Full-color InGaN/GaN dot-in-a-wire light emitting diodes on silicon

We report on the achievement of a new class of nanowire light emitting diodes (LEDs), incorporating InGaN/GaN dot-in-a-wire nanoscale heterostructures grown directly on Si(111) substrates. Strong emission across nearly the entire visible wavelength range can be realized by varying the dot composition. Moreover, we have demonstrated phosphor-free white LEDs by controlling the indium content in the dots in a single epitaxial growth step. Such devices can exhibit relatively high internal quantum efficiency (>20%) and no apparent efficiency droop for current densities up to ~ 200 A cm(-2).

[1]  Hadis Morkoç,et al.  Surface band bending of a-plane GaN studied by scanning Kelvin probe microscopy , 2006 .

[2]  Seong-Ju Park,et al.  Improvement of efficiency droop in InGaN/GaN multiple quantum well light-emitting diodes with trapezoidal wells , 2010 .

[3]  Shuji Nakamura,et al.  Measurement of electron overflow in 450 nm InGaN light-emitting diode structures , 2009 .

[4]  Hiroto Sekiguchi,et al.  Emission color control from blue to red with nanocolumn diameter of InGaN/GaN nanocolumn arrays grown on same substrate , 2010 .

[5]  Xing Li,et al.  The effect of ballistic and quasi‐ballistic electrons on the efficiency droop of InGaN light emitting diodes , 2010 .

[6]  H. Kuo,et al.  Efficiency Enhancement and Beam Shaping of GaN–InGaN Vertical-Injection Light-Emitting Diodes via High-Aspect-Ratio Nanorod Arrays , 2009, IEEE Photonics Technology Letters.

[7]  E. Fred Schubert,et al.  Origin of efficiency droop in GaN-based light-emitting diodes , 2007 .

[8]  D. Kim,et al.  High-Brightness Light Emitting Diodes Using Dislocation-Free Indium Gallium Nitride/Gallium Nitride Multiquantum-Well Nanorod Arrays , 2004 .

[9]  P. Bhattacharya,et al.  Catalyst-free InGaN/GaN nanowire light emitting diodes grown on (001) silicon by molecular beam epitaxy. , 2010, Nano letters.

[10]  J. Ristić,et al.  Wurtzite GaN nanocolumns grown on Si(001) by molecular beam epitaxy , 2006 .

[11]  G A Botton,et al.  p-Type modulation doped InGaN/GaN dot-in-a-wire white-light-emitting diodes monolithically grown on Si(111). , 2011, Nano letters.

[12]  S. Denbaars,et al.  Optical and structural properties of GaN nanopillar and nanostripe arrays with embedded InGaN∕GaN multi-quantum wells , 2006 .

[13]  Rainer G. Ulbrich,et al.  Atomic and electronic structure of the nonpolar GaN ( 1 1 ¯ 00 ) surface , 2009 .

[14]  Chris G. Van de Walle,et al.  Microscopic origins of surface states on nitride surfaces , 2007 .

[15]  Hadis Morkoç,et al.  Hot electron effects on efficiency degradation in InGaN light emitting diodes and designs to mitigate them , 2010 .

[16]  P. Couturier Japan , 1988, The Lancet.

[17]  Zetian Mi,et al.  High efficiency green, yellow, and amber emission from InGaN/GaN dot-in-a-wire heterostructures on Si"111… , 2010 .

[18]  Liann-Be Chang,et al.  Effect of Electron Leakage on Efficiency Droop in Wide-Well InGaN-Based Light-Emitting Diodes , 2011 .

[19]  Shuji Nakamura,et al.  Quantum-confined Stark effect on photoluminescence and electroluminescence characteristics of InGaN-based light-emitting diodes , 2008 .

[20]  Charles M. Lieber,et al.  Gallium Nitride-Based Nanowire Radial Heterostructures for Nanophotonics , 2004 .

[21]  Chih-Min Chuang,et al.  Piezoelectric effects in the optical properties of strained InGaN quantum wells , 1999 .

[22]  Charles M. Lieber,et al.  Core/multishell nanowire heterostructures as multicolor, high-efficiency light-emitting diodes. , 2005, Nano letters.

[23]  E. Schubert,et al.  Polarization-matched GaInN∕AlGaInN multi-quantum-well light-emitting diodes with reduced efficiency droop , 2008 .

[24]  K. Kishino,et al.  InGaN/GaN Multiple Quantum Disk Nanocolumn Light-Emitting Diodes Grown on (111) Si Substrate , 2004 .

[25]  A. Azam,et al.  DNA interaction studies of new nano metal based anticancer agent: validation by spectroscopic methods , 2010, Nanotechnology.

[26]  Z. Mi,et al.  Molecular beam epitaxial growth and characterization of non-tapered InN nanowires on Si(111) , 2009, Nanotechnology.

[27]  S. Aloni,et al.  Complete composition tunability of InGaN nanowires using a combinatorial approach. , 2007, Nature materials.

[28]  H. Lüth,et al.  Nucleation and growth of GaN nanowires on Si(111) performed by molecular beam epitaxy. , 2007, Nano letters.