Light scattering from a magnetically tunable dense random medium with dissipation: ferrofluid

Abstract We present a semi-phenomenological treatment of light transmission through and its reflection from a ferrofluid which we regard as a magnetically tunable system of dense random dielectric scatterers with dissipation. Partial spatial ordering is introduced by the application of a transverse magnetic field that superimposes a periodic modulation on the dielectric randomness. This causes Bragg scattering that effectively enhances the scattering due to the disorder alone, and thus reduces the elastic mean free path towards Anderson localization. A theoretical treatment, based on invariant imbedding, gives a simultaneous decrease of the transmission and the reflection without change of incident linear polarisation as the spatial order is tuned magnetically to the Bragg condition, namely the light wave vector being equal to half the Bragg vector (Q). Our experimental observations are in qualitative agreement with these results. We have also given expressions for the transit (sojourn) time of the light, and for the light energy stored in the random medium under a steady illumination. The ferrofluid thus provides an interesting physical realization of effectively a “Lossy Anderson-Bragg” (LAB) cavity with which to study the effect of interplay of the spatial disorder, partial order and the dissipation on light transport. Given current interests in the light propagation, optical limiting and the storage of light in ferrofluids, the present work seems topical.

[1]  W. Margulis,et al.  A spectrally tunable microstructured optical fibre Bragg grating utilizing an infiltrated ferrofluid. , 2010, Optics express.

[2]  C. Hong,et al.  Optical switch devices using the magnetic fluid thin films , 1999 .

[3]  P. Bomans,et al.  Direct observation of dipolar chains in iron ferrofluids by cryogenic electron microscopy , 2003, Nature materials.

[4]  P. Anderson Absence of Diffusion in Certain Random Lattices , 1958 .

[5]  S. Nair,et al.  An optical limiter based on ferrofluids , 2008 .

[6]  V. S. Abraham,et al.  Magnetic field induced assembling of nanoparticles in ferrofluidic liquid thin films based on NixFe1−xFe2O4 , 2004 .

[7]  Effect of periodic background loss on grating spectra. , 2002, Applied optics.

[8]  R. Rosenbaum,et al.  Experimental study of the Ioffe-Regel criterion for amorphous indium oxide films , 1998 .

[9]  S. John,et al.  Localization of Light , 1991 .

[10]  H. Ramachandran,et al.  Comment on "experimental evidence of zero forward scattering by magnetic spheres". , 2008, Physical review letters.

[11]  Nieuwenhuizen,et al.  Theory for multiple light scattering from Rayleigh scatterers in magnetic fields. , 1996, Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics.

[12]  K. Parekh,et al.  Experimental evidence of zero forward scattering by magnetic spheres. , 2006, Physical review letters.

[13]  B. Raj,et al.  Light scattering in a magnetically polarizable nanoparticle suspension. , 2008, Physical review. E, Statistical, nonlinear, and soft matter physics.

[14]  P. Sheng,et al.  Introduction to Wave Scattering, Localization and Mesoscopic Phenomena. Second edition , 1995 .

[15]  John,et al.  Strong localization of photons in certain disordered dielectric superlattices. , 1987, Physical review letters.

[16]  R. Rammal,et al.  Invariant imbedding approach to localization. I. General framework and basic equations , 1987 .

[17]  P. Wachter,et al.  Optical properties of magnetite (Fe3O4) , 1979 .

[18]  Kumar Resistance fluctuation in a one-dimensional conductor with static disorder. , 1985, Physical review. B, Condensed matter.

[19]  Jian Li,et al.  Field modulation of light transmission through ferrofluid film , 2007 .

[20]  Yan Huang,et al.  Field–induced transmission of light in ionic ferrofluids of tunable viscosity , 2004 .