The α‐particle excited scintillation response of YAG:Ce thin films grown by liquid phase epitaxy

Y3Al5O12:Ce (YAG:Ce) thin films were grown from PbO‐, BaO‐, and MoO3‐based fluxes using the liquid phase epitaxy (LPE) method. Photoelectron yield, its time dependence within 0.5–10 μs shaping time, and energy resolution of these samples were measured under α‐particle excitation. For comparison a sample of the Czochralski grown bulk YAG:Ce single crystal was measured as well. Photoelectron yield values of samples grown from the BaO‐based flux were found superior to other LPE films and comparable with that of the bulk single crystal. The same is valid also for the time dependence of photoelectron yield. Obtained results are discussed taking into account the influence of the flux and technology used. Additionally, α particle energy deposition in very thin films is modelled and discussed. (© 2009 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)

[1]  M. Nikl,et al.  Ce-doped YAG and LuAG Epitaxial Films for Scintillation Detectors , 2008, IEEE Transactions on Nuclear Science.

[2]  A. Vedda,et al.  Scintillation Response Comparison Among Ce-Doped Aluminum Garnets, Perovskites and Orthosilicates , 2008, IEEE Transactions on Nuclear Science.

[3]  B. Sopko,et al.  High-resolution application of YAG:Ce and LuAG:Ce imaging detectors with a CCD X-ray camera , 2008 .

[4]  J. Tous,et al.  The α-particle excited scintillation response of the liquid phase epitaxy grown LuAG:Ce thin films , 2008 .

[5]  A. Makhov,et al.  Luminescence characteristics of Pb2+ centres in undoped and Ce3+-doped Lu3Al5O12 single-crystalline films and Pb2+→Ce3+ energy transfer processes , 2007 .

[6]  A. Vedda,et al.  Shallow traps and radiative recombination processes in Lu3Al5O12:Ce single crystal scintillator , 2007 .

[7]  M. Nikl,et al.  Scintillation and optical properties of YAG:Ce films grown by liquid phase epitaxy , 2007 .

[8]  A. Vedda,et al.  Energy transfer and charge carrier capture processes in wide‐band‐gap scintillators , 2007 .

[9]  R. Grimes,et al.  Extrinsic defect structure of RE3Al5O12 garnets , 2006 .

[10]  T. Martin,et al.  Recent developments in X-ray imaging with micrometer spatial resolution. , 2006, Journal of synchrotron radiation.

[11]  M. Nikl Scintillation detectors for x-rays , 2006 .

[12]  A. Vedda,et al.  The antisite LuAl defect‐related trap in Lu3Al5O12:Ce single crystal , 2005 .

[13]  M. Nikl Energy transfer phenomena in the luminescence of wide band‐gap scintillators , 2005 .

[14]  Y. Zorenko Luminescence of isoelectronic impurities and antisite defects in garnets , 2005 .

[15]  M. Maryško,et al.  Growth and characterization of high purity epitaxial yttrium iron garnet films grown from BaO-B2O3-BaF2 flux , 2003 .

[16]  M. Martini,et al.  Traps and Timing Characteristics of LuAG:Ce3+ Scintillator , 2000 .

[17]  M. Kuklja Defects in yttrium aluminium perovskite and garnet crystals: atomistic study , 2000 .

[18]  J. Tuli Nuclear Data Sheets Update for A = 137 , 1994 .

[19]  M. Moszynski,et al.  Properties of the YAG:Ce scintillator , 1994 .

[20]  Y. A. Akovali Nuclear Data Sheets Update for A = 241 , 1994 .

[21]  M. Schmorak Nuclear data sheets update for A = 239* , 1992 .

[22]  E. N. Shurshikov,et al.  Nuclear data sheets for A = 244 , 1981 .

[23]  R Autrata,et al.  A single crystal of YAG-new fast scintillator in SEM , 1978 .

[24]  M. I. Timoshechkin,et al.  Spectroscopic study of stoichiometry deviation in crystals with garnet structure , 1977 .

[25]  G. Scott,et al.  Pb valence in iron garnets , 1977 .

[26]  W. Bonner A novel non-Pb flux system for the preparation of yttrium and rare earth iron gallium and aluminum garnets , 1977 .

[27]  A. S. Penfold,et al.  Range-Energy Relations for Electrons and the Determination of Beta-Ray End-Point Energies by Absorption , 1952 .

[28]  W. H. Bragg,et al.  XXXIX. On the α particles of radium, and their loss of range in passing through various atoms and molecules , 1905 .

[29]  W. J. Henwood XLVI. Notice of a geological survey of the mines of Cornwall; with a programme of an intended arrangement of the leading details of the metalliferous veins, &c , 1831 .