Memory effects and dynamics of optical bistability in CuCl

We study the time variation of the nonlinear absorption due to the creation of biexcitons by a high-intensity nanosecond pulsed laser in CuCl. We show that this variation is different at the beginning and at the end of the laser pulse. This memory effect depends on the photon energy and on the intensity of the laser beam. An explanation based on the time dependence of the population is suggested. We also make a time analysis of a bistable device composed of a sample of CuCl placed in a Fabry-Perot cavity. The switching times measured are of some hundredths of picoseconds. We stress the importance of the absorption present in the cavity and show that it may destroy the dispersive bistability. Finally, we give some trends of the spatial variation of hysteresis in the transverse section of the laser beam.

[1]  Bigot,et al.  Time evolution of the dielectric function in a three-level system under pulsed excitation. , 1985, Physical Review B (Condensed Matter).

[2]  J. B. Grun,et al.  The dispersion of excitons, polaritons and biexcitons in direct-gap semiconductors , 1985 .

[3]  B. Hönerlage,et al.  Optical bistability in CuCl , 1984, Philosophical Transactions of the Royal Society of London. Series A, Mathematical and Physical Sciences.

[4]  K. Bohnert,et al.  Plasma induced optical nonlinearities and optical bistability in CdS , 1984 .

[5]  J. Bigot,et al.  Dispersion and Absorption Anomalies in Three‐Level Systems , 1984 .

[6]  C. Bowden,et al.  Effects of mirror reflectivity in excitonic optical bistability , 1984 .

[7]  J. Bigot,et al.  On the Dielectric Function of Three‐Level Systems under High Excitation. II. Exciton—Biexciton Transitions and Population Effects in CuCl , 1984 .

[8]  T. Itoh,et al.  Relaxation Process of Excitonic Molecules in CuCl under the Two-Photon Resonant Excitation. I. Mutual Collision of Excitonic Molecules , 1984 .

[9]  J. Bigot,et al.  On the Dielectric Function of Three-Level Systems under High Excitation I. Theoretical Approach , 1984 .

[10]  H. Gibbs,et al.  Optical Nonlinearity and Bistability due to the Biexciton Two-Photon Resonance in CuCI , 1983, Topical Meeting on Optical Bistability.

[11]  J. Bigot,et al.  Energy and intensity dependence of renormalization effects in CuCl , 1983 .

[12]  I. Abram Nonlinear-optical properties of biexcitons: Single-beam propagation , 1983 .

[13]  A. Maruani,et al.  Calculation of the nonlinear dielectric function in semiconductors , 1982 .

[14]  Eitan Abraham,et al.  Optical bistability and related devices , 1982 .

[15]  N. Peyghambarian,et al.  Biexciton resonance linewidth in CuCl: Collision broadening or not? , 1982 .

[16]  D. Chemla,et al.  Nonlinear optical effects associated with excitonic-molecules in large gap semiconductors , 1982 .

[17]  Y. Masumoto,et al.  Superbroadened distribution of excitonic polaritons in CuCl , 1982 .

[18]  H. Haug Nonlinear optical phenomena and bistability in semiconductors , 1982 .

[19]  L. Lugiato Theory of Optical Bistability , 1982 .

[20]  N. Nagasawa,et al.  A Comment on the Broadening of the Excitonic Molecule Band in CuCl , 1981 .

[21]  E. Hanamura Optical bistable system responding in pico-second , 1981 .

[22]  H. Haug,et al.  Two-Photon Generation of Excitonic Molecules and Optical Bistability , 1981 .

[23]  H. Haug,et al.  Optical properties of dense exciton-biexciton systems , 1980 .

[24]  T. Kushida,et al.  Optical Studies of Resonantly Excited Excitonic Molecules in CuCl , 1978 .

[25]  L. Lugiato,et al.  Bistable absorption in a ring cavity , 1978 .

[26]  T. Itoh,et al.  Anomalous Dispersion of Excitonic Polariton Due to the Giant Two-Photon Absorption into Excitonic Molecule in CuCl , 1978 .