Chaotic mixing induced by a magnetic chain in a rotating magnetic field.

Chaotic mixing, induced by breakup and reformation of a magnetic chain under the influence of a rotating magnetic field, is studied. A direct simulation method combining the Maxwell stress tensor and a fictitious domain method is employed to solve flows with suspended magnetic particles. The motion of the chain is significantly dependent on the Mason number (Ma), the ratio of viscous force to magnetic force. The degree of chaos is characterized by the maximum Lyapunov exponents. We also track the interface of two fluids in time and calculate the rate of stretching as it is affected by the Mason number. The progress of mixing is visualized via a tracer particle-tracking method and is characterized by the discrete intensity of segregation. Within a limited range of Mason number, a magnetic chain rotates and breaks into smaller chains, and the detached chains connect again to form a single chain. The repeating topological changes of the chain lead to the most efficient way of chaotic mixing by stretching at chain breakup and folding due to rotational flows.

[1]  Patrick Patrick Anderson,et al.  Morphology Development in Kenics Static Mixers (Application of the Extended Mapping Method) , 2008 .

[2]  T. G. Kang,et al.  Colored particle tracking method for mixing analysis of chaotic micromixers , 2004 .

[3]  H. Aref Stirring by chaotic advection , 1984, Journal of Fluid Mechanics.

[4]  R Calhoun,et al.  Paramagnetic particles and mixing in micro-scale flows. , 2006, Lab on a chip.

[5]  S. Quake,et al.  Microfluidics: Fluid physics at the nanoliter scale , 2005 .

[6]  T. H. Kwon,et al.  Enhancement of mixing performance of single‐screw extrusion processes via chaotic flows: Part I. Basic concepts and experimental study , 1996 .

[7]  Dong Sung Kim,et al.  A barrier embedded chaotic micromixer , 2004 .

[8]  James E. Martin,et al.  Chain model of a magnetorheological suspension in a rotating field , 2003 .

[9]  Patrick Patrick Anderson,et al.  Analyzing Mixing in Periodic Flows by Distribution Matrices: Mapping Method , 2001 .

[10]  M. Gijs,et al.  Manipulation of self-assembled structures of magnetic beads for microfluidic mixing and assaying. , 2004, Analytical chemistry.

[11]  P. V. Danckwerts The Difinition and Measurement of Some Characteristics of Mixtures , 1953 .

[12]  Darwin R. Reyes,et al.  Micro total analysis systems. 1. Introduction, theory, and technology. , 2002, Analytical chemistry.

[13]  R. Glowinski,et al.  A distributed Lagrange multiplier/fictitious domain method for particulate flows , 1999 .

[14]  Wook Ryol Hwang,et al.  Direct simulation of particle suspensions in sliding bi-periodic frames , 2004 .

[15]  H. Brenner,et al.  Body versus surface forces in continuum mechanics: is the Maxwell stress tensor a physically objective Cauchy stress? , 2002, Physical review. E, Statistical, nonlinear, and soft matter physics.

[16]  Peter R. C. Gascoyne,et al.  General expressions for dielectrophoretic force and electrorotational torque derived using the Maxwell stress tensor method , 1997 .

[17]  Fuller,et al.  Structure and dynamics of magnetorheological fluids in rotating magnetic fields , 2000, Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics.

[18]  Andreas Manz,et al.  On-chip free-flow magnetophoresis: continuous flow separation of magnetic particles and agglomerates. , 2004, Analytical chemistry.

[19]  N. Kasagi,et al.  A chaotic mixer for magnetic bead-based micro cell sorter , 2004, Journal of Microelectromechanical Systems.

[20]  I. Mezić,et al.  Chaotic Mixer for Microchannels , 2002, Science.

[21]  Nicole Pamme,et al.  Magnetism and microfluidics. , 2006, Lab on a chip.

[22]  Martin A. M. Gijs,et al.  Magnetic bead handling on-chip: new opportunities for analytical applications , 2004 .

[23]  S. Melle,et al.  Microstructure evolution in magnetorheological suspensions governed by Mason number. , 2003, Physical review. E, Statistical, nonlinear, and soft matter physics.

[24]  A. Gast,et al.  Rotational dynamics of semiflexible paramagnetic particle chains. , 2004, Physical review. E, Statistical, nonlinear, and soft matter physics.

[25]  Patrick Patrick Anderson,et al.  An adaptive front tracking technique for three-dimensional transient flows , 2000 .