Site-selected Auger electron spectroscopy of N2O.

The N 1s Auger spectra for the two nonequivalent N atoms in N2O have been measured via Auger electron-photoelectron coincidence spectroscopy. The site-selected Auger spectra are compared with the normal Auger spectrum and with accurate theoretical calculations accounting for the effects of the dynamics of the nuclei on the energy and linewidth of the Auger bands. Such effects are found to be crucial factors in determining the different band shapes in the site-selected spectra.

[1]  K. Prince,et al.  Effects of nuclear dynamics in the low-kinetic-energy Auger spectra of CO and CO2. , 2005, The Journal of chemical physics.

[2]  Ian J. Bush,et al.  The GAMESS-UK electronic structure package: algorithms, developments and applications , 2005 .

[3]  M. Coreno,et al.  Photodouble ionization beyond the helium case , 2004 .

[4]  W. Stolte,et al.  Anionic and Cationic Photofragmentation of Core-Excited N2O , 2003 .

[5]  Marcello Coreno,et al.  The high resolution Gas Phase Photoemission beamline, Elettra , 1999 .

[6]  L. Cederbaum,et al.  Advances in the theoretical simulation of Auger spectra of polyatomic molecules: an example , 1995 .

[7]  A. Bianco,et al.  OPTIMIZATION OF SPHERICAL GRATING MONOCHROMATORS OPERATING WITH VARIABLE INCLUDED ANGLE FOR DIFFERENT APPLICATIONS , 1995 .

[8]  D. M. Hanson,et al.  Auger, zero-energy photoelectron, coincidence spectroscopy: Chemical-site-selective Auger electron spectroscopy , 1994 .

[9]  David E. Woon,et al.  Gaussian basis sets for use in correlated molecular calculations. IV. Calculation of static electrical response properties , 1994 .

[10]  L. Cederbaum,et al.  Nuclear dynamics of several decaying overlapping electronic states: A time-dependent formulation , 1993 .

[11]  L. Cederbaum,et al.  Nuclear dynamics of decaying states: A time‐dependent formulation , 1993 .

[12]  N. Kabachnik.  Angular correlation between photoelectron and Auger electron in two-step double photoionization of atoms , 1992 .

[13]  Kämmerling,et al.  Kämmerling and Schmidt reply. , 1992, Physical review letters.

[14]  Carlo Poloni,et al.  Status of the development of insertion devices for ELETTRA , 1992 .

[15]  L. Cederbaum,et al.  Band shape and vibrational structure in Auger spectra: Theory and application to carbon monoxide , 1991 .

[16]  W. Griffiths,et al.  Doubly ionized states of N2O studied by photon-induced Auger electron and double charge transfer spectroscopies , 1991 .

[17]  Schmidt,et al.  Complete fragmentation pattern for two-step double photoionization in xenon. , 1991, Physical review letters.

[18]  A. Kilcoyne,et al.  Angle‐resolved photoelectron spectroscopy of the core levels of N2O , 1991 .

[19]  L. Cederbaum,et al.  Many dicationic states and two-hole population analysis as a bridge to Auger spectra : strong localization phenomena in BF3 , 1991 .

[20]  D. M. Hanson.  Chemistry Induced by Core Electron Excitation , 2007 .

[21]  P. Millié,et al.  Potential energy surfaces of the low‐lying states of N2O++ and photodissociation mechanisms , 1990 .

[22]  B. Sonntag,et al.  Electron-electron coincidence studies of the decay of photoexcited rare gas core resonances , 1990 .

[23]  T. H. Dunning.  Gaussian basis sets for use in correlated molecular calculations. I. The atoms boron through neon and hydrogen , 1989 .

[24]  P. Millié,et al.  Electronic states and decay mechanisms of the N2O2+ dication , 1988 .

[25]  F. Larkins.  Interpretation of the Auger electron spectra of nitrous oxide , 1987 .

[26]  D. Urch,et al.  Auger electron spectroscopy , 1985 .

[27]  A. Barth,et al.  Higher-order approximations for the particle-particle propagator , 1984 .

[28]  H. Ågren.  On the interpretation of molecular valence Auger spectra , 1981 .

[29]  F. H. Read,et al.  Nitrogen K-shell excitation in N2, NO and N2O by high-resolution electron energy-loss spectroscopy , 1980 .

[30]  G. Sawatzky,et al.  AUGER-PHOTOELECTRON COINCIDENCE MEASUREMENTS IN COPPER , 1978 .

[31]  K. Nakamoto.  Infrared and Raman Spectra of Inorganic and Coordination Compounds , 1978 .

[32]  J. Kendrick,et al.  An experimental and theoretical study of the Auger spectrum of nitrous oxide , 1976 .

[33]  島内 みどり,et al.  G. Herzberg: Molecular Spectra and Molecular Structure. III. Electronic Spectra and Electronic Structure of Polyatomic Molecules, D. Van Nostrand, Prinston 1966, 745頁, 16.5×24cm, 8,000円. , 1968 .