, Nature Communications.