Hot-electron photodetection with a plasmonic nanostripe antenna.

Planar metal-oxide-metal structures can serve as photodetectors that do not rely on the usual electron-hole pair generation in a semiconductor. Instead, absorbed light in one of the metals can produce a current of hot electrons when the incident photon energy exceeds the oxide barrier energy. Despite the desirable traits of convenient fabrication and room-temperature operation at zero bias of this type of device, the low power conversion efficiency has limited its use. Here, we demonstrate the benefits of reshaping one of the metallic contacts into a plasmonic stripe antenna. We use measurements of the voltage-dependence, spectral-dependence, stripe-width dependence, and polarization-dependence of the photocurrent to show that surface plasmon excitations can result in a favorable redistribution in the electric fields in the stripe that enhances the photocurrent. We also provide a theoretical model that quantifies the spectral photocurrent in terms of the electrical and optical properties of the junction. This model provides an accurate estimate of the bias dependence of the external quantum efficiency of different devices and shows that both the spatial and vectorial properties of the electric field distribution are important to its operation.

[1]  Yurii K. Gun'ko,et al.  Theory of Photoinjection of Hot Plasmonic Carriers from Metal Nanostructures into Semiconductors and Surface Molecules , 2013 .

[2]  N. Melosh,et al.  Power-independent wavelength determination by hot carrier collection in metal-insulator-metal devices , 2013, Nature Communications.

[3]  G. Konstantatos,et al.  Photoelectric energy conversion of plasmon-generated hot carriers in metal-insulator-semiconductor structures. , 2013, ACS nano.

[4]  Peter Nordlander,et al.  Embedding plasmonic nanostructure diodes enhances hot electron emission. , 2013, Nano letters.

[5]  Joseph Shappir,et al.  Waveguide based compact silicon Schottky photodetector with enhanced responsivity in the telecom spectral band. , 2012, Optics express.

[6]  N. Melosh,et al.  Plasmonic energy collection through hot carrier extraction. , 2011, Nano letters.

[7]  Naomi J. Halas,et al.  Photodetection with Active Optical Antennas , 2011, Science.

[8]  J A Bean,et al.  Performance Optimization of Antenna-Coupled ${\rm Al}/{\rm AlO}_{x}/{\rm Pt}$ Tunnel Diode Infrared Detectors , 2011, IEEE Journal of Quantum Electronics.

[9]  Pierre Berini,et al.  Thin-Film Schottky Barrier Photodetector Models , 2010, IEEE Journal of Quantum Electronics.

[10]  K. Saraswat,et al.  Nanometre-scale germanium photodetector enhanced by a near-infrared dipole antenna , 2008 .

[11]  S. Bozhevolnyi,et al.  Strip and gap plasmon polariton optical resonators , 2008 .

[12]  D. Diesing,et al.  Photo and particle induced transport of excited carriers in thin film tunnel junctions , 2007 .

[13]  Tzu-Ying Lin,et al.  Energy-band parameters of atomic-layer-deposition Al2O3/InGaAs heterostructure , 2006 .

[14]  C. Fumeaux,et al.  Lithographic antennas at visible frequencies. , 1999, Optics letters.

[15]  Moskovits,et al.  Light-induced kinetic effects in solids. , 1996, Physical review. B, Condensed matter.

[16]  T. Gaylord,et al.  Electron wave optics in semiconductors , 1989 .

[17]  J. Becher,et al.  Surface-plasmon-assisted photoemission , 1981 .

[18]  W. A. Dench,et al.  Quantitative electron spectroscopy of surfaces: A standard data base for electron inelastic mean free paths in solids , 1979 .

[19]  J. Whinnery,et al.  Characteristics of integrated MOM junctions at DC and at optical frequencies , 1978, IEEE Journal of Quantum Electronics.

[20]  W. E. Spicer,et al.  Negative affinity 3–5 photocathodes: Their physics and technology , 1977 .

[21]  William C. Brown,et al.  Optimization of the Efficiency and Other Properties of the Rectenna Element , 1976 .

[22]  J. Levinson,et al.  Photo-induced tunnel currents in Al-Al2O3-Au structures , 1975 .

[23]  S. M. Faris,et al.  Detection of optical and infrared radiation with DC-biased electron-tunneling metal-barrier-metal diodes , 1973 .

[24]  Vikram L. Dalal,et al.  Simple Model for Internal Photoemission , 1971 .

[25]  W. Spicer,et al.  Photoemission studies of the noble metals. II - Gold , 1970 .

[26]  W. Steinmann,et al.  Plasma Resonance in the Photoemission of Silver , 1968 .

[27]  E. Kane Simple Model for Collision Effects in Photoemission , 1966 .

[28]  Simon M. Sze,et al.  Range-energy relation of hot electrons in gold , 1964 .

[29]  W. E. Spicer,et al.  Photoemissive, Photoconductive, and Optical Absorption Studies of Alkali-Antimony Compounds , 1958 .

[30]  R. Fowler,et al.  The Analysis of Photoelectric Sensitivity Curves for Clean Metals at Various Temperatures , 1931 .